ORCID Profile
0000-0003-2866-4944
Current Organisation
Australian National University
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In Research Link Australia (RLA), "Research Topics" refer to ANZSRC FOR and SEO codes. These topics are either sourced from ANZSRC FOR and SEO codes listed in researchers' related grants or generated by a large language model (LLM) based on their publications.
Geology | Soil Sciences | Land Capability And Soil Degradation | Instruments And Techniques | Geomorphology | Geochronology | Synchrotrons; Accelerators; Instruments and Techniques | Sedimentology | Climatology (Incl. Palaeoclimatology) | Atomic, Molecular, Nuclear, Particle and Plasma Physics | Geochemistry | Physical Geography and Environmental Geoscience | Applied Hydrology (Drainage, Flooding, Irrigation, Quality, Etc.) | Geochronology And Isotope Geochemistry | Exploration Geochemistry | Environmental Management And Rehabilitation | Archaeological Science | Marine Geoscience | Geochronology | Groundwater Hydrology | Isotope Geochemistry | Environmental Management | Land Capability and Soil Degradation | High Energy Astrophysics; Cosmic Rays | Nuclear Physics |
Land and water management | Climate change | Land and water management | Land and water management | Expanding Knowledge in the Earth Sciences | Expanding Knowledge in the Physical Sciences | Climate Variability (excl. Social Impacts) | Marine protected areas | Biological sciences | Climate variability | Land and water management | Oceanic processes (excl. climate related) | Farmland, Arable Cropland and Permanent Cropland Land Management | Forest and Woodlands Land Management | Other
Publisher: Elsevier BV
Date: 12-2016
DOI: 10.1016/J.JENVRAD.2016.09.015
Abstract: A comprehensive series of nuclear tests were carried out by the United States at Enewetak Atoll in the Marshall Islands, especially between 1952 and 1958. A Porites Lutea coral that was growing in the Enewetak lagoon within a few km of all of the high-yield tests contains a continuous record of isotopes, which are of interest (e.g.
Publisher: Elsevier BV
Date: 04-2010
Publisher: Elsevier BV
Date: 11-2006
Publisher: Elsevier BV
Date: 07-1985
Publisher: Elsevier BV
Date: 04-1984
Publisher: Elsevier BV
Date: 06-2007
Publisher: Elsevier BV
Date: 06-2014
DOI: 10.1016/J.JENVRAD.2014.02.022
Abstract: The variation of the (236)U and (239)Pu concentrations as a function of depth has been studied in a soil profile at a site in the Southern Hemisphere well removed from nuclear weapon test sites. Total inventories of (236)U and (239)Pu as well as the (236)U/(239)Pu isotopic ratio were derived. For this investigation a soil core from an undisturbed forest area in the Herbert River catchment (17°30' - 19°S) which is located in north-eastern Queensland (Australia) was chosen. The chemical separation of U and Pu was carried out with a double column which has the advantage of the extraction of both elements from a relatively large soil s le (∼20 g) within a day. The s les were measured by Accelerator Mass Spectrometry using the 14UD pelletron accelerator at the Australian National University. The highest atom concentrations of both (236)U and (239)Pu were found at a depth of 2-3 cm. The (236)U/(239)Pu isotopic ratio in fallout at this site, as deduced from the ratio of the (236)U and (239)Pu inventories, is 0.085 ± 0.003 which is clearly lower than the Northern Hemisphere value of ∼0.2. The (236)U inventory of (8.4 ± 0.3) × 10(11) at/m(2) was more than an order of magnitude lower than values reported for the Northern Hemisphere. The (239)Pu activity concentrations are in excellent agreement with a previous study and the (239+240)Pu inventory was (13.85 ± 0.29) Bq/m(2). The weighted mean (240)Pu/(239)Pu isotopic ratio of 0.142 ± 0.005 is slightly lower than the value for global fallout, but our results are consistent with the average ratio of 0.173 ± 0.027 for the southern equatorial region (0-30°S).
Publisher: American Physical Society (APS)
Date: 28-01-2015
Publisher: Elsevier BV
Date: 06-2004
Publisher: Elsevier BV
Date: 06-2013
Publisher: Elsevier BV
Date: 08-2004
Publisher: Elsevier BV
Date: 04-1991
Publisher: Elsevier BV
Date: 08-2004
Publisher: Elsevier BV
Date: 2018
Publisher: Elsevier BV
Date: 02-1983
Publisher: Wiley
Date: 2006
DOI: 10.1002/JQS.1075
Publisher: Elsevier BV
Date: 09-1977
Publisher: Elsevier BV
Date: 2010
Publisher: Elsevier BV
Date: 04-2009
DOI: 10.1016/J.JENVRAD.2008.12.016
Abstract: The present study applied sequential extraction techniques to investigate the binding and mobility of plutonium (Pu) in sediments from the rivers and estuaries of the Ob and Yenisey. As a study site, the Ob and Yenisey are particularly interesting as both rivers have weapons-grade Pu sources in their catchment areas, including the Russian Pu production and reprocessing plants at Mayak, Tomsk-7 and Krashnoyarsk, and the Semipalantinsk nuclear weapons testing site in Kazakhstan. Plutonium activity and (240)Pu/(239)Pu ratios were determined using accelerator mass spectrometry (AMS). Sequential extractions showed that between 47 and 80% of the Pu in Yenisey River sediments and 35-53% of the Pu in soils around the Techa River are mobilized with weak oxidising agents, which can indicate that Pu is bound to organic material. In contrast, Pu in Ob and Yenisey Estuarine sediments was more strongly bound, with 60-100% being found in the HNO(3)-extractable fraction. This change in speciation could reflect either that Pu bound to organic material in the Techa and Yenisey River sediments becomes more fixed to the sediments with time, or that organic-bound Pu is mobilized and released to the water when the sediments encounter the more saline water of the Ob and Yenisey estuaries. In general, (240)Pu/(239)Pu ratios were relatively consistent between different extraction fractions, although, in whole sediments, an increase in ratio was observed with distance from the source. This reflects the increased influence of weapon fallout from catchment runoff within the river systems, as compared to the weapons-grade sources close to the production and reprocessing plants. Knowledge of Pu speciation in the Ob and Yenisey Rivers, and the processes controlling its behaviour in estuarine systems, can improve predictions of its transfer and subsequent environmental impact to Arctic Seas.
Publisher: Elsevier BV
Date: 07-1985
Publisher: Elsevier BV
Date: 10-2015
Publisher: Elsevier BV
Date: 04-1985
Publisher: Elsevier BV
Date: 10-1983
Publisher: Elsevier BV
Date: 04-2010
Publisher: Elsevier BV
Date: 02-2008
DOI: 10.1016/J.JENVRAD.2007.10.019
Abstract: Following atmospheric nuclear weapons testing in the 1950s and 1960s significant quantities of (137)Cs and (239+240)Pu were deposited worldwide. In recent decades, (137)Cs has been commonly used as a tracer of soil erosion and sedimentation, particularly in the Northern Hemisphere where atomic deposition was three times as great as in the Southern Hemisphere. The relatively short 30-year half-life of this isotope means that its sensitivity as a tracer is rapidly decreasing. In contrast, with half-lives of 24,110 and 6561 years, the sensitivity of the two plutonium isotopes remains essentially the same as when it was deposited. Here we use the technique of Accelerator Mass Spectrometry to demonstrate the potential of anthropogenic Pu as an alternative to (137)Cs as a tracer of soil transport in Australia. We measure an average (137)Cs/(239+240)Pu activity ratio of 27.3+/-1.5 and an average (240)Pu/(239)Pu atom ratio of 0.149+/-0.003, both slightly lower than the global average.
Publisher: Elsevier BV
Date: 04-2010
Publisher: Elsevier BV
Date: 07-2015
Publisher: Geological Society of America
Date: 2009
DOI: 10.1130/G25042A.1
Publisher: Proceedings of the National Academy of Sciences
Date: 24-08-2020
Abstract: Nearby supernova explosions shape the interstellar medium. Ejecta, containing fresh nucleosynthetic products, may traverse the solar system as a transient passage, or alternatively the solar system may traverse local clouds that may represent isolated remnants of supernova explosions. Such scenarios may modulate the galactic cosmic-ray flux intensity to which Earth is exposed. Varying conditions of the traversed interstellar medium could have impacts on climate and can be imprinted in the terrestrial geological record. Some radionuclides, such as 60 Fe, are not produced on Earth or within the solar system in significant quantities. Their existence in deep-sea sediments demonstrates recent production in close-by supernova explosions with a continued influx of 60 Fe until today.
Publisher: Elsevier BV
Date: 06-1994
Publisher: Elsevier BV
Date: 1988
Publisher: Elsevier BV
Date: 10-2000
Publisher: Elsevier BV
Date: 08-2004
Publisher: Geological Society of America
Date: 2005
DOI: 10.1130/G21746.1
Publisher: Elsevier BV
Date: 08-2019
DOI: 10.1016/J.SCITOTENV.2019.04.251
Abstract: The
Publisher: Elsevier BV
Date: 04-1973
Publisher: American Physical Society (APS)
Date: 03-1993
Publisher: American Physical Society (APS)
Date: 04-1977
Publisher: Springer Science and Business Media LLC
Date: 16-07-2009
Publisher: Cambridge University Press (CUP)
Date: 2000
DOI: 10.1017/S0033822200030320
Abstract: Uranium series and radiocarbon ages were measured in corals from the uplifted coral terraces of Huon Peninsula (HP), Papua New Guinea, to provide a calibration for the 14 C time scale beyond 30 ka (kilo annum). Improved analytical procedures, and quantitative criteria for s le selection, helped discriminate diagenetically altered s les. The base-line of the calibration curve follows the trend of increasing ergence from calendar ages, as established by previous studies. Superimposed on this trend, four well-defined peaks of excess atmospheric radiocarbon were found ranging in magnitude from 100% to 700%, relative to current levels. They are related to episodes of sea-level rise and reef growth at HP. These peaks appear to be synchronous with Heinrich Events and concentrations of ice-rafted debris found in North Atlantic deep-sea cores. Relative timing of sea-level rise and atmospheric 14 C excess imply the following sequence of events: An initial sea-level high is followed by a large increase in atmospheric 14 C as the sea-level subsides. Over about 1800 years, the atmospheric radiocarbon drops to below present ambient levels. This cycle bears a close resemblance to ice-calving episodes of Dansgaard-Oeschger and Bond cycles and the slow-down or complete interruption of the North Atlantic thermohaline circulation. The increases in the atmospheric 14 C levels are attributed to the cessation of the North Atlantic circulation.
Publisher: Springer Science and Business Media LLC
Date: 30-07-2007
Publisher: Elsevier BV
Date: 11-1996
Publisher: Elsevier BV
Date: 07-2018
DOI: 10.1016/J.JENVRAD.2018.02.001
Abstract: The nuclear fuel reprocessing plants on the Sellafield site (UK) have released low-level effluents into the Irish Sea under authorisation since 1952. This has led to the labelling of nearby offshore sediments with a range of artificial radionuclides. In turn, these sediments act as a long-term secondary source of both soluble and particle-associated radionuclides to coastal areas. These radionuclides are of interest both in assessing possible environmental impacts and as tracers for marine processes. Here we present results from a study of the geochemistry of natural (
Publisher: Royal Society of Chemistry (RSC)
Date: 2001
DOI: 10.1039/B009764K
Abstract: 236U is produced only by neutron irradiation of uranium and therefore is potentially useful as a marker for anthropogenic uranium in the environment. Accelerator mass spectrometry (AMS) provides a technique for the determination of very low concentrations of actinide nuclides, and has now been applied to the determination of 236U:235U ratios in an intertidal sediment core collected from the North Irish Sea. Combining measurements of the 238U mass concentrations calculated from alpha spectrometry with 238U:235U ratios from ICP-MS and 236U:235U ratios from AMS has allowed the estimation of the mass concentrations of 236U in the sediments. 236U mass concentrations are in the range 10(-8) to 10(-9) g kg-1, and 236U:238U atom ratios in the range from 10(-5) to 10(-6), well above natural baseline levels. Uncertainties based on propagation of measurement errors were less than +/- 10% although +/- 15% is perhaps a more realistic estimate of overall uncertainty.
Publisher: Royal Society of Chemistry (RSC)
Date: 1997
DOI: 10.1039/A702002C
Abstract: Studies of the biological chemistry of aluminium can gain significantly from the use of the long-lived isotope 26Al as a tracer, although the cost of the isotope often precludes its determination by radiochemical counting techniques. Accelerator mass spectrometry (AMS) provides an ultra-sensitive method of determination, free from isobaric interference from atomic (26Mg) or molecular species. The source materials for AMS can be aluminium oxide or phosphate, both of which can be readily prepared at a sufficient level of purity from biological substrates. Natural aluminium (27Al, 100%) is added to the preparations as a chemical yield monitor and to provide the reference for the isotope ratio measurement. 26Al/27Al ratios can be determined over the range 10(-14)-10(-7), implying a limit of detection for 26Al of around 10(-18) g. The precision of measurement and long-term reproducibility are < 5% and < 7% (RSD), respectively. Chemical methodologies for routine measurements on blood and urine s les have been developed.
Publisher: Elsevier BV
Date: 2013
Publisher: American Association for the Advancement of Science (AAAS)
Date: 05-10-2007
Abstract: As the climate warmed at the end of the last glacial period, a rapid reversal in temperature, the Younger Dryas (YD) event, briefly returned much of the North Atlantic region to near full-glacial conditions. The event was associated with climate reversals in many other areas of the Northern Hemisphere and also with warming over and near Antarctica. However, the expression of the YD in the mid- to low latitudes of the Southern Hemisphere (and the southwest Pacific region in particular) is much more controversial. Here we show that the Waiho Loop advance of the Franz Josef Glacier in New Zealand was not a YD event, as previously thought, and that the adjacent ocean warmed throughout the YD.
Publisher: Elsevier BV
Date: 08-1976
Publisher: Elsevier BV
Date: 02-2017
Publisher: EDP Sciences
Date: 2012
Publisher: Elsevier BV
Date: 06-2007
Publisher: Elsevier BV
Date: 02-1993
Publisher: SAGE Publications
Date: 06-1998
Publisher: EDP Sciences
Date: 2012
Publisher: Springer Science and Business Media LLC
Date: 2001
Publisher: Elsevier BV
Date: 02-2011
Publisher: Elsevier BV
Date: 12-1990
Publisher: Elsevier BV
Date: 04-2002
Publisher: Elsevier BV
Date: 11-1987
Publisher: IOP Publishing
Date: 12-1991
Publisher: Informa UK Limited
Date: 1990
DOI: 10.3109/00365529009095526
Abstract: Simultaneous recordings of pressure and slow-wave activity were obtained from the sphincter of Oddi (SO) and the duodenum in anesthetized rabbits. Histographic analysis of the recordings was performed when the following criteria were fulfilled: 1) slow waves must be present in the EMG recordings from both compartments and 2) only pressure recordings with sufficient pressure activity (greater than 50 peaks in 10 min) would be considered. Of 12 animals fulfilling the criteria for histographic analysis of 4 channels, a common basic-mode activity was found in all channels in 9 animals (75%). Of three animals fulfilling the criteria for histographic analysis of three channels, a common basic-mode activity was seen in all channels in all animals (100%). A correlation between the litude of the slow waves and the litude of the elicited pressure peaks in the SO was significant at a 5% level or better in 12 animals (80%). In some of the animals episodes of low- litude pressure activity was observed in the SO, occurring synchronously with slow waves devoid of spike activity. It is concluded that rabbit SO and duodenum are paced by slow waves with a common basic-mode activity in most animals. Slow waves may not only be the chief determinant of the contractile rhythm but may also have a certain influence on the force of the in idual SO contractions. It is suggested that slow waves per se may be able to mediate contractile activity.
Publisher: Geological Society of America
Date: 2006
Publisher: Elsevier BV
Date: 09-1982
Publisher: IOP Publishing
Date: 06-1980
Publisher: American Physical Society (APS)
Date: 11-1984
Publisher: Wiley
Date: 2009
DOI: 10.1002/JQS.1179
Publisher: The Royal Society
Date: 15-01-2005
Abstract: Coral reefs in the southwest Indian Ocean cover an area of ca. 18530 km 2 compared with a global reef area of nearly 300000 km 2 . These regions are important as fishing grounds, tourist attractions and as a significant component of the global carbon cycle. The mass of calcium carbonate stored within Holocene neritic sediments is a number that we are only now beginning to quantify with any confidence, in stark contrast to the mass and sedimentation rates associated with pelagic calcium carbonate, which have been relatively well defined for decades. We report new data that demonstrate that the reefs at Rodrigues, like those at Réunion and Mauritius, only reached a mature state (reached sea level) by 2–3 ka: thousands of years later than most of the reefs in the Australasian region. Yet field observations show that the large lagoon at Rodrigues is already completely full of carbonate detritus (typical lagoon depth less than 1 m at low spring tide). The presence of aeolian dunes at Rodrigues indicates periodic exposure of past lagoons throughout the Pleistocene. The absence of elevated Pleistocene reef deposits on the island indicates that the island has not been uplifted. Most Holocene reefs are between 15 and 20 m in thickness and those in the southwest Indian Ocean appear to be consistent with this observation. We support the view that the CO 2 flux associated with coral–reef growth acts as a climate change lifier during deglaciation, adding CO 2 to a warming world. southwest Indian Ocean reefs could have added 7–10% to this global flux during the Holocene.
Publisher: American Physical Society (APS)
Date: 09-1976
Publisher: Elsevier BV
Date: 2001
Publisher: Elsevier BV
Date: 04-1983
Publisher: Elsevier BV
Date: 07-2008
Publisher: American Physical Society (APS)
Date: 06-1993
Publisher: Wiley
Date: 2005
DOI: 10.1002/ESP.1254
Publisher: Elsevier BV
Date: 08-2004
Publisher: Wiley
Date: 09-2019
DOI: 10.1111/MAPS.13378
Publisher: Elsevier BV
Date: 08-1983
Publisher: SAGE Publications
Date: 04-1998
DOI: 10.1191/095968398666797200
Abstract: Major postglacial rock slope failures are a common feature of the Scottish Highlands and other mountainous areas that were deglaciated at the end of the Pleistocene, but evaluation of the causes and triggers of failure has been hindered by a lack of reliable dating evidence. We report the result of a pilot study designed to establish the absolute age of a large postglacial rotational rockslide at The Storr on the Isle of Skye, Scotland, using 36 Cl surface exposure dating. Exposure ages of 6.3 ± 0.7 cal. ka BP and 6.6 ± 0.8 cal. ka BP were obtained for rock s les from two separate landslide blocks, giving an overall age estimate of 6.5 ± 0.5 cal. ka BP for rock slope failure at this site. This date is consistent with AMS radiocarbon dating of windblown sand derived from the failure scarp, and with previous inferences (based on relative dating evidence) concerning an early-Holocene age for most rock slope failures in the Scottish Highlands. The long time lag (. 7 ka) between deglaciation and failure suggests that progressive joint extension and shearing of rock bridges and asperities were of critical importance in conditioning failure, though a seismic trigger cannot be ruled out. The methodology of surface exposure dating in this context is described and its future potential assessed.
Publisher: Elsevier BV
Date: 02-1998
DOI: 10.1016/S0162-0134(97)10016-2
Abstract: Silicon is possibly important in human physiology in protecting against the toxic effects of aluminium, but the kinetics of uptake and excretion of silicic acid, the bioavailable form, are not well characterised. We have used 32Si as a tracer in a human uptake experiment to determine a gastrointestinal uptake factor for silicic acid, and to elucidate the kinetics of renal elimination. Urine collections were made for extending intervals from 2 to 12 h over 2 days following ingestion by a single human subject of a neutral silicic acid solution containing tracer levels of 32Si (t1/2 approximately 150 y). Silicon was isolated as SiO2 and the 32Si content determined by accelerator mass spectrometry (AMS), using a gas-filled magnet technique to eliminate a prolific isobaric interference from 32S. Silicon uptake appears to have been essentially complete within 2 h of ingestion. Elimination occurred by two simultaneous first-order processes with half-lives of 2.7 and 11.3 h, representing around 90% and 10%, respectively, of the total output. The rapidly eliminated 32Si was probably retained in the extracellular fluid volume, whilst the slower component may represent intracellular uptake and release. Elimination of absorbed 32Si was essentially complete after 48 h and was equivalent to 36% of the ingested dose. This establishes only a lower limit for gastrointestinal absorption as, although there was no evidence for longer term retention of additional 32Si, the possibility could not be excluded by these results.
Publisher: Elsevier BV
Date: 04-2010
Publisher: Elsevier BV
Date: 10-2015
Publisher: Geological Society of America
Date: 2006
Publisher: Elsevier BV
Date: 11-2017
DOI: 10.1016/J.APRADISO.2017.08.015
Abstract: Based on AMS analysis, it is shown that no Pu signals from the Fukushima accident could be discerned in marine sediments collected 1.5-57km away from the Fukushima Da-ichi power plant (FDNPP), which were clearly influenced by accident-derived radiocesium. The
Publisher: Elsevier BV
Date: 11-2009
DOI: 10.1016/J.JHEVOL.2009.01.003
Abstract: A robust timeframe for the extant cave deposits at Liang Bua, and for the river terraces in the adjoining Wae Racang valley, is essential to constrain the period of existence and time of extinction of Homo floresiensis and other biota that have been excavated at this hominin type locality. Reliable age control is also required for the variety of artifacts excavated from these deposits, and to assist in environmental reconstructions for this river valley and for the region more broadly. In this paper, we summarize the available geochronological information for Liang Bua and its immediate environs, obtained using seven numerical-age methods: radiocarbon, thermoluminescence, optically- and infrared-stimulated luminescence (collectively known as optical dating), uranium-series, electron spin resonance, and coupled electron spin resonance/uranium-series. We synthesize the large number of numerical age determinations reported previously and present additional age estimates germane to questions of hominin evolution and extinction.
Publisher: American Physical Society (APS)
Date: 16-09-1996
Publisher: Elsevier BV
Date: 07-2004
Publisher: Cambridge University Press (CUP)
Date: 2012
DOI: 10.1071/AS11070
Abstract: An enhanced concentration of 60 Fe was found in a deep ocean crust in 2004 in a layer corresponding to an age of ∼2 Myr. The confirmation of this signal in terrestrial archives as supernova-induced and the detection of other supernova-produced radionuclides is of great interest. We have identified two suitable marine sediment cores from the South Australian Basin and estimated the intensity of a possible signal of the supernova-produced radionuclides 26 Al, 53 Mn, 60 Fe, and the pure r -process element 244 Pu in these cores. The finding of these radionuclides in a sediment core might allow us to improve the time resolution of the signal and thus to link the signal to a supernova event in the solar vicinity ∼2 Myr ago. Furthermore, it gives us an insight into nucleosynthesis scenarios in massive stars, condensation into dust grains and transport mechanisms from the supernova shell into the solar system.
Publisher: Elsevier BV
Date: 04-2003
Publisher: Elsevier BV
Date: 11-1988
Publisher: American Geophysical Union (AGU)
Date: 24-08-2010
DOI: 10.1029/2008JF001187
Publisher: Elsevier BV
Date: 2002
Publisher: Elsevier BV
Date: 11-2008
Publisher: Springer Science and Business Media LLC
Date: 12-2002
Publisher: Elsevier BV
Date: 07-2004
Publisher: Elsevier BV
Date: 09-1996
Publisher: Elsevier BV
Date: 09-2007
Publisher: EDP Sciences
Date: 04-2012
Publisher: Elsevier BV
Date: 10-1994
Publisher: Elsevier BV
Date: 04-2010
Publisher: Proceedings of the National Academy of Sciences
Date: 26-08-2008
Abstract: Establishing the cause of past extinctions is critical if we are to understand better what might trigger future occurrences and how to prevent them. The mechanisms of continental late Pleistocene megafaunal extinction, however, are still fiercely contested. Potential factors contributing to their demise include climatic change, human impact, or some combination. On the Australian mainland, 90% of the megafauna became extinct by ≈46 thousand years (ka) ago, soon after the first archaeological evidence for human colonization of the continent. Yet, on the neighboring island of Tasmania (which was connected to the mainland when sea levels were lower), megafaunal extinction appears to have taken place before the initial human arrival between 43 and 40 ka, which would seem to exonerate people as a contributing factor in the extirpation of the island megafauna. Age estimates for the last megafauna, however, are poorly constrained. Here, we show, by direct dating of fossil remains and their associated sediments, that some Tasmanian megafauna survived until at least 41 ka (i.e., after their extinction on the Australian mainland) and thus overlapped with humans. Furthermore, a vegetation record for Tasmania spanning the last 130 ka shows that no significant regional climatic or environmental change occurred between 43 and 37 ka, when a land bridge existed between Tasmania and the mainland. Our results are consistent with a model of human-induced extinction for the Tasmanian megafauna, most probably driven by hunting, and they reaffirm the value of islands adjacent to continental landmasses as tests of competing hypotheses for late Quaternary megafaunal extinctions.
Publisher: Elsevier BV
Date: 11-2005
Publisher: Cambridge University Press (CUP)
Date: 03-2001
Abstract: Late Pleistocene glaciation of the Australian mainland was restricted to a small area of the southeastern highlands. Geomorphic mapping of the area and exposure dating using the in situ produced cosmogenic isotope 10 Be provides evidence for at least two distinct glaciations. The Early Kosciuszko glaciation consisted of a single glacier advance before 59,300 ± 5400 years ago (Snowy River Advance). The Late Kosciuszko glaciation comprised three glacier advances 32,000 ± 2500 (Headley Tarn Advance), 19,100 ± 1600 (Blue Lake Advance), and 16,800 ± 1400 years ago (Mt. Twynam Advance). The Early Kosciuszko glaciation was the most extensive and the Late Kosciuszko advances were progressively less extensive. These periods of glaciation in the highlands correspond to episodes of periglacial activity and peaks in lake levels and river discharge at lower elevations in southeastern Australia. Glacier advances on the Kosciuszko Massif correlate with advances in Tasmania, South America, and New Zealand and are broadly representative of hemispheric climate changes during the last glacial cycle.
Publisher: Elsevier BV
Date: 2009
Publisher: Elsevier BV
Date: 02-1996
Publisher: Elsevier BV
Date: 12-1983
Publisher: American Association for the Advancement of Science (AAAS)
Date: 06-11-2020
Abstract: Walczak et al. report that increases in Pacific Ocean ventilation and periods of rapid production of icebergs from the Cordilleran Ice Sheet during the last glacial period preceded episodic iceberg discharges into the Atlantic Ocean (see the Perspective by Jaeger and Shevenell). Marine sediments from the Gulf of Alaska show that increases in vertical mixing of the ocean there correspond with intense iceberg calving from the ice sheet that covered much of high-latitude western North America and that these changes occurred before the analogous Heinrich events in the North Atlantic. Thus, these Pacific climate system reorganizations may have been an early part of a cascade of dynamic climate events with global repercussions. Science , this issue p. 716 see also p. 662
Publisher: Cambridge University Press (CUP)
Date: 1999
DOI: 10.1017/S0033822200019482
Abstract: We present results that validate a new wet oxidation, stepped-combustion procedure for dating “old” charcoal s les. An acid–base–wet oxidation (ABOX) pretreatment procedure has been developed that is used in place of the conventional acid-base-acid (ABA) pretreatment. Combustions and graphitizations are performed in a vacuum line that is insulated from the atmosphere by a second backing vacuum to eliminate the risk of atmospheric leakage into the line at any stage of the procedure. Combustions are performed at 3 temperatures (330 °, 630 ° and 850 °) with a graphite target produced from the CO 2 evolved during each combustion step. In this way, the removal of any contamination can be monitored, and a high degree of confidence can be placed on the final age. The pretreatment, combustion, graphitization, and measurement blank for the procedure, based on the analysis of a “radiocarbon-dead” graphite, is 0.5 ± 0.5 μg C (1σ, n=14), equivalent to 0.04 ± 0.02 pMC or an “age” of approximately 60 ka for a 1 mg graphite target. Analyses of a “radiocarbon-dead” natural charcoal after ABOX pretreatment and stepped combustion suggest that the total blank (including contamination not removed by pretreatment) may be higher than for graphite, ranging up to 0.10 ± 0.02 pMC. Additional experiments confirm good agreement with accepted values for the international low- 14 C “New Kauri” standard (0.16–0.25 pMC). They also confirm excellent reproducibility, with 3 separate dates on different aliquots of a charcoal s le from Ngarrabullgan Cave (Queensland, Australia) ranging from 35.2 to 35.5 ka 14 C BP. It is also demonstrated that the ABOX pretreatment, in conjunction with the new vacuum line described here, is able to remove contamination not removed by the conventional ABA pretreatment, suggesting that the technique can be used to produce reliable 14 C dates on charcoal up to at least 50 ka.
Publisher: Elsevier BV
Date: 05-2002
Publisher: Elsevier BV
Date: 05-1997
Publisher: Elsevier BV
Date: 05-1991
Publisher: Elsevier BV
Date: 02-2006
Publisher: American Chemical Society (ACS)
Date: 02-09-2000
DOI: 10.1021/ES0009976
Publisher: Wiley
Date: 25-03-2020
DOI: 10.1111/AOR.13670
Publisher: Elsevier BV
Date: 10-2019
Publisher: Springer Science and Business Media LLC
Date: 2002
Publisher: American Geophysical Union (AGU)
Date: 24-10-2006
DOI: 10.1029/2006JF000461
Publisher: Informa UK Limited
Date: 03-10-2015
Publisher: Elsevier BV
Date: 05-1978
Publisher: Wiley
Date: 2005
DOI: 10.1002/ESP.1311
Publisher: Elsevier BV
Date: 09-2015
Publisher: Elsevier BV
Date: 10-1987
Publisher: Wiley
Date: 03-1998
Publisher: American Physical Society (APS)
Date: 12-1973
Publisher: Springer Science and Business Media LLC
Date: 17-08-2000
DOI: 10.1038/35021035
Abstract: During the Last Glacial Maximum, ice sheets covered large areas in northern latitudes and global temperatures were significantly lower than today. But few direct estimates exist of the volume of the ice sheets, or the timing and rates of change during their advance and retreat. Here we analyse four distinct sediment facies in the shallow, tectonically stable Bonaparte Gulf, Australia--each of which is characteristic of a distinct range in sea level--to estimate the maximum volume of land-based ice during the last glaciation and the timing of the initial melting phase. We use faunal assemblages and preservation status of the sediments to distinguish open marine, shallow marine, marginal marine and brackish conditions, and estimate the timing and the mass of the ice sheets using radiocarbon dating and glacio-hydro-isostatic modelling. Our results indicate that from at least 22,000 to 19,000 (calendar) years before present, land-based ice volume was at its maximum, exceeding today's grounded ice sheets by 52.5 x 10(6) km. A rapid decrease in ice volume by about 10% within a few hundred years terminated the Last Glacial Maximum at 19,000 +/- 250 years.
Publisher: Springer Science and Business Media LLC
Date: 27-06-2009
Publisher: Elsevier BV
Date: 12-1992
Publisher: Elsevier BV
Date: 02-2015
Publisher: Elsevier BV
Date: 2013
Publisher: Springer Science and Business Media LLC
Date: 2002
Publisher: Geological Society of London
Date: 03-1999
Publisher: Elsevier BV
Date: 04-2010
Publisher: Elsevier BV
Date: 06-2007
Publisher: Springer Science and Business Media LLC
Date: 06-01-2006
Publisher: Elsevier BV
Date: 05-2023
Publisher: Elsevier BV
Date: 2019
Publisher: Wiley
Date: 2007
DOI: 10.1002/ESP.1459
Publisher: Elsevier BV
Date: 08-2019
Publisher: Elsevier BV
Date: 03-2004
Publisher: Elsevier BV
Date: 04-1985
Publisher: Elsevier BV
Date: 12-1981
Publisher: Wiley
Date: 02-11-2015
Publisher: Elsevier BV
Date: 02-2009
Publisher: Cambridge University Press (CUP)
Date: 05-2004
DOI: 10.1016/J.YQRES.2004.02.004
Abstract: Moraines on Schnells Ridge, southwest Tasmania, have been dated using in situ 10 Be. An age of 19,400 ± 600 yr is indicated for the well-preserved innermost moraine from consistent measurements on four large quartzite boulders. This corresponds closely with exposure ages reported by T.T. Barrows et al. (2002, Quaternary Science Reviews 21, 159–173) for Last Glacial Maximum glacial features farther north in Tasmania and southeast Australia. In contrast, ages between 39,000 and 141,000 yr were obtained from a series of boulders on a more extensive outer moraine, indicating that this has had a more complex history.
Publisher: Elsevier BV
Date: 02-2004
Publisher: Elsevier BV
Date: 06-2007
Publisher: American Geophysical Union (AGU)
Date: 06-1994
DOI: 10.1029/94WR00161
Publisher: Elsevier BV
Date: 06-2007
Publisher: Cambridge University Press (CUP)
Date: 2004
DOI: 10.1017/S0033822200039734
Abstract: This study estimates the maximum and minimum degrees of autocompaction for radiocarbon-dated Holocene mangrove sediments in Singapore, in order to correct apparent sediment accretion rates for the effects of sediment compression due to autocompaction. Relationships developed for a suite of modern (surface) sediment s les between bulk density, particle-size distribution, and organic matter content were used to estimate the initial (uncompacted) bulk density of buried and variably compressed Holocene sediments, based on the grain-size distribution and organic matter content of the sediment. The difference between measured (compacted) and initial (uncompacted) bulk density of each buried sediment interval can be interpreted as the amount of length shortening experienced by each interval since burial. This allows the elevation of s les selected for 14 C dating to be corrected for the effects of autocompaction of the underlying sediment sequence, so that accurate estimates of vertical sediment accretion rates can be calculated. The 3 Holocene mangrove sequences analyzed and dated for this study ranged in age from 2000 to 8500 cal BP. The effects of autocompaction are significant, even in comparatively thin sequences, with subsidence of up to 56 cm calculated for carbon-dated s les presently 2 m above incompressible basement. The vertical sediment accretion rates for these mangrove sequences ranged from 0.99 to 6.84 mm/yr and carbon sequestration rates ranged from 0.9 to 1.7 t/ha/yr, all within the range observed for comparable Holocene and modern mangrove sediments elsewhere.
Publisher: Elsevier BV
Date: 08-2008
Publisher: AIP
Date: 2013
DOI: 10.1063/1.4792817
Publisher: S. Karger AG
Date: 2000
DOI: 10.1159/000017216
Abstract: Although chromosomal abnormalities underpin some early onset cases of familial Alzheimer’s disease (AD), most cases are sporadic and not associated with such abnormalities. Aluminium (Al) is a significant but controversial risk factor for sporadic AD, and studies have reported associations between Al and the principal pathological features of AD, senile plaques and neurofibrillary tangles. The present study measured gastrointestinal (GI) absorption of Al under normal dietary conditions using sup /sup Al tracer and accelerator mass spectrometry (AMS). Following overnight fast, 13 AD patients (aged 63–76 years) and 13 age-matched controls (aged 62–76 years) ingested a fruit drink containing 27 ng sup /sup Al. Plasma s les were obtained before and 1 h after the drink and from these the fraction of sup /sup Al absorbed across the GI tract was estimated. The GI tract rigorously excludes Al with only 0.06–0.1% of the ingested Al being absorbed. The mean fraction absorbed by AD subjects exceeded controls by a factor of 1.64 (p≤0.05, Anova). AMS is capable of determining sup –16 /sup g of sup /sup Al with many orders of magnitude more sensitivity than other techniques. Using this sensitivity, we have shown, under normal physiological conditions, that the ability of the GI tract to exclude Al is reduced in AD, possibly leading to greater systemic exposure to Al. Public health measures to limit Al dietary uptake or bioavailability may decrease the prevalence of AD in the community and should be considered.
Publisher: Elsevier BV
Date: 07-2000
Publisher: Elsevier BV
Date: 04-1983
Publisher: Elsevier BV
Date: 02-1974
Publisher: Elsevier BV
Date: 10-2005
Publisher: Elsevier BV
Date: 09-2015
Publisher: Elsevier BV
Date: 03-1997
Publisher: Elsevier BV
Date: 12-2014
DOI: 10.1016/J.JENVRAD.2014.07.008
Abstract: After the explosion of the Chernobyl Nuclear Power Plant in April 1986, contaminated material was buried in shallow trenches within the exclusion zone. A (90)Sr plume was evidenced downgradient of one of these trenches, trench T22. Due to its conservative properties, (36)Cl is investigated here as a potential tracer to determine the maximal extent of the contamination plume from the trench in groundwater. (36)Cl/Cl ratios measured in groundwater, trench soil water and leaf leachates are 1-5 orders of magnitude higher than the theoretical natural (36)Cl/Cl ratio. This contamination occurred after the Chernobyl explosion and currently persists. Trench T22 acts as an obvious modern point source of (36)Cl, however other sources have to be involved to explain such contamination. (36)Cl contamination of groundwater can be explained by dilution of trench soil water by uncontaminated water (rainwater or deep groundwater). With a plume extending further than that of (90)Sr, radionuclide which is impacted by retention and decay processes, (36)Cl can be considered as a suitable tracer of contamination from the trench in groundwater provided that modern release processes of (36)Cl from trench soil are better characterized.
Publisher: Elsevier BV
Date: 2019
Publisher: Informa UK Limited
Date: 18-05-2016
Publisher: American Association for the Advancement of Science (AAAS)
Date: 02-07-1999
DOI: 10.1126/SCIENCE.285.5424.85
Abstract: Two main types of material survive from the Canyon Diablo impactor, which produced Meteor Crater in Arizona: iron meteorites, which did not melt during the impact and spheroids, which did. Ultrasensitive measurements using accelerator mass spectrometry show that the meteorites contain about seven times as much nickel-59 as the spheroids. Lower average nickel-59 contents in the spheroids indicate that they typically came from 0.5 to 1 meter deeper in the impactor than did the meteorites. Numerical modeling for an impact velocity of 20 kilometers per second shows that a shell 1.5 to 2 meters thick, corresponding to 16 percent of the projectile volume, remained solid on the rear surface that most of the projectile melted and that little, if any, vaporized.
Publisher: IOP Publishing
Date: 03-1978
Publisher: Elsevier BV
Date: 12-2006
Publisher: Elsevier BV
Date: 06-2007
Publisher: Springer Science and Business Media LLC
Date: 06-1992
DOI: 10.1007/BF01291696
Publisher: Elsevier BV
Date: 2013
Publisher: IOP Publishing
Date: 04-1979
Publisher: American Chemical Society (ACS)
Date: 27-10-2004
DOI: 10.1021/ES0492900
Abstract: Ice cores from glaciers situated near anthropogenic sources of air pollution provide important archives of the emissions of species with short atmospheric lifetimes. Here we present the history of atmospheric Pu fallout reconstructed from an ice core from the Belukha glacier in the Siberian Altai. Fourteen ice core s les covering the time period 1941-1986 were selected for Pu analysis, chemically processed, and measured using accelerator mass spectrometry. The Pu concentration peaks in 1963, coinciding with the maximum of the nuclear weapons tests and in concordance with the 3H activity concentration peak. The shapes of the 239Pu and 3H profiles reflect two main periods of atmospheric nuclear test activity: premoratorium testing before 1958 and postmoratorium testing in 1961 and 1962. Premoratorium tests contribute about 45% of the integrated Pu inventory. The average 240Pu/239Pu isotopic ratio is 0.18 +/- 0.05, indicating that a large majority of the Pu in the Belukha glacier originates from global stratospheric fallout rather than from direct tropospheric input.
Publisher: EDP Sciences
Date: 2015
Publisher: EDP Sciences
Date: 2015
Publisher: American Physical Society (APS)
Date: 11-1974
Publisher: Cambridge University Press (CUP)
Date: 2008
DOI: 10.1017/S003382220004337X
Abstract: We report radiocarbon ages on cellulose isolated from the gut contents of a Diprotodon found at Lake Callabonna, South Australia. The maximum age obtained corresponds to a minimum age of ,400 BP for this extinct giant marsupial. This is older than, and hence consistent with, the generally accepted Australian megafauna extinction window. We argue that dichromate and other strong oxidants are less selective than chlorite for lignin destruction in wood, and our results suggest that ages approaching laboratory background can be obtained using a repeated pretreatment sequence of chlorite-alkali-acid and measurement of the sometimes discarded 330°C combustion fraction.
Publisher: Elsevier BV
Date: 11-2017
DOI: 10.1016/J.JENVRAD.2017.05.009
Abstract: A slice from a Porites Lutea coral core collected inside the Enewetak Atoll lagoon, within 15 km of all major nuclear tests conducted at the atoll, was analysed for
Publisher: Elsevier BV
Date: 09-2019
DOI: 10.1016/J.JENVRAD.2019.05.003
Abstract: Anthropogenic radionuclides, like
Publisher: IOP Publishing
Date: 30-07-1999
Publisher: Wiley
Date: 2001
DOI: 10.1002/JQS.643
Publisher: American Association for the Advancement of Science (AAAS)
Date: 09-05-2008
Abstract: Barrows et al . (Reports, 5 October 2007, p. 86) presented cosmogenic exposure dates and data from an ocean sediment core that challenge evidence for glacier advance in New Zealand during the Younger Dryas event. We use modeling of geomorphic processes to argue that their cosmogenic exposure dates are inconclusive.
Publisher: American Physical Society (APS)
Date: 12-1973
Publisher: Geological Society of America
Date: 09-2010
DOI: 10.1130/G31066.1
Publisher: Elsevier BV
Date: 06-2012
Publisher: Elsevier BV
Date: 10-1978
Publisher: Elsevier BV
Date: 1980
Publisher: Elsevier BV
Date: 10-1993
Publisher: SAGE Publications
Date: 02-06-2021
DOI: 10.1177/15266028211016431
Abstract: To compare the flow patterns and hemodynamics of the AFX stent-graft and the covered endovascular reconstruction of aortic bifurcation (CERAB) configuration using laser particle image velocimetry (PIV) experiments. Two anatomically realistic aortoiliac phantoms were constructed using polydimethylsiloxane polymer. An AFX stent-graft with a transparent cover made with a new method was inserted into one phantom. A CERAB configuration using Atrium’s Avanta V12 with transparent covers made with a previously established method was inserted into the other phantom, both modified stent-grafts were suitable for laser PIV, enabling visualization of the flow fields and quantification of time average wall shear stress (TAWSS), oscillatory shear index (OSI), and relative residence time (RRT). Disturbed flow was observed at the bifurcation region of the AFX, especially at the end systolic velocity (ESV) time-point where recirculation was noticeable due to vortical flow. In contrast, predominantly unidirectional flow was observed at the CERAB bifurcation. These observations were confirmed by the quantified hemodynamic results from PIV analysis where mean TAWSS of 0.078 Pa (range: 0.009–0.242 Pa) was significantly lower in AFX as compared with 0.229 Pa (range: 0.013–0.906 Pa) for CERAB (p .001). Mean OSI of 0.318 (range: 0.123–0.496) in AFX was significantly higher than 0.252 (range: 0.055–0.472) in CERAB (p .001). Likewise, mean RRT of 180 Pa −1 (range: 9–3603 Pa −1 ) in AFX was also significantly higher than 88 Pa −1 (range: 2–840 Pa −1 ) in CERAB (p=0.0086). In this in vitro study, the flow pattern of a modified AFX stent-graft was found to be more disturbed especially at the end systolic phase, its hemodynamic outcomes less desirable than CERAB configuration. While the AFX stent-graft has an advantage over the CERAB configuration in eliminating radial mismatch, and maintaining the anatomical bifurcation for future endovascular intervention, this in vitro study revealed that the associated lower TAWSS, higher OSI and RRT may predispose to thrombosis and are, thus, less desirable as compared to a CERAB configuration. Further investigation is warranted to confirm whether these findings translate into the clinical setting.
Publisher: Elsevier BV
Date: 09-2011
Publisher: Springer Science and Business Media LLC
Date: 08-1999
Publisher: Elsevier BV
Date: 06-1994
Publisher: EDP Sciences
Date: 2013
Publisher: EDP Sciences
Date: 2013
Publisher: Elsevier BV
Date: 11-2022
Publisher: EDP Sciences
Date: 2013
Publisher: Elsevier BV
Date: 06-1989
Publisher: Elsevier BV
Date: 08-2004
Publisher: Springer Science and Business Media LLC
Date: 17-03-2017
DOI: 10.1038/SREP44679
Abstract: Unusually high concentrations of americium and plutonium have been observed in a sediment core collected from the eastern Lombok Basin between Sumba and Sumbawa Islands in the Indonesian Archipelago. Gamma spectrometry and accelerator mass spectrometry data together with radiometric dating of the core provide a high-resolution record of ongoing deposition of anthropogenic radionuclides. A plutonium signature characteristic of the Pacific Proving Grounds (PPG) dominates in the first two decades after the start of the high yield atmospheric tests in 1950’s. Approximately 40–70% of plutonium at this site in the post 1970 period originates from the PPG. This sediment record of transuranic isotopes deposition over the last 55 years provides evidence for the continuous long-distance transport of particle-reactive radionuclides from the Pacific Ocean towards the Indian Ocean.
Publisher: Elsevier BV
Date: 10-2015
Publisher: Elsevier BV
Date: 07-2006
Publisher: Elsevier BV
Date: 2016
DOI: 10.1016/J.JENVRAD.2015.06.021
Abstract: The isotopes (236)U and (239)Pu, both produced during nuclear weapons tests carried out in the 1950s and 1960s, are present in the environment and may be used as tracers for soil erosion studies. Although these radionuclides occur only at ultra-trace levels in nature, they can be readily measured by accelerator mass spectrometry with the 14UD heavy ion accelerator at the Australian National University. We have analysed a series of vegetation s les for their (236)U and (239)Pu concentration and compared the results with those found in the surrounding soil. (236)U could be measured in all collected s les whereas (239)Pu could not be detected in several vegetation s les due to its very low concentration, although it was readily detectable in the soil. We find that, relative to plutonium, (236)U is preferentially taken up by plants with enrichment factors ((236)U/(239)Pu)veg/((236)U/(239)Pu)soil that range between 7 and 52 in the present study.
Publisher: Wiley
Date: 02-2006
Publisher: Elsevier BV
Date: 10-2015
Publisher: Elsevier BV
Date: 2016
DOI: 10.1016/J.JENVRAD.2015.06.020
Abstract: The isotopes (236)U, (239)Pu and (240)Pu are present in surface soils as a result of global fallout from nuclear weapons tests carried out in the 1950's and 1960's. These isotopes potentially constitute artificial tracers of recent soil erosion and sediment movement. Only Accelerator Mass Spectrometry has the requisite sensitivity to measure all three isotopes at these environmental levels. Coupled with its relatively high throughput capabilities, this makes it feasible to conduct studies of erosion across the geographical extent of the Australian continent. In the Australian context, however, global fallout is not the only source of these isotopes. As part of its weapons development program the United Kingdom carried out a series of atmospheric and surface nuclear weapons tests at Maralinga, South Australia in 1956 and 1957. The tests have made a significant contribution to the Pu isotopic abundances present in the region around Maralinga and out to distances ∼1000 km, and impact on the assessment techniques used in the soil and sediment tracer studies. Quantification of the relative fallout contribution derived from detonations at Maralinga is complicated owing to significant contamination around the test site from numerous nuclear weapons safety trials that were also carried out around the site. We show that (236)U can provide new information on the component of the fallout that is derived from the local nuclear weapons tests, and highlight the potential of (236)U as a new fallout tracer.
Publisher: The Royal Society
Date: 06-2022
DOI: 10.1098/RSOS.220312
Abstract: Glaciation during the late Middle Pleistocene is widely recognized across continental northwest Europe, but its extent and palaeoenvironmental significance in the British Isles are disputed. Although glaciogenic sediments at Wolston, Warwickshire, in the English West Midlands, have been used to define the stratotype of the Wolstonian Stage, their age has been variably assigned between marine isotope stages (MIS) 12 and 6. Here we present sedimentological and stratigraphical observations from five sites across the English West Midlands whose chronology is constrained by new luminescence ages from glaciofluvial sediments, supplemented by cosmogenic 36 Cl exposure dating of erratic boulders. The ages suggest that between 199 ± 5 and 147 ± 2.5 ka the British Ice Sheet advanced into the English West Midlands as far south as Moreton-in-Marsh, Gloucestershire. This advance is assigned to the Moreton Stadial of the Late Wolstonian Substage. Dating of the glaciation to this substage allows correlation of the Moreton Stadial glacial deposits in the English West Midlands with those of the Drenthe Stadial during the Late Saalian Substage across continental northwest Europe.
Publisher: Elsevier BV
Date: 10-2012
Publisher: Elsevier BV
Date: 02-2017
Publisher: Elsevier BV
Date: 10-2022
Publisher: EDP Sciences
Date: 2012
Publisher: IOP Publishing
Date: 23-09-2011
Publisher: Elsevier BV
Date: 06-1994
Publisher: Elsevier BV
Date: 03-1990
Publisher: Wiley
Date: 2006
DOI: 10.1002/JQS.989
Publisher: American Physical Society (APS)
Date: 27-11-2018
Publisher: Elsevier BV
Date: 2010
DOI: 10.1016/J.JENVRAD.2009.08.011
Abstract: To study the Pu concentration and isotope ratio distributions present in China, the (239+240)Pu total activities and (240)Pu/(239)Pu atom ratios in core soil s les from Hubei Province in central China were investigated using Accelerator Mass Spectrometry (AMS). The activities ranged from 0.019 to 0.502 mBqg(-1) and the (239+240)Pu inventories of 45 and approximately 55 Bqm(-2) agree well with that expected from global fallout. The (240)Pu/(239)Pu atom ratios in the soil ranged from 0.172 to 0.220. The ratios are similar to typical global fallout values. Hence, any close-in fallout contribution from the Chinese nuclear weapons tests, mainly conducted in the 1970s, must have either been negligible or had a similar (240)Pu/(239)Pu ratio to that of global fallout. The top 10 cm layer of the soil contributes approximately 90% of the total inventory and the maximum concentrations appeared in the 2-4 cm or 4-6 cm layers. It is suggested that climatic conditions and organic content are the two main factors that affect the vertical migration of plutonium in soil.
Publisher: Elsevier BV
Date: 06-1994
Publisher: Wiley
Date: 10-03-2011
DOI: 10.1002/ESP.2058
Publisher: Elsevier BV
Date: 09-2017
Publisher: Elsevier BV
Date: 2020
DOI: 10.1016/J.JENVRAD.2019.106085
Abstract: The Daly River drains a large (52500 km
Publisher: Elsevier BV
Date: 2016
DOI: 10.1016/J.JENVRAD.2015.10.013
Abstract: During the operations at the Sellafield nuclear fuel reprocessing complex, artificial radionuclides are discharged to the Irish Sea under authorisation, where they are dispersed. In this study, the southern distribution and transport of Sellafield derived radionuclides have been investigated. Both natural and artificial radionuclides have been studied in a soil core from the riverbank of the Afon Goch in Anglesey, North Wales. Particulate input is dominant for all artificial radionuclides (including the more soluble (137)Cs and (236)U) with an estimated lag time of about a decade. The preferential northward seawater movement in the NE Irish Sea limits solution input of (137)Cs and (236)U to the areas south of Sellafield. The relatively long lag time reflects both the water circulation pattern and distance between the study site in north Wales and the source point in Cumbria. Two redox active zones are observed in the top and the bottom of this core, although there is no evidence for any redistribution of Pu and natural uranium by these redox processes. However, (236)U, derived from irradiated uranium, showed variable distribution in the core. This could be a potential response to the geochemical conditions, showing that (236)U may be a promising tracer for the environmental processes and a signature of the Sellafield historical discharges of irradiated uranium.
Publisher: IOP Publishing
Date: 02-1976
Publisher: Wiley
Date: 02-2002
Publisher: Wiley
Date: 2007
DOI: 10.1002/ESP.1415
Publisher: American Physical Society (APS)
Date: 18-09-1972
Publisher: Elsevier BV
Date: 11-1993
Publisher: IOP Publishing
Date: 03-1978
Publisher: Elsevier BV
Date: 09-2015
DOI: 10.1016/J.APRADISO.2015.06.011
Abstract: The Accelerator Mass Spectrometry (AMS) is the most sensitive technique, compared either to the Inductively Coupled Plasma (ICP-MS) or Thermal Ionization (TI-MS) mass spectrometer, for the actinide (e.g. (236)U, (x)Pu isotopes) measurements. They are present in environmental s les at the ultra trace level since atmospheric tests of Nuclear Weapons (NWs) performed in the past, deliberate dumping of nuclear waste, nuclear fuel reprocessing, on a large scale, and operation of Nuclear Power Plants (NPPs), on a small scale, have led to the release of a wide range of radioactive nuclides in the environment. At the Center for Isotopic Research on Cultural and Environmental heritage (CIRCE) in Caserta, Italy, an upgraded actinide AMS system, based on a 3-MV pelletron tandem accelerator, has been developed and routinely operated. At CIRCE a charge state distribution as a function of terminal voltage, the beam emittance, measured in the 20° actinides dedicated beam line, as well as the energy and position validation of the U ions were performed in order to determine the best measurement conditions. A (236)U/(238)U isotopic ratio background level of about 5×10(-12) or 3×10(-13), depending on the Time of Flight-Energy (TOF-E) configurations, as well as the spatial distribution of the (235)U, (238)U interferences ions and a (236)U contamination mass of about 0.5 fg have been determined.
Publisher: Elsevier BV
Date: 06-2010
Publisher: Elsevier BV
Date: 02-1998
Publisher: Springer Science and Business Media LLC
Date: 27-09-2017
Publisher: American Geophysical Union (AGU)
Date: 02-2000
DOI: 10.1029/2000WR900019
Publisher: Springer Science and Business Media LLC
Date: 07-1996
DOI: 10.1007/BF00817919
Publisher: Elsevier BV
Date: 06-1994
Publisher: SAGE Publications
Date: 06-02-2013
Abstract: Reconstructed Holocene lake-level curves from two saline, hydrologically closed maar crater lakes in southwestern Victoria, Australia, show near synchronous lake-level changes throughout the Holocene. We show that lake levels, reconstructed from sediment particle size and ostracod valve chemistry (δ 18 O and Sr/Ca) have undergone rapid ( yr), large ( m) fluctuations throughout the Holocene. Finer s ling resolution shows a more sensitive response to Holocene climate than was previously presented for Lake Keilambete. Both maar crater lakes show a short-lived maximum in Holocene lake levels around 7.2 ka. The period of lake filling leading to peak lake levels matches the phase of most effective precipitation (7.4–7.0 ka) reconstructed from a high-resolution speleothem record from northern Tasmania. Water levels declined in both lakes during the mid Holocene, with a more substantive decline after ~5 ka which coincides with the end of the Southern Hemisphere hypsithermal. Water levels continued to oscillate with a periodicity of around 300–700 years, before reaching a late-Holocene nadir around 1.8 ka (Keilambete) and 1.3 ka (Gnotuk). The trend and periodicity of oscillations in the maar water levels show commonalities to δD in the Dome C ice core, and suggest that temperature may be a significant component in influencing the Precipitation/Evaporation (P/E) ratio in southeastern Australia during the Holocene.
Publisher: Elsevier BV
Date: 2016
DOI: 10.1016/J.JENVRAD.2015.06.008
Abstract: Anthropogenic (236)U and (239)Pu were measured in European roe deer antlers hunted between 1955 and 1977 which covers and extends beyond the period of intensive nuclear weapons testing (1954-1962). The antlers were hunting trophies, and hence the hunting area, the year of shooting and the approximate age of each animal is given. Uranium and plutonium are known to deposit in skeletal tissue. Since antler histology is similar to bone, both elements were expected in antlers. Furthermore, roe deer shed their antlers annually, and hence antlers may provide a time-resolved environmental archive for fallout radionuclides. The radiochemical procedure is based on a Pu separation step by anion exchange (Dowex 1 × 8) and a subsequent U purification by extraction chromatography using UTEVA(®). The s les were measured by Accelerator Mass Spectrometry at the VERA facility (University of Vienna). In addition to the (236)U and (239)Pu concentrations, the (240)Pu/(239)Pu isotopic ratios were determined with a mean value of 0.172 ± 0.023 which is in agreement with the ratio of global fallout (∼0.18). Rather high (236)U/(238)U ratios of the order of 10(-6) were observed. These measured ratios, where the (236)U arises only from global fallout, have implications for the use of the (236)U/(238)U ratio as a fingerprint for nuclear accidents or releases from nuclear facilities. Our investigations have shown the potential to use antlers as a temporally resolved archive for the uptake of actinides from the environment.
Publisher: Elsevier BV
Date: 07-2003
Publisher: Royal Society of Chemistry (RSC)
Date: 2001
DOI: 10.1039/B007493O
Abstract: Accelerator mass spectrometry (AMS) was used to measure 237Np in environmental water s les extracted from Irish Sea sediments. The s les were of limited volume (approximately 700 ml) and of low activity (0.06-0.79 mBq l-1 2.30-30.3 pg l-1). AMS proved to have the required sensitivity for measuring these s les, and was in principle capable of measuring much smaller amounts, as low as 0.4 microBq (3.9 x 10(7) atoms). However, the background level in the procedural blanks showed that there was a systematic low level 237Np contamination of each s le, arising from the 239Np yield monitor used in the separations procedure, which effectively increased the detection limit of these analyses.
Publisher: American Chemical Society (ACS)
Date: 23-08-2013
DOI: 10.1021/ES400610H
Abstract: Measurements of total iodine (I) and iodine-129 ((129)I) concentrations in rivers and lakes of Argentina are presented. Their latitudinal distribution can be explained by taking into account their main sources (oceanic emissions and biomass burning for I, and atmospheric nuclear tests for (129)I), transport mechanisms, and fallout patterns. From the measured (129)I concentrations in the studied lakes, deposition fluences for their catchment areas were estimated. These results agree with a model of the global deposition pattern due to the (129)I released by atmospheric nuclear weapon tests and with other fluences reported for the southern hemisphere. In addition, the first measurements of (129)I in shallow seawater from the South Atlantic Ocean are presented and discussed.
Publisher: Elsevier BV
Date: 05-1977
Publisher: Geological Society of London
Date: 2010
DOI: 10.1144/SP346.12
Publisher: Elsevier BV
Date: 09-2012
Publisher: American Geophysical Union (AGU)
Date: 10-11-2004
DOI: 10.1029/2004PA001047
Publisher: Elsevier BV
Date: 11-2003
Publisher: Elsevier BV
Date: 11-2017
DOI: 10.1016/J.JENVRAD.2017.08.009
Abstract: At present there is a need for the development of new radioisotopes for soil erosion and sediment tracing especially as fallout
Publisher: Elsevier BV
Date: 08-1987
Publisher: Geological Society of America
Date: 2007
DOI: 10.1130/G23641A.1
Publisher: Elsevier BV
Date: 08-2008
Publisher: Elsevier BV
Date: 12-1981
Publisher: Elsevier BV
Date: 02-2007
Publisher: Geological Society of America
Date: 17-02-2017
DOI: 10.1130/B31373.1
Publisher: Elsevier BV
Date: 2013
Publisher: Elsevier BV
Date: 05-2014
Publisher: Elsevier BV
Date: 11-1988
Publisher: Geological Society of London
Date: 2014
DOI: 10.1144/SP395.15
Publisher: Elsevier BV
Date: 09-2013
DOI: 10.1016/J.ENVINT.2013.05.017
Abstract: A combination of state-of-the-art isotopic fingerprinting techniques and atmospheric transport modelling using real-time historical meteorological data has been used to demonstrate direct tropospheric transport of radioactive debris from specific nuclear detonations at the Semipalatinsk test site in Kazakhstan to Norway via large areas of Europe. A selection of archived air filters collected at ground level at 9 stations in Norway during the most intensive atmospheric nuclear weapon testing periods (1957-1958 and 1961-1962) has been screened for radioactive particles and analysed with respect to the concentrations and atom ratios of plutonium (Pu) and uranium (U) using accelerator mass spectrometry (AMS). Digital autoradiography screening demonstrated the presence of radioactive particles in the filters. Concentrations of (236)U (0.17-23nBqm(-3)) and (239+240)Pu (1.3-782μBqm(-3)) as well as the atom ratios (240)Pu/(239)Pu (0.0517-0.237) and (236)U/(239)Pu (0.0188-0.7) varied widely indicating several different sources. Filter s les from autumn and winter tended to have lower atom ratios than those s led in spring and summer, and this likely reflects a tropospheric influence in months with little stratospheric fallout. Very high (236)U, (239+240)Pu and gross beta activity concentrations as well as low (240)Pu/(239)Pu (0.0517-0.077), (241)Pu/(239)Pu (0.00025-0.00062) and (236)U/(239)Pu (0.0188-0.046) atom ratios, characteristic of close-in and tropospheric fallout, were observed in filters collected at all stations in Nov 1962, 7-12days after three low-yield detonations at Semipalatinsk (Kazakhstan). Atmospheric transport modelling (NOAA HYSPLIT_4) using real-time meteorological data confirmed that long range transport of radionuclides, and possibly radioactive particles, from Semipalatinsk to Norway during this period was plausible. The present work shows that direct tropospheric transport of fallout from atmospheric nuclear detonations periodically may have had much larger influence on radionuclide air concentrations and deposition than previously anticipated.
Publisher: American Physical Society (APS)
Date: 08-1975
Publisher: Elsevier BV
Date: 06-1979
Publisher: Elsevier BV
Date: 02-1987
Publisher: Elsevier BV
Date: 12-1990
Publisher: Elsevier BV
Date: 09-2018
DOI: 10.1016/J.CANLET.2018.05.044
Abstract: MicroRNAs (miRNAs) are endogenous small, non-coding RNAs that regulate genome expression at the post-transcriptional level. They are involved in a wide range of physiological processes including the maintenance of immune homeostasis and normal function. Accumulating evidence from animal studies show that alterations in pan or specific miRNA expression would break immunological tolerance, leading to autoimmunity. Differential miRNA expressions have also been documented in patients of many autoimmune disorders. In this review, we highlight the evidence that signifies the critical role of miRNAs in autoimmunity, specifically on their regulatory roles in the pathogenesis of several rheumatic diseases including systemic lupus erythematosus, rheumatoid arthritis and spondyloarthritis. The potential of miRNAs as biomarkers and therapeutic targets is also discussed. Manipulation of dysregulated miRNAs in vivo through miRNA delivery or inhibition offers promise for new therapeutic strategies in treating rheumatic diseases.
Publisher: Elsevier BV
Date: 1989
Publisher: Elsevier BV
Date: 10-2011
DOI: 10.1016/J.JENVRAD.2010.06.010
Abstract: A study has been carried out to assess the potential of using fallout plutonium (Pu), which originated from atmospheric nuclear-weapons tests, as a tool to investigate recent erosional processes within the lower Cotter water-supply catchment in the Australian Capital Territory. This catchment, which was predominantly pine plantation, was severely affected by a major bush fire in 2003. Accelerator mass spectrometry has been used to measure Pu in soil s les collected from a number of sites across the catchment. The results indicate that less than 1cm of surface soil had been lost since the early 1960s over much of the catchment. Areas of more erodible soil have, however, lost 2-4cm of topsoil, and a loss of ∼6cm of soil was identified at one particular site.
Publisher: Informa UK Limited
Date: 11-2002
Publisher: Elsevier BV
Date: 07-2010
Publisher: Elsevier
Date: 2008
Publisher: Elsevier BV
Date: 04-2006
Publisher: Elsevier BV
Date: 10-1989
Publisher: Wiley
Date: 03-1996
Publisher: Elsevier BV
Date: 11-2006
Publisher: Elsevier BV
Date: 10-2009
Publisher: Elsevier BV
Date: 08-2004
Publisher: Elsevier BV
Date: 09-2013
DOI: 10.1016/J.SCITOTENV.2013.05.054
Abstract: In the present work, state of the art isotopic fingerprinting techniques are applied to an Arctic ice core in order to quantify deposition of U and Pu, and to identify possible tropospheric transport of debris from former Soviet Union test sites Semipalatinsk (Central Asia) and Novaya Zemlya (Arctic Ocean). An ice core chronology of (236)U, (239)Pu, and (240)Pu concentrations, and atom ratios, measured by accelerator mass spectrometry in a 28.6m deep ice core from the Austfonna glacier at Nordaustlandet, Svalbard is presented. The ice core chronology corresponds to the period 1949 to 1999. The main sources of Pu and (236)U contamination in the Arctic were the atmospheric nuclear detonations in the period 1945 to 1980, as global fallout, and tropospheric fallout from the former Soviet Union test sites Novaya Zemlya and Semipalatinsk. Activity concentrations of (239+240)Pu ranged from 0.008 to 0.254 mBq cm(-2) and (236)U from 0.0039 to 0.053 μBq cm(-2). Concentrations varied in concordance with (137)Cs concentrations in the same ice core. In contrast to previous published results, the concentrations of Pu and (236)U were found to be higher at depths corresponding to the pre-moratorium period (1949 to 1959) than to the post-moratorium period (1961 and 1962). The (240)Pu/(239)Pu ratio ranged from 0.15 to 0.19, and (236)U/(239)Pu ranged from 0.18 to 1.4. The Pu atom ratios ranged within the limits of global fallout in the most intensive period of nuclear atmospheric testing (1952 to 1962). To the best knowledge of the authors the present work is the first publication on biogeochemical cycles with respect to (236)U concentrations and (236)U/(239)Pu atom ratios in the Arctic and in ice cores.
Publisher: Elsevier BV
Date: 10-2011
DOI: 10.1016/J.JENVRAD.2010.05.012
Abstract: A sediment core collected from the sub-aqueous delta of the Yangtze River estuary was subjected to analyses of (137)Cs and plutonium (Pu) isotopes. The (137)Cs was measured using γ-spectrometry at the laboratories at the Nanjing University and Pu isotopes were determined with Accelerator Mass Spectrometry (AMS), measurements made at the Australian National University. The results show considerable structure in the depth concentration profiles of the (137)Cs and (239+240)Pu. The shape of the vertical (137)Cs distribution in the sediment core was similar to that of the Pu. The maximum (137)Cs and (239+240)Pu concentrations were 16.21 ± 0.95 mBq/g and 0.716 ± 0.030 mBq/g, respectively, and appear at same depth. The average (240)Pu/(239)Pu atom ratio was 0.238 ± 0.007 in the sediment core, slightly higher than the average global fallout value. The changes in the (240)Pu/(239)Pu atom ratios in the sediment core indicate the presence of at least two different Pu sources, i.e., global fallout and another source, most likely close-in fallout from the Pacific Proving Grounds (PPG) in the Marshall Islands, and suggest the possibility that Pu isotopes are useful as a geochronological tool for coastal sediment studies. The (137)Cs and (239+240)Pu inventories were estimated to be 7100 ± 1200 Bq/m(2) and 407 ± 27 Bq/m(2), respectively. Approximately 40% of the (239+240)Pu inventory originated from the PPG close-in fallout and about 50% has derived from land-origin global fallout transported to the estuary by the river. This study confirms that AMS is a useful tool to measure (240)Pu/(239)Pu atom ratio and can provide valuable information on sedimentary processes in the coastal environment.
Publisher: Elsevier BV
Date: 05-2013
Publisher: Elsevier BV
Date: 03-1994
Publisher: Springer Science and Business Media LLC
Date: 03-2004
DOI: 10.1038/NATURE02386
Publisher: Elsevier BV
Date: 04-1997
Publisher: Elsevier BV
Date: 07-1988
Publisher: American Physical Society (APS)
Date: 10-1974
Publisher: Elsevier BV
Date: 02-1983
Publisher: Elsevier BV
Date: 2019
Publisher: Elsevier BV
Date: 02-2016
Publisher: Elsevier BV
Date: 02-2009
Publisher: Elsevier BV
Date: 12-2010
Publisher: Elsevier BV
Date: 10-2004
Publisher: Elsevier BV
Date: 07-1977
Publisher: Springer Science and Business Media LLC
Date: 06-04-2016
DOI: 10.1038/NATURE17196
Publisher: Elsevier
Date: 2001
Publisher: Elsevier BV
Date: 04-1984
Publisher: Elsevier BV
Date: 05-1973
Publisher: American Chemical Society (ACS)
Date: 14-04-2000
DOI: 10.1021/ES990847Z
Publisher: IOP Publishing
Date: 07-1980
Publisher: Elsevier BV
Date: 05-2006
Publisher: Springer Science and Business Media LLC
Date: 2001
Publisher: Elsevier BV
Date: 1989
Publisher: American Physical Society (APS)
Date: 04-1976
Publisher: Springer Science and Business Media LLC
Date: 30-04-2011
DOI: 10.1007/S00216-011-4979-2
Abstract: A first international (36)Cl interlaboratory comparison has been initiated. Evaluation of the final results of the eight participating accelerator mass spectrometry (AMS) laboratories on three synthetic AgCl s les with (36)Cl/Cl ratios at the 10(-11), 10(-12), and 10(-13) level shows no difference in the sense of simple statistical significance. However, more detailed statistical analyses demonstrate certain interlaboratory bias and underestimation of uncertainties by some laboratories. Following subsequent remeasurement and reanalysis of the data from some AMS facilities, the round-robin data indicate that (36)Cl/Cl data from two in idual AMS laboratories can differ by up to 17%. Thus, the demand for further work on harmonising the (36)Cl-system on a worldwide scale and enlarging the improvement of measurements is obvious.
Publisher: Cambridge University Press (CUP)
Date: 2001
DOI: 10.1017/S0033822200031611
Abstract: Lynch's Crater in northeastern Australia provides a long, continuous record of environmental change within the Late Quaternary. Here, we present newly determined radiocarbon ages, using acid-base-acid stepped combustion (ABA-SC) and acid-base-wet oxidation stepped combustion (ABOX-SC) pretreatment strategies. The new results largely confirm the original untreated radiocarbon results for the uppermost 9 m of sediments, (ca. 35 ka BP). Below this depth, results from both pretreatment methods are in stratigraphic agreement and extend the dating of the record from 38 ka BP to about 48 ka BP, although an apparent increased sedimentation rate below 12 m is questionable. The scarcity of “charcoal” in several of the s les raises questions regarding the application of ABOX-SC to lake or sw sediments, with evidence for contributions from younger, chemically resistant bacterial carbon along with fine “charcoal” in some s les. However, the extent to which this phenomenon is significant to the final age estimate appears to be s le specific, and is probably dependent upon the length of the wet oxidation step in the pretreatment.
Publisher: Springer Science and Business Media LLC
Date: 10-2004
DOI: 10.1038/NATURE02956
Abstract: Excavations at Liang Bua, a large limestone cave on the island of Flores in eastern Indonesia, have yielded evidence for a population of tiny hominins, sufficiently distinct anatomically to be assigned to a new species, Homo floresiensis. The finds comprise the cranial and some post-cranial remains of one in idual, as well as a premolar from another in idual in older deposits. Here we describe their context, implications and the remaining archaeological uncertainties. Dating by radiocarbon (14C), luminescence, uranium-series and electron spin resonance (ESR) methods indicates that H. floresiensis existed from before 38,000 years ago (kyr) until at least 18 kyr. Associated deposits contain stone artefacts and animal remains, including Komodo dragon and an endemic, dwarfed species of Stegodon. H. floresiensis originated from an early dispersal of Homo erectus (including specimens referred to as Homo ergaster and Homo georgicus) that reached Flores, and then survived on this island refuge until relatively recently. It overlapped significantly in time with Homo sapiens in the region, but we do not know if or how the two species interacted.
Publisher: Elsevier BV
Date: 08-2004
Location: United Kingdom of Great Britain and Northern Ireland
Start Date: 02-2018
End Date: 12-2021
Amount: $520,865.00
Funder: Australian Research Council
View Funded ActivityStart Date: 04-2011
End Date: 09-2014
Amount: $556,800.00
Funder: Australian Research Council
View Funded ActivityStart Date: 04-2013
End Date: 12-2016
Amount: $360,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2007
End Date: 12-2009
Amount: $378,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2009
End Date: 12-2012
Amount: $290,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2003
End Date: 12-2005
Amount: $295,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2005
End Date: 12-2005
Amount: $854,354.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2005
End Date: 12-2008
Amount: $150,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2005
End Date: 12-2006
Amount: $267,767.00
Funder: Australian Research Council
View Funded ActivityStart Date: 07-2007
End Date: 12-2011
Amount: $700,000.00
Funder: Australian Research Council
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