ORCID Profile
0000-0002-9022-6833
Current Organisation
University of Reading
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Publisher: American Meteorological Society
Date: 05-2015
DOI: 10.1175/BAMS-D-12-00245.1
Abstract: Air quality and heat are strong health drivers, and their accurate assessment and forecast are important in densely populated urban areas. However, the sources and processes leading to high concentrations of main pollutants, such as ozone, nitrogen dioxide, and fine and coarse particulate matter, in complex urban areas are not fully understood, limiting our ability to forecast air quality accurately. This paper introduces the Clean Air for London (ClearfLo www.clearflo.ac.uk) project’s interdisciplinary approach to investigate the processes leading to poor air quality and elevated temperatures. Within ClearfLo, a large multi-institutional project funded by the U.K. Natural Environment Research Council (NERC), integrated measurements of meteorology and gaseous, and particulate composition/loading within the atmosphere of London, United Kingdom, were undertaken to understand the processes underlying poor air quality. Long-term measurement infrastructure installed at multiple levels (street and elevated), and at urban background, curbside, and rural locations were complemented with high-resolution numerical atmospheric simulations. Combining these (measurement–modeling) enhances understanding of seasonal variations in meteorology and composition together with the controlling processes. Two intensive observation periods (winter 2012 and the Summer Olympics of 2012) focus upon the vertical structure and evolution of the urban boundary layer chemical controls on nitrogen dioxide and ozone production—in particular, the role of volatile organic compounds and processes controlling the evolution, size, distribution, and composition of particulate matter. The paper shows that mixing heights are deeper over London than in the rural surroundings and that the seasonality of the urban boundary layer evolution controls when concentrations peak. The composition also reflects the seasonality of sources such as domestic burning and biogenic emissions.
Publisher: Copernicus GmbH
Date: 05-06-2019
Abstract: Abstract. The Atmospheric Pollution and Human Health in a Chinese Megacity (APHH-Beijing) programme is an international collaborative project focusing on understanding the sources, processes and health effects of air pollution in the Beijing megacity. APHH-Beijing brings together leading China and UK research groups, state-of-the-art infrastructure and air quality models to work on four research themes: (1) sources and emissions of air pollutants (2) atmospheric processes affecting urban air pollution (3) air pollution exposure and health impacts and (4) interventions and solutions. Themes 1 and 2 are closely integrated and support Theme 3, while Themes 1–3 provide scientific data for Theme 4 to develop cost-effective air pollution mitigation solutions. This paper provides an introduction to (i) the rationale of the APHH-Beijing programme and (ii) the measurement and modelling activities performed as part of it. In addition, this paper introduces the meteorology and air quality conditions during two joint intensive field c aigns – a core integration activity in APHH-Beijing. The coordinated c aigns provided observations of the atmospheric chemistry and physics at two sites: (i) the Institute of Atmospheric Physics in central Beijing and (ii) Pinggu in rural Beijing during 10 November–10 December 2016 (winter) and 21 May–22 June 2017 (summer). The c aigns were complemented by numerical modelling and automatic air quality and low-cost sensor observations in the Beijing megacity. In summary, the paper provides background information on the APHH-Beijing programme and sets the scene for more focused papers addressing specific aspects, processes and effects of air pollution in Beijing.
Publisher: Elsevier BV
Date: 06-2019
Publisher: Copernicus GmbH
Date: 20-03-2015
Abstract: Abstract. Determining the contribution of wood smoke to air pollution in large cities such as London is becoming increasingly important due to the changing nature of domestic heating in urban areas. During winter, biomass burning emissions have been identified as a major cause of exceedances of European air quality limits. The aim of this work was to quantify the contribution of biomass burning in London to concentrations of PM2.5 and determine whether local emissions or regional contributions were the main source of biomass smoke. To achieve this, a number of biomass burning chemical tracers were analysed at a site within central London and two sites in surrounding rural areas. Concentrations of levoglucosan, elemental carbon (EC), organic carbon (OC) and K+ were generally well correlated across the three sites. At all the sites, biomass burning was found to be a source of OC and EC, with the largest contribution of EC from traffic emissions, while for OC the dominant fraction included contributions from secondary organic aerosols, primary biogenic and cooking sources. Source apportionment of the EC and OC was found to give reasonable estimation of the total carbon from non-fossil and fossil fuel sources based upon comparison with estimates derived from 14C analysis. Aethalometer-derived black carbon data were also apportioned into the contributions from biomass burning and traffic and showed trends similar to those observed for EC. Mean wood smoke mass at the sites was estimated to range from 0.78 to 1.0 μg m−3 during the c aign in January–February 2012. Measurements on a 160 m tower in London suggested a similar ratio of brown to black carbon (reflecting wood burning and traffic respectively) in regional and London air. Peaks in the levoglucosan and K+ concentrations were observed to coincide with low ambient temperature, consistent with domestic heating as a major contributing local source in London. Overall, the source of biomass smoke in London was concluded to be a background regional source overlaid by contributions from local domestic burning emissions. This could have implications when considering future emission control strategies during winter and may be the focus of future work in order to better determine the contributing local sources.
Publisher: American Meteorological Society
Date: 10-2017
Publisher: Springer Science and Business Media LLC
Date: 24-08-2021
DOI: 10.1007/S10546-021-00658-6
Abstract: Good representation of turbulence in urban canopy models is necessary for accurate prediction of momentum and scalar distribution in and above urban canopies. To develop and improve turbulence closure schemes for one-dimensional multi-layer urban canopy models, turbulence characteristics are investigated here by analyzing existing large-eddy simulation and direct numerical simulation data. A range of geometries and flow regimes are analyzed that span packing densities of 0.0625 to 0.44, different building array configurations (cubes and cuboids, aligned and staggered arrays, and variable building height), and different incident wind directions ( $$0^\\circ $$ 0 ∘ and $$45^\\circ $$ 45 ∘ with regards to the building face). Momentum mixing-length profiles share similar characteristics across the range of geometries, making a first-order momentum mixing-length turbulence closure a promising approach. In vegetation canopies turbulence is dominated by mixing-layer eddies of a scale determined by the canopy-top shear length scale. No relationship was found between the depth-averaged momentum mixing length within the canopy and the canopy-top shear length scale in the present study. By careful specification of the intrinsic averaging operator in the canopy, an often-overlooked term that accounts for changes in plan area density with height is included in a first-order momentum mixing-length turbulence closure model. For an array of variable-height buildings, its omission leads to velocity overestimation of up to $$17\\%$$ 17 % . Additionally, we observe that the von Kármán coefficient varies between 0.20 and 0.51 across simulations, which is the first time such a range of values has been documented. When driving flow is oblique to the building faces, the ratio of dispersive to turbulent momentum flux is larger than unity in the lower half of the canopy, and wake production becomes significant compared to shear production of turbulent momentum flux. It is probable that dispersive momentum fluxes are more significant than previously thought in real urban settings, where the wind direction is almost always oblique.
Location: United Kingdom of Great Britain and Northern Ireland
No related grants have been discovered for Janet Fraser Barlow.