ORCID Profile
0000-0003-1135-1810
Current Organisations
University of Queensland
,
Australian Nuclear Science and Technology Organisation
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Quaternary Environments | Environmental Chemistry (incl. Atmospheric Chemistry) | Physical Geography and Environmental Geoscience | Conservation and Biodiversity
Expanding Knowledge in the Environmental Sciences | Environmental Management Systems | Climate Change Mitigation Strategies |
Publisher: Copernicus GmbH
Date: 27-09-2010
Abstract: Abstract. A time-dependent map of radon-222 flux density at the Australian land surface has been constructed with a spatial resolution of 0.05° and temporal resolution of one month. Radon flux density was calculated from a simple model utilising data from national gamma-ray aerial surveys modelled soil moisture, available from 1900 in near real-time and maps of soil properties. The model was calibrated against a data set of accumulation chamber measurements, thereby constraining it with experimental data. A notable application of the map is in atmospheric mixing and transport studies which use radon as a tracer, where it is a clear improvement on the common assumption of uniform radon flux density.
Publisher: Copernicus GmbH
Date: 09-03-2022
DOI: 10.5194/ACP-2022-104
Abstract: Abstract. Despite considerable efforts during the last decade, real-time characterization of the marine boundary layer and aerosol optical properties over the Southern Ocean remains scarce. We conducted simultaneous measurements of the marine boundary layer utilizing a synergy of remote sensing technology at the Baseline Air Pollution Station at Cape Grim in northwestern Tasmania, Australia, from 14 May to 16 July 2019. Aerosol optical properties were monitored by lidar (miniMPL) and a ceilometer to identify the boundary layer height, and sodar provided wind profiles to investigate their influences on the layer evolution. Boundary layer heights simulated using the Weather Research and Forecasting (WRF) model were also employed for comparison purposes. Through complementary analyses of three cases representing different source influences (marine, sea breeze and continental), this paper evaluates two algorithms (Image Edge Detection Algorithm (IEDA) and gradient method) for boundary layer height detection and examines the vertical aerosol distribution within the boundary layer at Cape Grim with an emphasis on the contributions of regional and local meteorology. We found IEDA generally performed better than the gradient method, especially during the marine-flow-influenced period with a convective layer structure. Different features of boundary layer structures in three episodes, including differential boundary layer growth and interaction with wind evolutionary processes were investigated. One was characterized by a diurnal variation with a boundary layer height of approximately 0.2–0.5 km, associated with the veering of the wind vector within the marine boundary layer during the development of a sea breeze. The other showed a thermally stable layer below 0.3 km with an enhanced extinction coefficient and linear depolarization ratio under the influence of continental sources, which was also validated by the observation from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite. The increasing extinction coefficient and depolarization ratio with wind speeds may be attributed to the increased wet sea salt production and regional transportation from mainland Australia.
Publisher: Copernicus GmbH
Date: 14-06-2017
Abstract: Abstract. Terrestrial data spanning the Last Glacial Maximum (LGM) and deglaciation from the southern Australian region are sparse and limited to discontinuous sedimentological and geomorphological records with relatively large chronological uncertainties. This dearth of records has hindered a critical assessment of the role of the Southern Hemisphere mid-latitude westerly winds on the region's climate during this time period. In this study, two precisely dated speleothem records for Mairs Cave, Flinders Ranges, are presented, providing for the first time a detailed terrestrial hydroclimatic record for the southern Australian drylands during 23–15 ka. Recharge to Mairs Cave is interpreted from the speleothem record by the activation of growth, physical flood layering, and δ18O and δ13C minima. Periods of lowered recharge are indicated by 18O and 13C enrichment, primarily affecting δ18O, argued to be driven by evaporation of shallow soil/epikarst water in this water-limited environment. A hydrological driver is supported by calcite fabric changes. These include the presence of laminae, visible organic colloids, and occasional dissolution features, related to recharge, as well as the presence of sediment bands representing cave floor flooding. A shift to slower-growing, more compact calcite and an absence of lamination is interpreted to represent reduced recharge. The Mairs Cave record indicates that the Flinders Ranges were relatively wet during the LGM and early deglaciation, particularly over the interval 18.9–15.8 ka. This wetter phase ended abruptly with a shift to drier conditions at 15.8 ka. These findings are in agreement with the geomorphic archives for this region, as well as the timing of events in records from the broader Australasian region. The recharge phases identified in the Mairs Cave record are correlated with, but antiphase to, the position of the westerly winds interpreted from marine core MD03-2611, located 550 km south of Mairs Cave in the Murray Canyons region. The implication is that the mid-latitude westerlies are located further south during the period of enhanced recharge in the Mairs Cave record (18.9–16 ka) and conversely are located further north when greater aridity is interpreted in the speleothem record. A further comparison with speleothem records from the northern Australasian region reveals that the availability of tropical moisture is the most likely explanation driving enhanced recharge, with further lification of recharge occurring during the early half of Heinrich Stadial 1 (HS1), possibly influenced by a more southerly displaced Intertropical Convergence Zone (ITCZ). A rapid transition to aridity at 15.8 ka is consistent with a retraction of this tropical moisture source.
Publisher: Taiwan Association for Aerosol Research
Date: 2016
Publisher: Copernicus GmbH
Date: 29-03-2023
Abstract: Abstract. The remoteness and extreme conditions of the Southern Ocean and Antarctic region have meant that observations in this region are rare, and typically restricted to summertime during research or resupply voyages. Observations of aerosols outside of the summer season are typically limited to long-term stations, such as Kennaook / Cape Grim (KCG 40.7∘ S, 144.7∘ E), which is situated in the northern latitudes of the Southern Ocean, and Antarctic research stations, such as the Japanese operated Syowa (SYO 69.0∘ S, 39.6∘ E). Measurements in the midlatitudes of the Southern Ocean are important, particularly in light of recent observations that highlighted the latitudinal gradient that exists across the region in summertime. Here we present 2 years (March 2016–March 2018) of observations from Macquarie Island (MQI 54.5∘ S, 159.0∘ E) of aerosol (condensation nuclei larger than 10 nm, CN10) and cloud condensation nuclei (CCN at various supersaturations) concentrations. This important multi-year data set is characterised, and its features are compared with the long-term data sets from KCG and SYO together with those from recent, regionally relevant voyages. CN10 concentrations were the highest at KCG by a factor of ∼50 % across all non-winter seasons compared to the other two stations, which were similar (summer medians of 530, 426 and 468 cm−3 at KCG, MQI and SYO, respectively). In wintertime, seasonal minima at KCG and MQI were similar (142 and 152 cm−3, respectively), with SYO being distinctly lower (87 cm−3), likely the result of the reduction in sea spray aerosol generation due to the sea ice ocean cover around the site. CN10 seasonal maxima were observed at the stations at different times of year, with KCG and MQI exhibiting January maxima and SYO having a distinct February high. Comparison of CCN0.5 data between KCG and MQI showed similar overall trends with summertime maxima and wintertime minima however, KCG exhibited slightly (∼10 %) higher concentrations in summer (medians of 158 and 145 cm−3, respectively), whereas KCG showed ∼40 % lower concentrations than MQI in winter (medians of 57 and 92 cm−3, respectively). Spatial and temporal trends in the data were analysed further by contrasting data to coincident observations that occurred aboard several voyages of the RSV Aurora Australis and the RV Investigator. Results from this study are important for validating and improving our models and highlight the heterogeneity of this pristine region and the need for further long-term observations that capture the seasonal cycles.
Publisher: Copernicus GmbH
Date: 28-09-2017
DOI: 10.5194/ACP-17-11623-2017
Abstract: Abstract. Mercury is a toxic element of serious concern for human and environmental health. Understanding its natural cycling in the environment is an important goal towards assessing its impacts and the effectiveness of mitigation strategies. Due to the unique chemical and physical properties of mercury, the atmosphere is the dominant transport pathway for this heavy metal, with the consequence that regions far removed from sources can be impacted. However, there exists a dearth of long-term monitoring of atmospheric mercury, particularly in the tropics and Southern Hemisphere. This paper presents the first 2 years of gaseous elemental mercury (GEM) measurements taken at the Australian Tropical Atmospheric Research Station (ATARS) in northern Australia, as part of the Global Mercury Observation System (GMOS). Annual mean GEM concentrations determined at ATARS (0.95 ± 0.12 ng m−3) are consistent with recent observations at other sites in the Southern Hemisphere. Comparison with GEM data from other Australian monitoring sites suggests a concentration gradient that decreases with increasing latitude. Seasonal analysis shows that GEM concentrations at ATARS are significantly lower in the distinct wet monsoon season than in the dry season. This result provides insight into alterations of natural mercury cycling processes as a result of changes in atmospheric humidity, oceanic/terrestrial fetch, and convective mixing, and invites future investigation using wet mercury deposition measurements. Due to its location relative to the atmospheric equator, ATARS intermittently s les air originating from the Northern Hemisphere, allowing an opportunity to gain greater understanding of inter-hemispheric transport of mercury and other atmospheric species. Diurnal cycles of GEM at ATARS show distinct nocturnal depletion events that are attributed to dry deposition under stable boundary layer conditions. These cycles provide strong further evidence supportive of a multi-hop model of GEM cycling, characterised by multiple surface depositions and re-emissions, in addition to long-range transport through the atmosphere.
Publisher: Copernicus GmbH
Date: 04-07-2014
DOI: 10.5194/ACPD-14-18083-2014
Abstract: Abstract. Atmospheric composition measurements at Jungfraujoch are affected intermittently by thermally-driven (anabatic) mountain winds as well as by other vertical transport mechanisms. Using radon-222 observations, and a new analysis method, we quantify the land surface influence hour-by-hour and detect the presence of anabatic winds on a daily basis. During 2010–2011, anabatic winds occurred on roughly 40% of days, but only from April–September. Anabatic wind days were associated with warmer air temperatures over a large fraction of Europe and with a shift in airmass properties. Shifts were evident even when comparing the same radon concentrations, a proxy for land-surface influence. Aerosol washout, when quantified as a function of rain-rate using a radon normalisation technique, was also influenced by anabatic winds being more pronounced on non-anabatic days. Excluding the influence of anabatic winds, however, did not lead to a better definition of the unperturbed aerosol background than a definition based on radon alone, supporting the use of a radon threshold to identify periods with weak land-surface influence.
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 2013
Publisher: MDPI AG
Date: 04-07-2019
Abstract: The ability of meteorological models to accurately characterise regional meteorology plays a crucial role in the performance of photochemical simulations of air pollution. As part of the research funded by the Australian government’s Department of the Environment Clean Air and Urban Landscape hub, this study set out to complete an intercomparison of air quality models over the Sydney region. This intercomparison would test existing modelling capabilities, identify any problems and provide the necessary validation of models in the region. The first component of the intercomparison study was to assess the ability of the models to reproduce meteorological observations, since it is a significant driver of air quality. To evaluate the meteorological component of these air quality modelling systems, seven different simulations based on varying configurations of inputs, integrations and physical parameterizations of two meteorological models (the Weather Research and Forecasting (WRF) and Conformal Cubic Atmospheric Model (CCAM)) were examined. The modelling was conducted for three periods coinciding with comprehensive air quality measurement c aigns (the Sydney Particle Studies (SPS) 1 and 2 and the Measurement of Urban, Marine and Biogenic Air (MUMBA)). The analysis focuses on meteorological variables (temperature, mixing ratio of water, wind (via wind speed and zonal wind components), precipitation and planetary boundary layer height), that are relevant to air quality. The surface meteorology simulations were evaluated against observations from seven Bureau of Meteorology (BoM) Automatic Weather Stations through composite diurnal plots, Taylor plots and paired mean bias plots. Simulated vertical profiles of temperature, mixing ratio of water and wind (via wind speed and zonal wind components) were assessed through comparison with radiosonde data from the Sydney Airport BoM site. The statistical comparisons with observations identified systematic overestimations of wind speeds that were more pronounced overnight. The temperature was well simulated, with biases generally between ±2 °C and the largest biases seen overnight (up to 4 °C). The models tend to have a drier lower atmosphere than observed, implying that better representations of soil moisture and surface moisture fluxes would improve the subsequent air quality simulations. On average the models captured local-scale meteorological features, like the sea breeze, which is a critical feature driving ozone formation in the Sydney Basin. The overall performance and model biases were generally within the recommended benchmark values (e.g., ±1 °C mean bias in temperature, ±1 g/kg mean bias of water vapour mixing ratio and ±1.5 m s−1 mean bias of wind speed) except at either end of the scale, where the bias tends to be larger. The model biases reported here are similar to those seen in other model intercomparisons.
Publisher: Copernicus GmbH
Date: 15-05-2023
DOI: 10.5194/EGUSPHERE-EGU23-2947
Abstract: The influence of karst hydrology or & #8216 flowpaths& #8217 on speleothem oxygen isotopic (& #948 O) values has been simulated using karst forward models. & Cave monitoring studies have also shown that variability in dripwater & #948 O can be directly related to whether flowpaths are dominated by preferential/quick flow or diffuse/slow flow which challenges the paradigm of speleothems as archives of past variability in mean rainfall & #948 O.& Yet it is not known how common this flowpath effect is and whether it should be considered in the interpretation of speleothem & #948 O records. & Recently, Treble et al. (2022) analysed two global databases: SISAL v2 (Comas-Bru et al., 2020) and an extended compilation of dripwater from Baker et al. (2019).& It was demonstrated that within-cave variability in mean & #948 O values were common worldwide in both datasets. & An analysis of cave meta-data demonstrated that the flowpath effect is unrelated to climate, cave depth or lithology further supporting the ubiquitous nature of flowpaths, i.e., there is (1) a mixture of preferential and diffuse flow for all karstified carbonate rocks due to its triple-porosity nature (primary=matrix, secondary=fracture, tertiary=pipes and conduit) and (2) differences in soil/epikarst water storage and drainage characteristics.We demonstrate how a mechanistic understanding of flowpaths can lead to a more robust interpretation using a case study that is also relevant for managing water resources in the Mediterranean-type climate of south-west Australia.& Using seven modern stalagmite records from four caves, plus dripwater data, we demonstrate that the cave & #948 O record shows a common response to a sustained decrease in rainfall that impacted the region in the 1970s, characterised by a rise or & #8216 uptick& #8217 in & #948 O (Priestley et al., 2022).& Mean annual rainfall & #948 O values over the same period were quantified using observed and modelled data to have varied by & #8722 .4 to +0.1 & #8240 whereas the speleothem uptick is +1.5 & #8240 .& The much larger magnitude of the uptick is consistent with a reduction in the preferential-flow component to these caves driven by reduced rainfall recharge. & Preferential flow is an important contribution to groundwater. & The & #8216 uptick& #8217 or reduction in preferential flow implies that rainfall recharge to groundwater across the study region may no longer be reliably occurring.& The longer paleo-record for south-west Australia confirms that no replicated upticks are seen in the last 800 years in stalagmites from the region and highlights the impact of climate change to water security in a region heavily dependent on groundwater.& Comas-Bru, L. et al. SISALv2 (2020). A comprehensive speleothem isotope database with multiple age-depth models. Earth Syst. Sci. Data 12, 2579& #8211 (2020).Priestley, S., et al. (2022). Caves provide early warning of unprecedented decrease in rainfall recharge of groundwater. Research Square. doi:0.21203/rs.3.rs-1556439/v1Treble, P. C., et al. (2022). Ubiquitous karst hydrological control on speleothem oxygen isotope variability in a global study. Communications Earth & Environment, 3(1), 29. doi:10.1038/s43247-022-00347-3.
Publisher: Stockholm University Press
Date: 2016
Publisher: Copernicus GmbH
Date: 05-12-2014
DOI: 10.5194/ACP-14-12763-2014
Abstract: Abstract. Atmospheric composition measurements at Jungfraujoch are affected intermittently by boundary-layer air which is brought to the station by processes including thermally driven (anabatic) mountain winds. Using observations of radon-222, and a new objective analysis method, we quantify the land-surface influence at Jungfraujoch hour by hour and detect the presence of anabatic winds on a daily basis. During 2010–2011, anabatic winds occurred on 40% of days, but only from April to September. Anabatic wind days were associated with warmer air temperatures over a large fraction of Europe and with a shift in air-mass properties, even when comparing days with a similar mean radon concentration. Excluding days with anabatic winds, however, did not lead to a better definition of the unperturbed aerosol background than a definition based on radon alone. This implies that a radon threshold reliably excludes local influences from both anabatic and non-anabatic vertical-transport processes.
Publisher: IEEE
Date: 07-2018
Publisher: IEEE
Date: 07-2018
Publisher: Elsevier BV
Date: 05-2020
DOI: 10.1016/J.SCITOTENV.2019.135105
Abstract: The isotopic composition of groundwater can be a useful indicator of recharge conditions and may be used as an archive to infer past climate variability. Groundwater from two largely confined aquifers in south-west Australia, recharged at the northernmost extent of the westerly wind belt, can help constrain the palaeoclimate record in this region. We demonstrate that radiocarbon age measurements of dissolved inorganic carbon are appropriate for dating groundwater from the Leederville aquifer and Yarragadee aquifer within the Perth Basin. Variations in groundwater δ
Publisher: IEEE
Date: 06-2016
Publisher: Copernicus GmbH
Date: 24-02-2016
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 05-2022
Publisher: Copernicus GmbH
Date: 08-03-2016
Publisher: Copernicus GmbH
Date: 21-04-2017
DOI: 10.5194/ACP-2017-307
Abstract: Abstract. Mercury is a toxic element of serious concern for human and environmental health. Understanding its natural cycling in the environment is an important goal towards assessing its impacts and the effectiveness of mitigation strategies. Due to the unique chemical and physical properties of mercury, the atmosphere is the dominant transport pathway for this heavy metal, with the consequence that regions far removed from sources can be impacted. However, there exists a dearth of long-term monitoring of atmospheric mercury, particularly in the tropics and southern hemisphere. This paper presents the first two years of gaseous elemental mercury (GEM) measurements taken at the Australian Tropical Atmospheric Research Station (ATARS) in northern Australia, as part of the Global Mercury Observation System (GMOS). Annual mean GEM concentrations determined at ATARS (0.95 ± 0.12 ng m−3) are consistent with recent observations at other sites in the southern hemisphere. Comparison with GEM data from other Australian monitoring sites suggests a concentration gradient that decreases with increasing latitude. Seasonal analysis shows that GEM concentrations at ATARS are significantly lower in the distinct wet monsoon season than in the dry season. This result provides insight into alterations of natural mercury cycling processes as a result of changes in atmospheric humidity, oceanic/terrestrial fetch and convective mixing, and invites future investigation using wet mercury deposition measurements. Due to its location relative to the atmospheric equator, ATARS intermittently s les air originating from the northern hemisphere, allowing an opportunity to gain greater understanding of inter-hemispheric transport of mercury and other atmospheric species. Diurnal cycles of GEM at ATARS show distinct nocturnal depletion events that are attributed to dry deposition under stable boundary layer conditions. These cycles provide strong further evidence for the multi-hop model of global GEM cycling, whereby long-range transport is characterised by multiple surface depositions and re-emissions, rather than continuous transport over long distances.
Publisher: Copernicus GmbH
Date: 08-03-2016
Publisher: Elsevier BV
Date: 04-2015
Publisher: Copernicus GmbH
Date: 26-11-2020
Publisher: Scientific Research Publishing, Inc.
Date: 2017
Publisher: Copernicus GmbH
Date: 28-06-2016
Abstract: Abstract. Dual-flow-loop two-filter radon detectors have a slow time response, which can affect the interpretation of their output when making continuous observations of near-surface atmospheric radon concentrations. While concentrations are routinely reported hourly, a calibrated model of detector performance shows that ∼ 40 % of the signal arrives more than an hour after a radon pulse is delivered. After investigating several possible ways to correct for the detector's slow time response, we show that a Bayesian approach using a Markov chain Monte Carlo s ler is an effective method. After deconvolution, the detector's output is redistributed into the appropriate counting interval and a 10 min temporal resolution can be achieved under test conditions when the radon concentration is controlled. In the case of existing archived observations, collected under less ideal conditions, the data can be retrospectively reprocessed at 30 min resolution. In one case study, we demonstrate that a deconvolved radon time series was consistent with the following: measurements from a fast-response carbon dioxide monitor grab s les from an aircraft and a simple mixing height model. In another case study, during a period of stable nights and days with well-developed convective boundary layers, a bias of 18 % in the mean daily minimum radon concentration was eliminated by correcting for the instrument response.
Publisher: Copernicus GmbH
Date: 03-03-2021
DOI: 10.5194/EGUSPHERE-EGU21-196
Abstract: & & An overlapping need exists between the climate science, air quality and radiological protection communities for a robust, portable and direct monitor of atmospheric & sup& & /sup& Rn concentrations typical of the ambient outdoor atmosphere. To reliably characterise afternoon radon concentrations, or resolve daytime vertical radon gradients in the atmospheric boundary layer (requirements for radon measurements to be used to evaluate the performance of chemical transport models), detection limits of & #8804 .2 Bq m& sup& -3& /sup& at an hourly temporal resolution are required. Commercial portable radon detectors are mainly designed for indoor use, and the best of these has a detection limit of & #8805 Bq m& sup& -3& /sup& for hourly s ling, with an approximate uncertainty of 60% at typical outdoor daytime radon concentrations.& Here we introduce a portable (200 L) version of the two-filter dual-flow-loop radon detector, designed and built by ANSTO in collaboration with the EMPIR 19ENV01 traceRadon project. While not as compact as commercial monitors (standing 1.6 m tall, and 0.48 m wide), its longest component is 1.2 m, enabling transportation in a standard utility vehicle or 4x4 (and can fit inside a 19& #8221 instrument rack). Constructed of marine grade stainless steel, it is weather resistant, robust, and suitable for long-term, continuous, autonomous deployment in fact it is fully remotely controllable if a networked computer is available. The estimated lower limit of detection is 0.17 Bq m& sup& -3& /sup& for hourly observations, and the counting uncertainty at typical ambient outdoor radon concentrations is around 7%. Additional uncertainty associated with current calibration techniques, which inject calibration gas on top of ambient s led air, varies from 2-6%. Some objectives of the traceRadon project include establishing direct calibration traceability to the SI and developing an improved closed-loop calibration technique, using a new, low activity Radium-226 source. If successful, the absolute accuracy of the 200 L radon detector at typical ambient outdoor concentrations could be kept well below 15% for hourly observations. This project has received funding from the EMPIR programme co-financed by the Participating States and from the European Union's Horizon 2020 research and innovation programme. 19ENV01 traceRadon denotes the EMPIR project reference.& &
Publisher: Taiwan Association for Aerosol Research
Date: 2017
Publisher: Wiley
Date: 08-2019
DOI: 10.1002/ENG2.12026
Publisher: California Digital Library (CDL)
Date: 05-03-2019
Publisher: Copernicus GmbH
Date: 19-01-2016
DOI: 10.5194/AMT-2015-381
Abstract: Abstract. Dual-flow-loop two-filter radon detectors have a slow time response, which can affect the interpretation of their output when making continuous observations of near-surface atmospheric radon concentrations. While concentrations are routinely reported hourly, a calibrated model of detector performance shows that ∼40% of the signal arrives more than an hour after a radon pulse is delivered. After investigating several possible ways to correct for the detector’s slow time response, we show that a Bayesian approach using a Markov Chain Monte Carlo s ler is an effective method. After deconvolution, the detector’s output is redistributed into the appropriate counting interval and a 10 minute temporal resolution can be achieved under test conditions when the radon concentration is controlled. In the case of existing archived observations, collected under less ideal conditions, the data can be retrospectively reprocessed at 30 minute resolution. In one case study, we demonstrate that a deconvolved radon time series was consistent with: measurements from a fast-response carbon dioxide monitor grab s les from an aircraft and a simple mixing height model. In another case study, a bias of 18% in the mean daily minimum radon concentration was eliminated by correcting for the instrument response during a period of stable nights and days with well-developed convective boundary layers.
Publisher: Copernicus GmbH
Date: 28-01-2011
DOI: 10.5194/ACPD-11-3251-2011
Abstract: Abstract. The radioactive decay of radon and its progeny can lead to ionization of air molecules and consequently influence aerosol size distribution. In order to provide a global estimate of the radon-related ionization rate, we use the global atmospheric model ECHAM5 to simulate transport and decay processes of the radioactive tracers. A global radon emission map is put together using regional fluxes reported recently in the literature. The near-surface radon concentrations simulated with this new map compare well with measurements. Radon-related ionization rate is calculated and compared to that caused by cosmic rays. The contribution of radon and its progeny clearly exceeds that of the cosmic rays in the mid- and low-latitude land areas in the surface layer. In winter, strong radon-related ionization coincides with low temperature in China, USA, and Russia, providing favorable condition for the formation of aerosol particles. This suggests that it is probably useful to include the radon-induced ionization in global models when investigating the interaction between aerosol and climate.
Publisher: Copernicus GmbH
Date: 08-10-2014
DOI: 10.5194/ACPD-14-25411-2014
Abstract: Abstract. Radon is increasingly being used as a tool for quantifying stability influences on urban pollutant concentrations. Bulk radon gradients are ideal for this purpose, since the vertical differencing substantially removes contributions from processes on timescales greater than diurnal and (assuming a constant radon source) gradients are directly related to the intensity of nocturnal mixing. More commonly, however, radon measurements are available only at a single height. In this study we argue that single-height radon observations should not be used quantitatively as an indicator of atmospheric stability without prior conditioning of the time series to remove contributions from larger-scale "non-local" processes. We outline a simple technique to obtain an approximation of the diurnal radon gradient signal from a single-height measurement time series, and use it to derive a 4-category classification scheme for atmospheric stability on a "whole night" basis. A selection of climatological and pollution observations in the Sydney region are then sub ided according to the radon-based scheme on an annual and seasonal basis. We compare the radon-based scheme against a commonly-used Pasquil-Gifford (P-G) type stability classification and reveal that the most stable category in the P-G scheme is less selective of the strongly stable nights than the radon-based scheme this lead to significant underestimation of pollutant concentrations on the most stable nights by the P-G scheme. Lastly, we applied the radon-based classification scheme to mixing height estimates calculated from the diurnal radon accumulation time series, which provided insight to the range of nocturnal mixing depths expected at the site for each of the stability classes.
Publisher: MDPI AG
Date: 05-01-2022
DOI: 10.3390/ELECTRONICS11010169
Abstract: Next-generation communication systems and wearable technologies aim to achieve high data rates, low energy consumption, and massive connections because of the extensive increase in the number of Internet-of-Things (IoT) and wearable devices. These devices will be employed for many services such as cellular, environment monitoring, telemedicine, biomedical, and smart traffic, etc. Therefore, it is challenging for the current communication devices to accommodate such a high number of services. This article summarizes the motivation and potential of the 6G communication system and discusses its key features. Afterward, the current state-of-the-art of 5G antenna technology, which includes existing 5G antennas and arrays and 5G wearable antennas, are summarized. The article also described the useful methods and techniques of exiting antenna design works that could mitigate the challenges and concerns of the emerging 5G and 6G applications. The key features and requirements of the wearable antennas for next-generation technology are also presented at the end of the paper.
Publisher: InTech
Date: 15-11-2017
Publisher: Elsevier BV
Date: 11-2015
Publisher: IEEE
Date: 07-2018
Publisher: American Geophysical Union (AGU)
Date: 16-01-2013
DOI: 10.1029/2012JD018212
Publisher: Wiley
Date: 24-02-2016
DOI: 10.1002/MOP.29711
Publisher: Copernicus GmbH
Date: 23-06-2021
Abstract: Abstract. Aerosol measurements over the Southern Ocean have been identified as critical to an improved understanding of aerosol–radiation and aerosol–cloud interactions, as there currently exists significant discrepancies between model results and measurements in this region. The atmosphere above the Southern Ocean provides crucial insight into an aerosol regime relatively free from anthropogenic influence, yet its remoteness ensures atmospheric measurements are relatively rare. Here we present observations from the Polar Cell Aerosol Nucleation (PCAN) c aign, hosted aboard the RV Investigator during a summer (January–March) 2017 voyage from Hobart, Australia, to the East Antarctic seasonal sea ice zone. A median particle number concentration (condensation nuclei 3 nm CN3) of 354 (95 % CI 345–363) cm−3 was observed from the voyage. Median cloud condensation nuclei (CCN) concentrations were 167 (95 % CI 158–176) cm−3. Measured particle size distributions suggested that aerosol populations had undergone significant cloud processing. To understand the variability in aerosol observations, measurements were classified by meteorological variables. Wind direction and absolute humidity were used to identify different air masses, and aerosol measurements were compared based on these identifications. CN3 concentrations measured during SE wind directions (median 594 cm−3) were higher than those measured during wind directions from the NW (median 265 cm−3). Increased frequency of measurements from these wind directions suggests the influence of large-scale atmospheric transport mechanisms on the local aerosol population in the boundary layer of the East Antarctic seasonal ice zone. Modelled back trajectories imply different air mass histories for each measurement group, supporting this suggestion. CN3 and CCN concentrations were higher during periods where the absolute humidity was less than 4.3 gH2O/m3, indicative of free tropospheric or Antarctic continental air masses, compared to other periods of the voyage. Increased aerosol concentration in air masses originating close to the Antarctic coastline have been observed in numerous other studies. However, the smaller changes observed in the present analyses suggest seasonal differences in atmospheric circulation, including lesser impact of synoptic low-pressure systems in summer. Further measurements in the region are required before a more comprehensive picture of atmospheric circulation in this region can be captured and its influence on local aerosol populations understood.
Publisher: MDPI AG
Date: 27-11-2018
DOI: 10.3390/ATMOS9120466
Abstract: Poor air quality is often associated with hot weather, but the quantitative attribution of high temperatures on air quality remains unclear. In this study, the effect of elevated temperatures on air quality is investigated in Greater Sydney using January 2013, a period of extreme heat during which temperatures at times exceeded 40 ∘ C, as a case study. Using observations from 17 measurement sites and the Weather Research and Forecasting Chemistry (WRF-Chem) model, we analyse the effect of elevated temperatures on ozone in Sydney by running a number of sensitivity studies in which: (1) the model is run with biogenic emissions generated by MEGAN and separately run with monthly average Model of Emissions of Gases and Aerosols from Nature ( MEGAN) biogenic emissions (for January 2013) (2) the model results from the standard run are compared with those in which average temperatures (for January 2013) are only applied to the chemistry (3) the model is run using both averaged biogenic emissions and temperatures and (4 and 5) the model is run with half and zero biogenic emissions. The results show that the impact on simulated ozone through the effect of temperature on reaction rates is similar to the impact via the effect of temperature on biogenic emissions and the relative impacts are largely additive when compared to the run in which both are averaged. When averaged across 17 sites in Greater Sydney, the differences between ozone simulated under standard and averaged model conditions are as high as 16 ppbv. Removing biogenic emissions in the model has the effect of removing all simulated ozone episodes during extreme heat periods, highlighting the important role of biogenic emissions in Australia, where Eucalypts are a key biogenic source.
Publisher: MDPI AG
Date: 17-12-2018
DOI: 10.3390/ATMOS9120500
Abstract: We present findings from the Measurements of Urban, Marine and Biogenic Air (MUMBA) c aign, which took place in the coastal city of Wollongong in New South Wales, Australia. We focus on a few key air quality indicators, along with a comparison to regional scale chemical transport model predictions at a spatial resolution of 1 km by 1 km. We find that the CSIRO chemical transport model provides accurate simulations of ozone concentrations at most times, but underestimates the ozone enhancements that occur during extreme temperature events. The model also meets previously published performance standards for fine particulate matter less than 2.5 microns in diameter (PM2.5), and the larger aerosol fraction (PM10). We explore the observed composition of the atmosphere within this urban air-shed during the MUMBA c aign and discuss the different influences on air quality in the city. Our findings suggest that further improvements to our ability to simulate air quality in this coastal city can be made through more accurate anthropogenic and biogenic emissions inventories and better understanding of the impact of extreme temperatures on air quality. The challenges in modelling air quality within the urban air-shed of Wollongong, including difficulties in accurate simulation of the local meteorology, are likely to be replicated in many other coastal cities in the Southern Hemisphere.
Publisher: Copernicus GmbH
Date: 19-09-2012
Abstract: Abstract. Surface-based radon (222Rn) measurements can be combined with lidar backscatter to obtain a higher quality time series of mixing height within the Planetary Boundary-Layer (PBL) than is possible from lidar alone, and a more quantitative measure of mixing height than is possible from only radon. The lidar measurements benefit because even when aerosol layers are detected, reliably attributing the mixing height to the correct layer presents a challenge. By combining lidar with a mixing length scale derived from a time series of radon concentration, automated and robust attribution is possible during the morning transition. Radon measurements also provide mixing information during the night and with the addition of lidar these measurements become insensitive to night-to-night changes in radon emissions. After calibration with lidar, the radon-derived equivalent mixing height agrees with other measures of mixing on daily and hourly time scales and is a potential method for studying intermittent mixing in nocturnal boundary layers.
Publisher: Elsevier BV
Date: 04-2015
Publisher: Wiley
Date: 12-11-2022
DOI: 10.1002/MOP.33499
Abstract: With the advanced communications systems, the integration of 5G bands, including sub‐6‐GHz and millimeter‐wave (mm‐wave) bands with the existing lower bands of 3G/4G has become an essential need for the future mobile handsets. This article proposes an integration between a large‐frequency‐ratio dual‐band tapered slot antenna with a multisection meander monopole antenna on a handset board. The tapered slot Vivaldi antenna (TSVA) functions as a resonant open‐ended slot at low frequencies (sub‐6 GHz) while also acting as a high‐gain Vivaldi antenna at higher frequencies (mm‐wave 28 GHz). The modification of the slot geometry, that is, generating multisections within the slot, is shown to improve the impedance bandwidth. Furthermore, the meander‐line monopole antenna covers the bands of the existing mobile generation (3G/4G) at 0.8, 1.8, 2.1, and 2.3 GHz. Most importantly, the compact size of the proposed antenna is realized by utilizing the side wall of a mobile board.
Publisher: Elsevier BV
Date: 02-2017
DOI: 10.1016/J.SCITOTENV.2016.09.151
Abstract: The combined influences of recent mitigation measures on urban air quality have been assessed using hourly observations of the criteria air pollutants (NO, NO
Publisher: Copernicus GmbH
Date: 07-09-2022
DOI: 10.5194/ACP-2022-568
Abstract: Abstract. The remoteness and extreme conditions of the Southern Ocean and Antarctic region have meant that observations in this region are rare, and typically restricted to summertime during research or resupply voyages. Observations of aerosols outside of the summer season are typically limited to long-term stations, such as Kennaook/Cape Grim (KCG, 40.7° S, 144.7° E) which is situated in the northern latitudes of the Southern Ocean, and Antarctic research stations, such as the Japanese operated Syowa (SYO, 69.0° S, 39.6° E). Measurements in the mid-latitudes of the Southern Ocean are important, particularly in light of recent observations that highlighted the latitudinal gradient that exists across the region in summertime. Here we present two years (March 2016–March 2018) of observations from Macquarie Island (MQI, 54.5° S, 159.0° E) of aerosol (condensation nuclei larger than 10 nm, CN10) and cloud condensation nuclei (CCN at various supersaturations) concentrations. This important multi-year data set is characterised, and its features are compared with the long-term data sets from KCG and SYO together with those from recent, regionally relevant voyages. CN10 concentrations were the highest at KCG by a factor of ∼50 % across all non-winter seasons compared to the other two stations which were similar (summer medians of 530 cm-3, 426 cm-3 and 468 cm-3 at KCG, MQI and SYO, respectively). In wintertime, seasonal minima at KCG and MQI were similar (142 cm-3 and 152 cm-3, respectively), with SYO being distinctly lower (87 cm-3), likely the result of the reduction in sea spray aerosol generation due to the sea-ice ocean cover around the site. CN10 seasonal maxima were observed at the stations at different times of year, with KCG and MQI exhibiting January maxima and SYO having a distinct February high. Comparison of CCN0.5 data between KCG and MQI showed similar overall trends with summertime maxima and wintertime minima, however KCG exhibited slightly (∼10 %) higher concentrations in summer (medians of 158 cm-3 and 145 cm-3, respectively), whereas KCG showed ∼40 % lower concentrations than MQI in winter (medians of 57 cm-3 and 92 cm-3, respectively). Spatial and temporal trends in the data were analysed further by contrasting data to coincident observations that occurred aboard several voyages of the RSV Aurora Australis and the RV Investigator. Results from this study are important for validating and improving our models, highlight the heterogeneity of this pristine region, and the need for further long-term observations that capture the seasonal cycles.
Publisher: Elsevier BV
Date: 02-2020
Publisher: Wiley
Date: 02-07-2021
Publisher: Copernicus GmbH
Date: 06-06-2017
Abstract: Abstract. The Measurements of Urban, Marine and Biogenic Air (MUMBA) c aign took place in Wollongong, New South Wales (a small coastal city approximately 80 km south of Sydney, Australia) from 21 December 2012 to 15 February 2013. Like many Australian cities, Wollongong is surrounded by dense eucalyptus forest, so the urban airshed is heavily influenced by biogenic emissions. Instruments were deployed during MUMBA to measure the gaseous and aerosol composition of the atmosphere with the aim of providing a detailed characterisation of the complex environment of the ocean–forest–urban interface that could be used to test the skill of atmospheric models. The gases measured included ozone, oxides of nitrogen, carbon monoxide, carbon dioxide, methane and many of the most abundant volatile organic compounds. The aerosol characterisation included total particle counts above 3 nm, total cloud condensation nuclei counts, mass concentration, number concentration size distribution, aerosol chemical analyses and elemental analysis.The c aign captured varied meteorological conditions, including two extreme heat events, providing a potentially valuable test for models of future air quality in a warmer climate. There was also an episode when the site s led clean marine air for many hours, providing a useful additional measure of the background concentrations of these trace gases within this poorly s led region of the globe. In this paper we describe the c aign, the meteorology and the resulting observations of atmospheric composition in general terms in order to equip the reader with a sufficient understanding of the Wollongong regional influences to use the MUMBA datasets as a case study for testing a chemical transport model. The data are available from PANGAEA (doi.pangaea.de/10.1594/PANGAEA.871982).
Publisher: Stockholm University Press
Date: 11-2011
Publisher: Wiley
Date: 13-10-2021
Publisher: Wiley
Date: 03-12-2021
Publisher: The Electromagnetics Academy
Date: 2019
Publisher: Copernicus GmbH
Date: 21-03-2022
Abstract: Abstract. We assess the performance of an isotope ratio infrared spectrometer (IRIS) to measure carbon (δ13C) and oxygen (δ18O) isotope ratios in atmospheric carbon dioxide (CO2) and report observations from a 26 d field deployment trial at Baring Head, New Zealand, NIWA's atmospheric observatory for Southern Ocean baseline air. Our study describes an operational method to improve the performance in comparison to previous publications on this analytical instrument. By using a calibration technique that reflected the principle of identical treatment of s le and reference gases, we achieved a reproducibility of 0.07 ‰ for δ13C-CO2 and 0.06 ‰ for δ18O-CO2 over multiple days. This performance is within the extended compatibility goal of 0.1 ‰ for both δ13C-CO2 and δ18O-CO2, which was recommended by the World Meteorological Organization (WMO). Further improvement in measurement performance is desirable to also meet the WMO network compatibility goals of 0.01 ‰ for δ13C-CO2 and 0.05 ‰ for δ18O-CO2, which is needed to resolve the small variability that is typical for background air observatories such as Baring Head. One objective of this study was to assess the capabilities and limitations of the IRIS analyser to resolve δ13C-CO2 and δ18O-CO2 variations under field conditions. Therefore, we selected multiple events within the 26 d record for Keeling plot analysis. This resolved the isotopic composition of endmembers with an uncertainty of ≤ 1 ‰ when the magnitude of CO2 signals is larger than 10 ppm. The uncertainty of the Keeling plot analysis strongly increased for smaller CO2 events (2–7 ppm), where the instrument performance is the limiting factor and may only allow for the distinction between very different endmembers, such as the role of terrestrial versus oceanic carbon cycle processes.
Publisher: Copernicus GmbH
Date: 30-06-2016
Abstract: Abstract. The stable isotopic composition of water vapour provides information about moisture sources and processes that is difficult to obtain with traditional measurement techniques. Recently, it has been proposed that the D-excess (dv = δ2H − 8 × δ18O) of water vapour can provide a diagnostic tracer of continental moisture recycling. However, D-excess exhibits a diurnal cycle that has been observed across a variety of ecosystems and may be influenced by a range of processes beyond regional scale moisture recycling, including local evaporation (ET) fluxes. There is a lack of measurements of D-excess in evaporation (ET) fluxes, which has made it difficult to assess how ET fluxes modify the D-excess in water vapour (dv). With this in mind, we employed a chamber based approach to directly measure D-excess in ET (dET) fluxes. We show that ET fluxes imposed a negative forcing on the ambient vapour and could not explain the higher daytime dv values. The low dET observed here was sourced from a soil water pool that had undergone an extended drying period, leading to low D-excess of the soil moisture. A strong correlation between daytime dv and locally measured relative humidity was consistent with an oceanic moisture source, suggesting that remote hydrological processes were the major contributor to daytime dv variability. During the early evening, ET fluxes into a shallow nocturnal inversion layer caused a lowering of the dv values near the surface. In addition, transient mixing of vapour with a higher D-excess from above the nocturnal inversion modified these values, causing large within night variability. These results indicate dET can generally be expected to show large spatial and temporal variability and to depend on the soil moisture state. For long periods between rain events, common in semi-arid environments, ET would be expected to impose negative forcing on the surface dv. The variability of D-excess in ET fluxes therefore needs to be considered when using dv to study moisture recycling and during extended dry periods may act as a tracer of the relative humidity of the oceanic moisture source.
Publisher: American Geophysical Union (AGU)
Date: 29-12-2022
DOI: 10.1029/2021JD035433
Abstract: The factors driving variability in rainfall stable water isotopes (specifically δ 18 O and deuterium excess, d = δ 2 H − 8 δ 18 O) were studied in a 13‐year data set of daily rainfall s les from coastal southwestern Western Australia (SWWA). Backwards dispersion modeling, automatic synoptic type classification, and a statistical model were used to establish causes of variability on a daily scale and predictions from the model were aggregated to longer temporal scales to discover the cause of variability on multiple timescales. Factors differ between δ 18 O and d and differ according to temporal scale. Rainfall intensity, both at the observation site and upwind, was most important for determining δ 18 O and this relationship was robust across all time scales (daily, seasonal, and interannual) as well as generalizing to a second observation site. The sensitivity of δ 18 O to rainfall intensity makes annual mean values particularly sensitive to the year's largest events. Projecting the rainfall intensity relationship back through ∼100 years of precipitation observations can explain ∼ –0.4‰ shifts in rainfall δ 18 O. Twentieth century speleothem records from the region exhibit signals of a similar magnitude, indicating that rainfall intensity should be taken into account during the interpretation of regional climate archives. For d , humidity during evaporation from the ocean was the most important driver of variability at the daily scale, as well as explaining the seasonal cycle, but source humidity failed to explain the longer‐term interannual variability.
Publisher: MDPI AG
Date: 28-08-2020
DOI: 10.3390/ELECTRONICS9091394
Abstract: In this study, a compact dual-band combined loop-slot planar antenna is proposed. (1) Background: multi-function antennas are desired for wireless communication to cover the desired frequency spectrum. (2) Methods: the proposed antenna consists of a semi-rectangular open-ended loop (OEL) operating at the lower frequency band 920 MHz, an open-ended slot (OES) transmission line that provides resonance at the higher band 2.4 GHz, and a feeding port using the asymmetric coplanar strip (ACS) line. The ACS is used to excite the antenna to achieve dual-band performance. The overall dimensions of the fabricated prototype are 32.5 × 53.5 mm2 (0.1λo×0.16λo), where λo represents the free-space wavelength at the lower frequency. (3) Results: from the calculations, the antenna shows two impedance bandwidths (estimated at −10dB) of 30 MHz (920–950 MHz) and 300 MHz (2.2–2.5 GHz) to cover the ISM band (920 MHz) and 2.45 GHz WiFi bands, respectively. Indeed, the antenna has stable radiation patterns and achieves peak measured realized gain of 1.8 dBi in the lower band and 4.2 dBi in the higher band. (4) Conclusion: the antenna shows the merits of low profile structure, single-layer, and low-cost fabrication. The proposed antenna not only achieves incremental increase in radiation efficiency, but also provides a lightweight, and small footprint.
Publisher: Copernicus GmbH
Date: 02-02-2015
Abstract: Abstract. Radon is increasingly being used as a tool for quantifying stability influences on urban pollutant concentrations. Bulk radon gradients are ideal for this purpose, since the vertical differencing substantially removes contributions from processes on timescales greater than diurnal and (assuming a constant radon source) gradients are directly related to the intensity of nocturnal mixing. More commonly, however, radon measurements are available only at a single height. In this study we argue that single-height radon observations should not be used quantitatively as an indicator of atmospheric stability without prior conditioning of the time series to remove contributions from larger-scale "non-local" processes. We outline a simple technique to obtain an approximation of the diurnal radon gradient signal from a single-height measurement time series, and use it to derive a four category classification scheme for atmospheric stability on a "whole night" basis. A selection of climatological and pollution observations in the Sydney region are then sub ided according to the radon-based scheme on an annual and seasonal basis. We compare the radon-based scheme against a commonly used Pasquill–Gifford (P–G) type stability classification and reveal that the most stable category in the P–G scheme is less selective of the strongly stable nights than the radon-based scheme this lead to significant underestimation of pollutant concentrations on the most stable nights by the P–G scheme. Lastly, we applied the radon-based classification scheme to mixing height estimates calculated from the diurnal radon accumulation time series, which provided insight to the range of nocturnal mixing depths expected at the site for each of the stability classes.
Publisher: Copernicus GmbH
Date: 18-05-2022
Abstract: Abstract. Little overlap exists in the required capabilities of 222Rn (radon) monitors for public health and atmospheric research. The former requires robust, compact, easily transportable instruments to characterise daily to yearly variability Bq m−3, whereas the latter requires static instruments capable of characterising sub-hourly variability between 0.1 and 100 Bq m−3. Consequently, detector development has evolved independently for the two research communities, and while many radon measurements are being made world-wide, the full potential of this measurement network can't be realised because not all results are comparable. Development of a monitor that satisfies the primary needs of both measurement communities, including a calibration traceable to the International System of Units (SI), would constitute an important step toward (i) increasing the availability of radon measurements to both research communities, and (ii) providing a means to harmonize and compare radon measurements across the existing eclectic global network of radon detectors. To this end, we describe a prototype detector built by the Australian Nuclear Science and Technology Organisation (ANSTO), in collaboration with the EMPIR 19ENV01 traceRadon Project and Physikalisch-Technische Bundesanstalt (PTB). This two-filter dual-flow-loop radon monitor can be transported in a standard vehicle, fits in a 19′′ instrument rack, has a 30 min temporal resolution, and a detection limit of ∼0.14 Bq m−3. It is capable of continuous, long-term, low-maintenance, low-power, indoor or outdoor monitoring with a high sensitivity and an uncertainty of ∼15 % at 1 Bq m−3. Furthermore, we demonstrate the successful transfer of an SI traceable calibration from this portable monitor to a 1500 L two-filter radon monitor under field conditions.
Publisher: Elsevier BV
Date: 05-2015
DOI: 10.5094/APR.2015.059
Publisher: Taiwan Association for Aerosol Research
Date: 2015
Publisher: MDPI AG
Date: 12-01-2023
DOI: 10.3390/RS15020461
Abstract: A comparative study and evaluation of boundary layer height (BLH) estimation was conducted during an experimental c aign conducted at the Cape Grim Air Pollution station, Australia, from 1 June to 13 July 2019. The temporal and spatial distributions of BLH were studied using data from a ceilometer, sodar, in situ meteorological measurements, and back-trajectory analyses. Generally, the BLH under continental sources is lower than that under marine sources. The BLH is featured with a shallow depth of 515 ± 340 m under the Melbourne/East Victoria continental source. Especially the mixed continental sources (Melbourne/East Victoria and Tasmania direction) lead to a rise in radon concentration and lower BLH. In comparison, the boundary layer reaches a higher averaged BLH value of 730 ± 305 m when marine air is prevalent. The BLH derived from ERA5 is positively biased compared to the ceilometer observations, except when the boundary layer is stable. The height at which wind profiles experience rapid changes corresponds to the BLH value. The wind flow within the boundary layer increased up to ∼200 m, where it then meandered up to ∼300 m. Furthermore, the statistic shows that BLH is positively associated with near-surface wind speed. This study firstly provides information on boundary layer structure in Cape Grim and the interaction with wind, which may aid in further evaluating their associated impacts on the climate and ecosystem.
Publisher: Elsevier BV
Date: 04-2016
DOI: 10.1016/J.JENVRAD.2016.01.010
Abstract: A radon-based nocturnal stability classification scheme is developed for a flat inland site near Bucharest, Romania, characterised by significant local surface roughness heterogeneity, and compared with traditional meteorologically-based techniques. Eight months of hourly meteorological and atmospheric radon observations from a 60 m tower at the IFIN-HH nuclear research facility are analysed. Heterogeneous surface roughness conditions in the 1 km radius exclusion zone around the site hinder accurate characterisation of nocturnal atmospheric mixing conditions using conventional meteorological techniques, so a radon-based scheme is trialled. When the nocturnal boundary layer is very stable, the Pasquill-Gifford "radiation" scheme overestimates the atmosphere's capacity to dilute pollutants with near-surface sources (such as tritiated water vapour) by 20% compared to the radon-based scheme. Under these conditions, near-surface wind speeds drop well below 1 m s(-1) and nocturnal mixing depths vary from ∼ 25 m to less than 10 m above ground level (a.g.l.). Combining nocturnal radon with daytime ceilometer data, we were able to reconstruct the full diurnal cycle of mixing depths. Average daytime mixing depths at this flat inland site range from 1200 to 1800 m a.g.l. in summer, and 500-900 m a.g.l. in winter. Using tower observations to constrain the nocturnal radon-derived effective mixing depth, we were able to estimate the seasonal range in the Bucharest regional radon flux as: 12 mBq m(-2) s(-1) in winter to 14 mBq m(-2) s(-1) in summer.
Publisher: MDPI AG
Date: 04-12-2019
Abstract: This paper presents a summary of the key findings of the special issue of Atmosphere on Air Quality in New South Wales and discusses the implications of the work for policy makers and in iduals. This special edition presents new air quality research in Australia undertaken by (or in association with) the Clean Air and Urban Landscapes hub, which is funded by the National Environmental Science Program on behalf of the Australian Government’s Department of the Environment and Energy. Air pollution in Australian cities is generally low, with typical concentrations of key pollutants at much lower levels than experienced in comparable cities in many other parts of the world. Australian cities do experience occasional exceedances in ozone and PM2.5 (above air pollution guidelines), as well as extreme pollution events, often as a result of bushfires, dust storms, or heatwaves. Even in the absence of extreme events, natural emissions play a significant role in influencing the Australian urban environment, due to the remoteness from large regional anthropogenic emission sources. By studying air quality in Australia, we can gain a greater understanding of the underlying atmospheric chemistry and health risks in less polluted atmospheric environments, and the health benefits of continued reduction in air pollution. These conditions may be representative of future air quality scenarios for parts of the Northern Hemisphere, as legislation and cleaner technologies reduce anthropogenic air pollution in European, American, and Asian cities. However, in many instances, current legislation regarding emissions in Australia is significantly more lax than in other developed countries, making Australia vulnerable to worsening air pollution in association with future population growth. The need to avoid complacency is highlighted by recent epidemiological research, reporting associations between air pollution and adverse health outcomes even at air pollutant concentrations that are lower than Australia’s national air quality standards. Improving air quality is expected to improve health outcomes at any pollution level, with specific benefits projected for reductions in long-term exposure to average PM2.5 concentrations.
Publisher: Springer Science and Business Media LLC
Date: 09-08-2013
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 10-2021
Publisher: Taiwan Association for Aerosol Research
Date: 2016
Publisher: Copernicus GmbH
Date: 30-06-2016
Publisher: Copernicus GmbH
Date: 03-08-2011
Abstract: Abstract. The radioactive decay of radon and its progeny can lead to ionization of air molecules and consequently influence aerosol size distribution. In order to provide a global estimate of the radon-related ionization rate, we use the global atmospheric model ECHAM5 to simulate transport and decay processes of the radioactive tracers. A global radon emission map is put together using regional fluxes reported recently in the literature. Near-surface radon concentrations simulated with this new map compare well with measurements. Radon-related ionization rate is calculated and compared to that caused by cosmic rays. The contribution of radon and its progeny clearly exceeds that of the cosmic rays in the mid- and low-latitude land areas in the surface layer. During cold seasons, at locations where high concentration of sulfuric acid gas and low temperature provide potentially favorable conditions for nucleation, the coexistence of high ionization rate may help enhance the particle formation processes. This suggests that it is probably worth investigating the impact of radon-induced ionization on aerosol-climate interaction in global models.
Publisher: Elsevier BV
Date: 11-2016
Publisher: Copernicus GmbH
Date: 08-05-2014
DOI: 10.5194/ACPD-14-11541-2014
Abstract: Abstract. We report on one year of high precision direct hourly radon observations at King Sejong Station (King George Island) beginning in February 2013. Findings are compared with historic and ongoing radon measurements from other Antarctic sites. Monthly median concentrations reduced from 72 mBq m−3 in late summer to 44 mBq m−3 in late-winter and early-spring. Monthly 10th percentiles, ranging from 29 to 49 mBq m−3, were typical of oceanic baseline values. Diurnal cycles were rarely evident and local influences were minor, consistent with regional radon flux estimates one tenth of the global average for ice-free land. The predominant fetch region for terrestrially influenced air masses was South America (47–53° S), with minor influences also attributed to aged Australian air masses and local sources. Plume dilution factors of 2.8–4.0 were estimated for the most terrestrially influenced (South American) air masses, and a seasonal cycle in terrestrial influence on tropospheric air descending at the pole was identified and characterised.
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 06-2022
Publisher: Copernicus GmbH
Date: 26-11-2020
Abstract: Abstract. Aerosol measurements over the Southern Ocean have been identified as critical to an improved understanding of aerosol-radiation and aerosol-cloud interactions, as there currently exists significant discrepancies between model results and measurements in this region. Previous springtime measurements from the East Antarctic seasonal ice zone revealed a significant increase in aerosol number concentrations when crossing the atmospheric polar front into the Polar cell. A return voyage in summer 2017 made a more extensive range of aerosols measurements, including in particular aerosol number concentrations and submicron size distributions. Again, significantly greater aerosol number concentrations were observed in the Polar cell than in the Ferrel cell. Unlike the previous spring voyage however, the polar front was unable to be identified by a step change in aerosol concentration. A possible explanation is that atmospheric mixing across the polar front occurs to a greater degree in summer, therefore weakening the atmospheric boundary at the front. This atmospheric mixing in summer complicates the determination of the polar front location. These changes, together with the increased source of precursors from phytoplankton emissions, are likely to explain the seasonal differences observed in the magnitude of aerosol populations between the Ferrel and Polar cell. In the present analysis, meteorological variables were used to identify different air-masses and then aerosol measurements were compared based on these identifications. CN3 concentrations measured during wind directions indicative of Polar cell airmasses (median 594 cm−3) were larger than those measured during wind directions indicative of Ferrel cell air (median 265 cm−3). CN3 and CCN concentrations were larger during periods where the absolute humidity was less than 4.3 gH2O/m3, indicative of free tropospheric or Antarctic continental airmasses, compared to other periods of the voyage. These results indicate that a persistently more concentrated aerosol population is present in the Polar cell over the East Antarctic seasonal ice zone, although the observed difference between the two cells may vary seasonally.
Publisher: Copernicus GmbH
Date: 21-12-2016
DOI: 10.5194/CP-2016-135
Abstract: Abstract. Terrestrial data spanning the Last Glacial Maximum (LGM) and deglaciation from the southern Australian region are sparse, and limited to discontinuous sedimentological and geomorphological records with relatively large chronological uncertainties. This dearth of records has prevented a critical assessment of the role of the Southern Hemisphere mid-latitude westerly winds on the region’s climate during this time period. In this study, two precisely-dated speleothem records for Mairs Cave, Flinders Ranges, are presented, providing a detailed terrestrial hydroclimatic record for the southern Australian drylands during 23–15 ka for the first time. Enhanced recharge to Mairs Cave is interpreted from the speleothem record by the activation of growth, physical flood layering and δ18O and δ13C minima. Periods of lowered recharge are indicated by isotopic enrichment, primarily affecting δ18O, argued to be driven by evaporation of shallow soil/epikarst water in this water-limited environment. A hydrological driver is supported by calcite fabric changes. The Mairs Cave record indicates that the Flinders Ranges were relatively wet during the LGM and early deglaciation, particularly over the interval 18.9–16 ka. This wetter phase ended abruptly with a shift to drier conditions at 15.8 ka. These findings are in agreement with the geomorphic archives for this region, as well as the timing of events in records from the broader Australasian region. The recharge phases identified in the Mairs Cave record are correlated with, but antiphase to, the position of the westerly winds interpreted from a marine core in the Great Australian Bight. The implication is that the mid-latitude westerlies are located further south during the period of enhanced recharge in the Mairs Cave record (18.9–16 ka), and conversely are located further north when greater aridity is interpreted in the speleothem record. A comparison with speleothem records from the northern Australasian region reveals that the availability of sub-tropical/tropical moisture is the most likely explanation driving enhanced recharge, with further lification of recharge occurring during the early half of Heinrich Stadial 1, possibly influenced by a more southerly-displaced Intertropical Convergence Zone (ITCZ). A rapid transition to aridity at 15.8 ka is consistent with a retraction of this tropical moisture source.
Publisher: Copernicus GmbH
Date: 13-05-2019
DOI: 10.5194/ESSD-2019-56
Abstract: Abstract. The Sydney Particle Study involved the comprehensive measurement of meteorology, particles and gases at a location in western Sydney during February/March 2011 and April/May 2012. The aim of this study was to increase scientific knowledge of the processes leading to particle formation and transformations in Sydney. In this paper we describe the methods used to collect and analyse particle and gaseous s les, as well as the methods employed for the continuous measurement of particle concentrations, particle microphysical properties and gaseous concentrations. This paper also provides a description of the data collected and is a meta data record for the data sets published in Keywood et al. (2016a) 0.4225/08/57903B83D6A5D and Keywood et al. (2016b) 0.4225/08/5791B5528BD63.
Publisher: American Geophysical Union (AGU)
Date: 27-01-2019
DOI: 10.1029/2018JD029507
Publisher: Taiwan Association for Aerosol Research
Date: 2016
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 2020
Publisher: Copernicus GmbH
Date: 21-12-2016
Publisher: Springer Science and Business Media LLC
Date: 09-06-2023
DOI: 10.1038/S43247-023-00858-7
Abstract: Billions of people worldwide rely on groundwater. As rainfall in many regions in the future is projected to decrease, it is critical to understand the impacts of climate change on groundwater recharge. The groundwater recharge response to a sustained decrease in rainfall across southwest Australia that began in the late 1960s was examined in seven modern speleothems and drip waters from four caves. These show a pronounced increase or uptick in regional drip water and speleothem oxygen isotopic composition (δ 18 O) that is not driven by a change in rainfall δ 18 O values, but is in response to the shallow karst aquifers becoming disconnected from rainfall recharge due to regional drying. Our findings imply that rainfall recharge to groundwater may no longer be reliably occurring in this region, which is highly dependent on groundwater resources. Examination of the longer speleothem record shows that this situation is unprecedented over the last 800 years.
Publisher: Elsevier BV
Date: 10-2015
Publisher: MDPI AG
Date: 16-05-2023
DOI: 10.3390/S23104782
Abstract: Since the CubeSats have become inherently used for the Internet of space things (IoST) applications, the limited spectral band at the ultra-high frequency (UHF) and very high frequency should be efficiently utilized to be sufficient for different applications of CubeSats. Therefore, cognitive radio (CR) has been used as an enabling technology for efficient, dynamic, and flexible spectrum utilization. So, this paper proposes a low-profile antenna for cognitive radio in IoST CubeSat applications at the UHF band. The proposed antenna comprises a circularly polarized wideband (WB) semi-hexagonal slot and two narrowband (NB) frequency reconfigurable loop slots integrated into a single-layer substrate. The semi-hexagonal-shaped slot antenna is excited by two orthogonal +/−45° tapered feed lines and loaded by a capacitor in order to achieve left/right-handed circular polarization in wide bandwidth from 0.57 GHz to 0.95 GHz. In addition, two NB frequency reconfigurable slot loop-based antennas are tuned over a wide frequency band from 0.6 GHz to 1.05 GH. The antenna tuning is achieved based on a varactor diode integrated into the slot loop antenna. The two NB antennas are designed as meander loops to miniaturize the physical length and point in different directions to achieve pattern ersity. The antenna design is fabricated on FR-4 substrate, and measured results have verified the simulated results.
Publisher: Elsevier BV
Date: 11-2016
Publisher: Optica Publishing Group
Date: 11-2005
DOI: 10.1364/AO.44.006653
Abstract: A sensor based on tunable diode laser absorption spectroscopy was constructed for time-resolved temperature and water vapor concentration measurements in a scramjet combustor. The sensor probed two absorption lines near 1390 nm with two time-multiplexed lasers used to measure temperature and water vapor concentration at up to 20 kHz. A demonstration experiment was performed in the supersonic, expanding exhaust region of the combustor, showing the measurement to be repeatable, able to resolve temporal trends during tunnel operation, and sensitive to changes in combustor operating conditions.
Publisher: Elsevier BV
Date: 02-2016
Publisher: MDPI AG
Date: 31-12-2020
Abstract: Volatile organic compounds (VOCs) play a key role in the formation of ozone and secondary organic aerosol, the two most important air pollutants in Sydney, Australia. Despite their importance, there are few available VOC measurements in the area. In this paper, we discuss continuous GC-MS measurements of 10 selected VOCs between February (summer in the southern hemisphere) and June (winter in the southern hemisphere) of 2019 in a semi-urban area between natural eucalypt forest and the Sydney metropolitan fringe. Combined, isoprene, methacrolein, methyl-vinyl-ketone, α-pinene, p-cymene, eucalyptol, benzene, toluene xylene and tri-methylbenzene provide a reasonable representation of variability in the total biogenic VOC (BVOC) and anthropogenic VOC (AVOC) loading in the area. Seasonal changes in environmental conditions were reflected in observed BVOC concentrations, with a summer peak of 8 ppb, dropping to approximately 0.1 ppb in winter. Isoprene, and its immediate oxidation products methacrolein (MACR) and methyl-vinyl-ketone (MVK), dominated BVOC concentrations during summer and early autumn, while monoterpenes comprised the larger fraction during winter. Temperature and solar radiation drive most of the seasonal variation observed in BVOCs. Observed levels of isoprene, MACR and MVK in the atmosphere are closely related with variations in temperature and photosynthetically active radiation (PAR), but chemistry and meteorology may play a more important role for the monoterpenes. Using a nonlinear model, temperature explains 51% and PAR 38% of the isoprene, MACR and MVK variation. Eucalyptol dominated the observed monoterpene fraction (contributing ~75%), with p-cymene (20%) and α-pinene (5%) also present. AVOCs maintain an average concentration of ~0.4 ppb, with a slight decrease during autumn–winter. The low AVOC concentrations observed indicate a relatively small anthropogenic influence, generally occurring when (rare) northerly winds transport Sydney emissions to the measurement site. The site is influenced by domestic, commercial and vehicle AVOC emissions. Our observed AVOC concentrations can be explained by the seasonal changes in meteorology and the emissions in the area as listed in the NSW emissions inventory and thereby act as an independent validation of this inventory. We conclude that the variations in atmospheric composition observed during the seasons are an important variable to consider when formulating air pollution control policies over Sydney given the influence of biogenic sources during summer, autumn and winter.
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 04-2022
Publisher: MDPI AG
Date: 28-01-2020
DOI: 10.3390/S20030713
Abstract: This paper introduces a novel antenna array synthesis for radar systems based on the concept of a virtual antenna array (VAA) and the method of moments/genetic algorithm (MoM/GA) synthesis method. The VAA concept is applied to both scanning and fixed radiation pattern arrays. The proposed VAA is introduced to simultaneously support the medium-range radar (MRR) and the long-range radar (LRR) with beam width ±7° for LRR and ±37° for MRR. The proposed VAA is distinguished by its minimum number of antenna elements, simple feeding network, high efficiency, and gain, but all of these are at the expense of a large aperture antenna size compared to the planar antenna array (PAA). The VAA has the ability to have the feeding network and the radiating elements on the same layer, as compared to the multilayer PAA. The newly proposed concept is analyzed and verified analytically and experimentally. Two orthogonal (16 elements) VAAs are designed to operate in the frequency range from 23.55 to 24.7 GHz and to support a flat-shoulder shape (FSS) radiation pattern for LRR/MRR. The antenna was fabricated and tested experimentally, and good agreements between the simulated and measured results were noticed. The proposed VAA is introduced to solve the problems of large size, low isolations, low efficiency, feeding network, low resolution, and small coverage range for the antenna arrays of automotive radars. The proposed antenna array is introduced for automotive radar applications at 24 GHz.
Publisher: MDPI AG
Date: 11-01-2019
Abstract: We propose a new technique to prepare statistically-robust benchmarking data for evaluating chemical transport model meteorology and air quality parameters within the urban boundary layer. The approach employs atmospheric class-typing, using nocturnal radon measurements to assign atmospheric mixing classes, and can be applied temporally (across the diurnal cycle), or spatially (to create angular distributions of pollutants as a top-down constraint on emissions inventories). In this study only a short ( -month) c aign is used, but grouping of the relative mixing classes based on nocturnal mean radon concentrations can be adjusted according to dataset length (i.e., number of days per category), or desired range of within-class variability. Calculating hourly distributions of observed and simulated values across diurnal composites of each class-type helps to: (i) bridge the gap between scales of simulation and observation, (ii) represent the variability associated with spatial and temporal heterogeneity of sources and meteorology without being confused by it, and (iii) provide an objective way to group results over whole diurnal cycles that separates ‘natural complicating factors’ (synoptic non-stationarity, rainfall, mesoscale motions, extreme stability, etc.) from problems related to parameterizations, or between-model differences. We demonstrate the utility of this technique using output from a suite of seven contemporary regional forecast and chemical transport models. Meteorological model skill varied across the diurnal cycle for all models, with an additional dependence on the atmospheric mixing class that varied between models. From an air quality perspective, model skill regarding the duration and magnitude of morning and evening “rush hour” pollution events varied strongly as a function of mixing class. Model skill was typically the lowest when public exposure would have been the highest, which has important implications for assessing potential health risks in new and rapidly evolving urban regions, and also for prioritizing the areas of model improvement for future applications.
Publisher: Copernicus GmbH
Date: 18-09-2014
Abstract: Abstract. We report on one year of high-precision direct hourly radon observations at King Sejong Station (King George Island) beginning in February 2013. Findings are compared with historic and ongoing radon measurements from other Antarctic sites. Monthly median concentrations reduced from 72 mBq m−3 in late-summer to 44 mBq m−3 in late winter and early spring. Monthly 10th percentiles, ranging from 29 to 49 mBq m−3, were typical of oceanic baseline values. Diurnal cycles were rarely evident and local influences were minor, consistent with regional radon flux estimates one tenth of the global average for ice-free land. The predominant fetch region for terrestrially influenced air masses was South America (47–53° S), with minor influences also attributed to aged Australian air masses and local sources. Plume dilution factors of 2.8–4.0 were estimated for the most terrestrially influenced (South American) air masses, and a seasonal cycle in terrestrial influence on tropospheric air descending at the pole was identified and characterised.
Publisher: Stockholm University Press
Date: 2011
Publisher: Springer Science and Business Media LLC
Date: 15-02-2022
DOI: 10.1038/S43247-022-00347-3
Abstract: Speleothem oxygen isotopic (δ 18 O) records are used to reconstruct past hydroclimate yet records from the same cave do not always replicate. We use a global database of speleothem δ 18 O to quantify the replicability of records to show that disagreement is common worldwide, occurs across timescales and is unrelated to climate, depth or lithology. Our global analysis demonstrates that within-cave differences in mean speleothem δ 18 O values are consistent with those of dripwater, supporting a ubiquitous influence of flowpaths. We present a case study of four new stalagmite records from Golgotha Cave, southwest Australia, where the isotopic differences between them are informed by cave monitoring. It is demonstrated that karst hydrology is a major driver of within-cave speleothem and dripwater δ 18 O variability, primarily due to the influence of fractures on flowpaths. Applying our understanding of water movement through fractures assists in quantitative reconstruction of past climate variability from speleothem δ 18 O records.
Publisher: Informa UK Limited
Date: 02-08-2022
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 06-2021
Publisher: Copernicus GmbH
Date: 23-02-2017
DOI: 10.5194/ESSD-2017-14
Abstract: Abstract. The Measurements of Urban, Marine and Biogenic Air (MUMBA) c aign took place in Wollongong, New South Wales (a small coastal city approximately 80 km south of Sydney, Australia), from 21st December 2012 to 15th February 2013. Like many Australian cities, Wollongong is surrounded by dense eucalyptus forest and so the urban air-shed is heavily influenced by biogenic emissions. Instruments were deployed during MUMBA to measure the gaseous and aerosol composition of the atmosphere with the aim of providing a detailed characterisation of the complex environment of the ocean/forest/urban interface that could be used to test the skill of atmospheric models. Gases measured included ozone, oxides of nitrogen, carbon monoxide, carbon dioxide, methane and many of the most abundant volatile organic compounds. Aerosol characterisation included total particle counts above 3 nm, total cloud condensation nuclei counts mass concentration, number concentration size distribution, aerosol chemical analyses and elemental analysis. The c aign captured varied meteorological conditions, including two extreme heat events, providing a potentially valuable test for models of future air quality in a warmer climate. There was also an episode when the site s led clean marine air for many hours, providing a useful additional measure of background concentrations of these trace gases within this poorly s led region of the globe. In this paper we describe the c aign, the meteorology and the resulting observations of atmospheric composition in general terms, in order to equip the reader with sufficient understanding of the Wollongong regional influences to use the MUMBA datasets as a case study for testing a chemical transport model. The data is available from PANGAEA (see doi.pangaea.de/10.1594/PANGAEA.871982).
Publisher: IEEE
Date: 07-2018
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 06-2021
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 2022
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 2023
Publisher: American Meteorological Society
Date: 2011
Abstract: Radon (222Rn) is a powerful natural tracer of mixing and exchange processes in the atmospheric boundary layer. The authors present and discuss the main features of a unique dataset of 50 high-resolution vertical radon profiles up to 3500 m above ground level, obtained in clear and cloudy daytime terrestrial boundary layers over an inland rural site in Australia using an instrumented motorized research glider. It is demonstrated that boundary layer radon profiles frequently exhibit a complex layered structure as a result of mixing and exchange processes of varying strengths and extents working in clear and cloudy conditions within the context of the diurnal cycle and the synoptic meteorology. Normalized aircraft radon measurements are presented, revealing the characteristic structure and variability of three major classes of daytime boundary layer: 1) dry convective boundary layers, 2) mixed layers topped with residual layers, and 3) convective boundary layers topped with coupled nonprecipitating clouds. Robust and unambiguous signatures of important atmospheric processes in the boundary layer are identifiable in the radon profiles, including “top-down” mixing associated with entrainment in clear-sky cases and strongly enhanced venting and subcloud-layer mixing when substantial active cumulus are present. In poorly mixed conditions, radon gradients in the daytime atmospheric surface layer significantly exceed those predicted by Monin–Obukhov similarity theory. In two case studies, it is demonstrated for the first time that a sequence of vertical radon profiles measured over the course of a single day can consistently reproduce major structural features of the evolving boundary layer.
Publisher: Wiley
Date: 03-2020
DOI: 10.1002/ENG2.12133
Publisher: Copernicus GmbH
Date: 02-2013
Abstract: Abstract. Surface-based radon (222Rn) measurements can be combined with lidar backscatter to obtain a higher quality time series of mixing height within the planetary boundary layer (PBL) than is possible from lidar alone, and a more quantitative measure of mixing height than is possible from only radon. The reason why lidar measurements are improved is that there are times when lidar signals are ambiguous, and reliably attributing the mixing height to the correct aerosol layer presents a challenge. By combining lidar with a mixing length scale derived from a time series of radon concentration, automated and robust attribution is possible during the morning transition. Radon measurements provide mixing information during the night, but concentrations also depend on the strength of surface emissions. After processing radon in combination with lidar, we obtain nightly measurements of radon emissions and are able to normalise the mixing length scale for changing emissions. After calibration with lidar, the radon-derived equivalent mixing height agrees with other measures of mixing on daily and hourly timescales and is a potential method for studying intermittent mixing in nocturnal boundary layers.
Publisher: The Electromagnetics Academy
Date: 2014
Publisher: Elsevier BV
Date: 02-2017
Publisher: Copernicus GmbH
Date: 27-01-2017
Abstract: Abstract. The stable isotopic composition of water vapour provides information about moisture sources and processes difficult to obtain with traditional measurement techniques. Recently, it has been proposed that the D-excess of water vapour (dv = δ2H − 8 × δ18O) can provide a diagnostic tracer of continental moisture recycling. However, D-excess exhibits a diurnal cycle that has been observed across a variety of ecosystems and may be influenced by a range of processes beyond regional-scale moisture recycling, including local evaporation (ET) fluxes. There is a lack of measurements of D-excess in evaporation (ET) fluxes, which has made it difficult to assess how ET fluxes modify the D-excess in water vapour (dv). With this in mind, we employed a chamber-based approach to directly measure D-excess in ET (dET) fluxes. We show that ET fluxes imposed a negative forcing on the ambient vapour and could not explain the higher daytime dv values. The low dET observed here was sourced from a soil water pool that had undergone an extended drying period, leading to low D-excess in the soil moisture pool. A strong correlation between daytime dv and locally measured relative humidity was consistent with an oceanic moisture source, suggesting that remote hydrological processes were the major contributor to daytime dv variability. During the early evening, ET fluxes into a shallow nocturnal inversion layer caused a lowering of dv values near the surface. In addition, transient mixing of vapour with a higher D-excess from above the nocturnal inversion modified these values, causing large variability during the night. These results indicate d
Publisher: Copernicus GmbH
Date: 02-12-2019
DOI: 10.5194/ESSD-11-1883-2019
Abstract: Abstract. The Sydney Particle Study involved the comprehensive measurement of meteorology, particles and gases at a location in western Sydney during February–March 2011 and April–May 2012. The aim of this study was to increase scientific understanding of particle formation and transformations in the Sydney airshed. In this paper we describe the methods used to collect and analyse particle and gaseous s les, as well as the methods employed for the continuous measurement of particle concentrations, particle microphysical properties, and gaseous concentrations. This paper also provides a description of the data collected and is a metadata record for the data sets published in Keywood et al. (2016a, 0.4225/08/57903B83D6A5D) and Keywood et al. (2016b, 0.4225/08/5791B5528BD63).
Publisher: IEEE
Date: 12-2012
Publisher: MDPI AG
Date: 10-09-2019
Abstract: Volatile organic compounds (VOCs) are important precursors to the formation of ozone and fine particulate matter, the two pollutants of most concern in Sydney, Australia. Despite this importance, there are very few published measurements of ambient VOC concentrations in Australia. In this paper, we present mole fractions of several important VOCs measured during the c aign known as MUMBA (Measurements of Urban, Marine and Biogenic Air) in the Australian city of Wollongong (34°S). We particularly focus on measurements made during periods when clean marine air impacted the measurement site and on VOCs of biogenic origin. Typical unpolluted marine air mole fractions during austral summer 2012-2013 at latitude 34°S were established for CO2 (391.0 ± 0.6 ppm), CH4 (1760.1 ± 0.4 ppb), N2O (325.04 ± 0.08 ppb), CO (52.4 ± 1.7 ppb), O3 (20.5 ± 1.1 ppb), acetaldehyde (190 ± 40 ppt), acetone (260 ± 30 ppt), dimethyl sulphide (50 ± 10 ppt), benzene (20 ± 10 ppt), toluene (30 ± 20 ppt), C8H10 aromatics (23 ± 6 ppt) and C9H12 aromatics (36 ± 7 ppt). The MUMBA site was frequently influenced by VOCs of biogenic origin from a nearby strip of forested parkland to the east due to the dominant north-easterly afternoon sea breeze. VOCs from the more distant densely forested escarpment to the west also impacted the site, especially during two days of extreme heat and strong westerly winds. The relative amounts of different biogenic VOCs observed for these two biomes differed, with much larger increases of isoprene than of monoterpenes or methanol during the hot westerly winds from the escarpment than with cooler winds from the east. However, whether this was due to different vegetation types or was solely the result of the extreme temperatures is not entirely clear. We conclude that the clean marine air and biogenic signatures measured during the MUMBA c aign provide useful information about the typical abundance of several key VOCs and can be used to constrain chemical transport model simulations of the atmosphere in this poorly s led region of the world.
Publisher: Hindawi Limited
Date: 2014
DOI: 10.1155/2014/946781
Abstract: Simple multiband planar antenna for wireless communication applications is presented. The proposed antenna performs four resonant modes covering multibands of wireless standards, including LTE 700, GSM, DCS, PCS, UMTS, and LTE 2300/2500. Furthermore, it covers the ISM, WiMAX, and the WLAN bands. The geometry of the proposed antenna consists of a single FR4 substrate where an open cavity fed by a coplanar U-shaped monopole is etched on one side and a short-circuited meander line in the opposite side. The cavity by its nature supports a wide range of higher frequencies, while its boundary that consists of a thin monopole resonates at 900 MHz. The meander line in the opposite side supports the LTE 700 band. The operating bands ranges are (680–748 MHz), (870–960 MHZ), (1.36–1.59 GHz), and (1.71–2.56 GHz). The antenna size is 30 × 18 × 0.8 mm 3 . The antenna not only has a compact size but also supports a low SAR radiation at all the operating frequencies. The proposed antenna is tested using the four recommended test positions of the CTIA association where the proposed antenna reveals good performance in all test cases in the presence of handset (keypad, battery, speaker camera, RF circuit, and LCD) in talking position, and in standby position.
Publisher: Stockholm University Press
Date: 2013
Publisher: American Geophysical Union (AGU)
Date: 26-12-2017
DOI: 10.1002/2017JD026833
Publisher: Elsevier BV
Date: 03-2010
Publisher: Elsevier BV
Date: 02-2020
Publisher: Frontiers Media SA
Date: 08-11-2018
Location: Australia
Start Date: 12-2022
End Date: 12-2025
Amount: $409,193.00
Funder: Australian Research Council
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