ORCID Profile
0000-0002-5434-2247
Current Organisation
FRS-FNRS
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Environmental Monitoring | Inorganic Geochemistry | Geochemistry | Isotope Geochemistry
Effects of Climate Change and Variability on Australia (excl. Social Impacts) | Physical and Chemical Conditions of Water in Fresh, Ground and Surface Water Environments (excl. Urban and Industrial Use) |
Publisher: Copernicus GmbH
Date: 23-03-2020
DOI: 10.5194/EGUSPHERE-EGU2020-17416
Abstract: & & Inland waters (rivers, lakes and ponds) are important conduits for the emission of terrestrial carbon in Arctic permafrost landscapes. These emissions are driven by turnover of contemporary terrestrial carbon and additional & #8220 re-aged& #8221 (Holocene and late-Pleistocene) carbon released from thawing permafrost soils, but the magnitude of these source contributions to total inland water carbon fluxes remains unknown. Here we present unique simultaneous radiocarbon age measurements of inland water CO& sub& & /sub& , CH& sub& & /sub& and dissolved and particulate organic carbon in northeast Siberia during summer. We show that & % of total inland water carbon emissions were contemporary in age, but that pre-aged carbon contributed & % at sites strongly affected by permafrost thaw. CO& sub& & /sub& and CH& sub& & /sub& were younger than dissolved and particulate organic carbon, suggesting emissions were primarily fuelled by contemporary carbon decomposition. The study region was a net carbon sink (-876.9 & #177 136.4 Mg C for 25 July to 17 August), but inland waters were a source of contemporary (16.8 Mg C) and pre-aged (3.7 Mg C) emissions that respectively offset 1.9 & #177 1.2% and 0.4 & #177 0.3% of CO& sub& & /sub& uptake by tundra (& #8209 & #177 115 Mg C). Our findings reveal that inland water carbon emissions from permafrost landscapes may be more sensitive to changes in contemporary carbon turnover than the release of pre-aged carbon from thawing permafrost.& &
Publisher: Copernicus GmbH
Date: 25-02-2009
Abstract: Abstract. The coastal ocean is a crucial link between land, the open ocean and the atmosphere. The shallowness of the water column permits close interactions between the sedimentary, aquatic and atmospheric compartments, which otherwise are decoupled at long time scales (≅ 1000 yr) in the open oceans. Despite the prominent role of the coastal oceans in absorbing atmospheric CO2 and transferring it into the deep oceans via the continental shelf pump, the underlying mechanisms remain only partly understood. Evaluating observations from the North Sea, a NW European shelf sea, we provide evidence that anaerobic degradation of organic matter, fuelled from land and ocean, generates total alkalinity (AT) and increases the CO2 buffer capacity of seawater. At both the basin wide and annual scales anaerobic AT generation in the North Sea's tidal mud flat area irreversibly facilitates 7–10%, or taking into consideration benthic denitrification in the North Sea, 20–25% of the North Sea's overall CO2 uptake. At the global scale, anaerobic AT generation could be accountable for as much as 60% of the uptake of CO2 in shelf and marginal seas, making this process, the anaerobic pump, a key player in the biological carbon pump. Under future high CO2 conditions oceanic CO2 storage via the anaerobic pump may even gain further relevance because of stimulated ocean productivity.
Publisher: Copernicus GmbH
Date: 27-09-2023
Publisher: Copernicus GmbH
Date: 03-07-2014
Abstract: Abstract. A globally integrated carbon observation and analysis system is needed to improve the fundamental understanding of the global carbon cycle, to improve our ability to project future changes, and to verify the effectiveness of policies aiming to reduce greenhouse gas emissions and increase carbon sequestration. Building an integrated carbon observation system requires transformational advances from the existing sparse, exploratory framework towards a dense, robust, and sustained system in all components: anthropogenic emissions, the atmosphere, the ocean, and the terrestrial biosphere. The paper is addressed to scientists, policymakers, and funding agencies who need to have a global picture of the current state of the ( erse) carbon observations. We identify the current state of carbon observations, and the needs and notional requirements for a global integrated carbon observation system that can be built in the next decade. A key conclusion is the substantial expansion of the ground-based observation networks required to reach the high spatial resolution for CO2 and CH4 fluxes, and for carbon stocks for addressing policy-relevant objectives, and attributing flux changes to underlying processes in each region. In order to establish flux and stock diagnostics over areas such as the southern oceans, tropical forests, and the Arctic, in situ observations will have to be complemented with remote-sensing measurements. Remote sensing offers the advantage of dense spatial coverage and frequent revisit. A key challenge is to bring remote-sensing measurements to a level of long-term consistency and accuracy so that they can be efficiently combined in models to reduce uncertainties, in synergy with ground-based data. Bringing tight observational constraints on fossil fuel and land use change emissions will be the biggest challenge for deployment of a policy-relevant integrated carbon observation system. This will require in situ and remotely sensed data at much higher resolution and density than currently achieved for natural fluxes, although over a small land area (cities, industrial sites, power plants), as well as the inclusion of fossil fuel CO2 proxy measurements such as radiocarbon in CO2 and carbon-fuel combustion tracers. Additionally, a policy-relevant carbon monitoring system should also provide mechanisms for reconciling regional top-down (atmosphere-based) and bottom-up (surface-based) flux estimates across the range of spatial and temporal scales relevant to mitigation policies. In addition, uncertainties for each observation data-stream should be assessed. The success of the system will rely on long-term commitments to monitoring, on improved international collaboration to fill gaps in the current observations, on sustained efforts to improve access to the different data streams and make databases interoperable, and on the calibration of each component of the system to agreed-upon international scales.
Publisher: Springer Science and Business Media LLC
Date: 22-04-2020
DOI: 10.1038/S41467-020-16005-1
Abstract: An amendment to this paper has been published and can be accessed via a link at the top of the paper.
Publisher: Springer Science and Business Media LLC
Date: 06-2006
DOI: 10.1007/BF02784990
Publisher: Copernicus GmbH
Date: 06-02-2008
Abstract: Abstract. We compiled a large data-set from 22 cruises spanning from 1991 to 2003, of the partial pressure of CO2 (pCO2) in surface waters over the continental shelf (CS) and adjacent open ocean (43° to 46° S 145° to 150° E), south of Tasmania. Climatological seasonal cycles of pCO2 in the CS, the subtropical zone (STZ) and the subAntarctic zone (SAZ) are described and used to determine monthly pCO2 anomalies. These are used in combination with monthly anomalies of sea surface temperature (SST) to investigate inter-annual variations of SST and pCO2. Monthly anomalies of SST (as intense as 2°C) are apparent in the CS, STZ and SAZ, and are indicative of strong inter-annual variability that seems to be related to large-scale coupled atmosphere-ocean oscillations. Anomalies of pCO2 normalized to a constant temperature are negatively related to SST anomalies. A reduced winter-time vertical input of dissolved inorganic carbon (DIC) during phases of positive SST anomalies, related to a poleward shift of westerly winds, and a concomitant local decrease in wind stress is the likely cause of the negative relationship between pCO2 and SST anomalies. The observed pattern is an increase of the sink for atmospheric CO2 associated with positive SST anomalies, although strongly modulated by inter-annual variability of wind speed. Assuming that phases of positive SST anomalies are indicative of the future evolution of regional ocean biogeochemistry under global warming, we show using a purely observational based approach that some provinces of the Southern Ocean could provide a potential negative feedback on increasing atmospheric CO2.
Publisher: Springer Science and Business Media LLC
Date: 02-04-2020
DOI: 10.1038/S41467-020-15511-6
Abstract: Inland waters (rivers, lakes and ponds) are important conduits for the emission of terrestrial carbon in Arctic permafrost landscapes. These emissions are driven by turnover of contemporary terrestrial carbon and additional pre-aged (Holocene and late-Pleistocene) carbon released from thawing permafrost soils, but the magnitude of these source contributions to total inland water carbon fluxes remains unknown. Here we present unique simultaneous radiocarbon age measurements of inland water CO 2 , CH 4 and dissolved and particulate organic carbon in northeast Siberia during summer. We show that % of total inland water carbon was contemporary in age, but pre-aged carbon contributed % at sites strongly affected by permafrost thaw. CO 2 and CH 4 were younger than dissolved and particulate organic carbon, suggesting emissions were primarily fuelled by contemporary carbon decomposition. Our findings reveal that inland water carbon emissions from permafrost landscapes may be more sensitive to changes in contemporary carbon turnover than the release of pre-aged carbon from thawing permafrost.
Publisher: Copernicus GmbH
Date: 04-04-2013
Abstract: Abstract. As a response to public demand for a well-documented, quality controlled, publically available, global surface ocean carbon dioxide (CO2) data set, the international marine carbon science community developed the Surface Ocean CO2 Atlas (SOCAT). The first SOCAT product is a collection of 6.3 million quality controlled surface CO2 data from the global oceans and coastal seas, spanning four decades (1968–2007). The SOCAT gridded data presented here is the second data product to come from the SOCAT project. Recognizing that some groups may have trouble working with millions of measurements, the SOCAT gridded product was generated to provide a robust, regularly spaced CO2 fugacity (fCO2) product with minimal spatial and temporal interpolation, which should be easier to work with for many applications. Gridded SOCAT is rich with information that has not been fully explored yet (e.g., regional differences in the seasonal cycles), but also contains biases and limitations that the user needs to recognize and address (e.g., local influences on values in some coastal regions).
Publisher: American Geophysical Union (AGU)
Date: 09-05-2008
DOI: 10.1029/2007GB003052
Publisher: Springer Science and Business Media LLC
Date: 04-2021
Publisher: Copernicus GmbH
Date: 04-04-2013
Abstract: Abstract. A well-documented, publicly available, global data set of surface ocean carbon dioxide (CO2) parameters has been called for by international groups for nearly two decades. The Surface Ocean CO2 Atlas (SOCAT) project was initiated by the international marine carbon science community in 2007 with the aim of providing a comprehensive, publicly available, regularly updated, global data set of marine surface CO2, which had been subject to quality control (QC). Many additional CO2 data, not yet made public via the Carbon Dioxide Information Analysis Center (CDIAC), were retrieved from data originators, public websites and other data centres. All data were put in a uniform format following a strict protocol. Quality control was carried out according to clearly defined criteria. Regional specialists performed the quality control, using state-of-the-art web-based tools, specially developed for accomplishing this global team effort. SOCAT version 1.5 was made public in September 2011 and holds 6.3 million quality controlled surface CO2 data points from the global oceans and coastal seas, spanning four decades (1968–2007). Three types of data products are available: in idual cruise files, a merged complete data set and gridded products. With the rapid expansion of marine CO2 data collection and the importance of quantifying net global oceanic CO2 uptake and its changes, sustained data synthesis and data access are priorities.
Start Date: 06-2020
End Date: 12-2025
Amount: $354,935.00
Funder: Australian Research Council
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