ORCID Profile
0000-0001-8738-9837
Current Organisation
University of Tokyo
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Publisher: American Chemical Society (ACS)
Date: 23-03-2015
Abstract: For improvement of solar cell performance, it is important to make efficient use of near-infrared light, which accounts for ∼40% of sunlight energy. Here we introduce plasmonic Ag nanocubes (NCs) to colloidal PbS quantum dot/ZnO nanowire (PbS QD/ZnO NW) bulk-heterojunction solar cells, which are characterized by high photocurrents, for further improvement in the photocurrent and power conversion efficiency (PCE) in the visible and near-infrared regions. The Ag NCs exhibit strong far field scattering and intense optical near field in the wavelength region where light absorption of PbS QDs is relatively weak. Photocurrents of the solar cells are enhanced by the Ag NCs particularly in the range 700-1200 nm because of plasmonic enhancement of light absorption and possible facilitation of exciton dissociation. As a result of the optimization of the position and amount of Ag NCs, the PCE of PbS QD/ZnO NW bulk-heterojunction solar cells is improved from 4.45% to 6.03% by 1.36 times.
Publisher: Royal Society of Chemistry (RSC)
Date: 2011
DOI: 10.1039/C1NR10416K
Abstract: Photocurrents of a ruthenium dye-TiO(2) system are enhanced by gold nanoparticles (100 or 40 nm diameter) embedded in TiO(2). As dye-particle spacing decreases to 10 nm, enhancement factor and intensity of localized electric fields at the TiO(2) surface increase. A further decrease in the spacing suppresses the enhancement.
Publisher: Wiley
Date: 29-10-2015
Publisher: Royal Society of Chemistry (RSC)
Date: 2015
DOI: 10.1039/C5CC01020A
Abstract: Potentiometric and conductometric sensors based on localized surface plasmon resonance that do not require light to pass through the s le solution were developed and applied to coloured and turbid s les.
Publisher: Royal Society of Chemistry (RSC)
Date: 15-10-2013
DOI: 10.1039/C3CP53625D
Abstract: For improvement of the conversion efficiency of solar cells, it is important to make effective use of near-infrared light, which accounts for about 40% of sunlight energy. Although solar cells based on quantum dots (QDs) such as PbS have been studied for the use of near-infrared light, their photoabsorption is not necessarily sufficient. In this study, we coupled PbS QD-sensitized solar cells with plasmonic Au nanoparticles (NPs) as light-harvesting antennae. As a result, the photocurrents of the cells were enhanced in the visible and near-infrared regions (500-1200 nm) due to interparticle plasmon coupling of spherical Au NPs. The maximum enhancement factor was 6. We also found that the optimum QD-NP spacing is shorter and that the maximum enhancement factor is higher when smaller QDs are used. These results suggest that a negative effect, quenching via energy transfer from QD to NP, is less significant for smaller PbS QDs.
Publisher: American Chemical Society (ACS)
Date: 31-01-2013
DOI: 10.1021/JP3120836
Publisher: American Chemical Society (ACS)
Date: 25-07-2017
DOI: 10.1021/ACS.JPCLETT.7B01620
Abstract: Single plasmonic nanoparticles can potentially serve as optical sensors for detecting local refractive index changes. However, simultaneous monitoring of the scattering spectra from multiple nanoparticles is not practical. Here we perform potential-scanning localized surface plasmon resonance (LSPR) sensing. Gold nanorods are immobilized on an ITO electrode. Instead of collecting the full spectrum, as is done in conventional LSPR sensing, the electrode potential is scanned while the rod spectra are monitored at a single wavelength. We demonstrate that refractive index changes can be determined from single wavelength experiments and we further find that gold nanorod (NR) dimers exhibit higher refractive index sensitivities than single NRs in both potential-scanning and conventional wavelength-scanning based LSPR sensing.
No related grants have been discovered for Tetsu Tatsuma.