ORCID Profile
0000-0002-2384-2249
Current Organisation
Baylor University
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Publisher: Springer Science and Business Media LLC
Date: 05-06-2020
DOI: 10.1038/S41467-020-16727-2
Abstract: Magnetoelectric coupling at room temperature in multiferroic materials, such as BiFeO 3 , is one of the leading candidates to develop low-power spintronics and emerging memory technologies. Although extensive research activity has been devoted recently to exploring the physical properties, especially focusing on ferroelectricity and antiferromagnetism in chemically modified BiFeO 3 , a concrete understanding of the magnetoelectric coupling is yet to be fulfilled. We have discovered that La substitutions at the Bi-site lead to a progressive increase in the degeneracy of the potential energy landscape of the BiFeO 3 system exemplified by a rotation of the polar axis away from the 〈111〉 pc towards the 〈112〉 pc discretion. This is accompanied by corresponding rotation of the antiferromagnetic axis as well, thus maintaining the right-handed vectorial relationship between ferroelectric polarization, antiferromagnetic vector and the Dzyaloshinskii-Moriya vector. As a consequence, La-BiFeO 3 films exhibit a magnetoelectric coupling that is distinctly different from the undoped BiFeO 3 films.
Publisher: American Association for the Advancement of Science (AAAS)
Date: 02-2019
Abstract: We present direct, real-time observations of emergent magnetic monopole dynamics in highly frustrated artificial spin ice.
Publisher: American Physical Society (APS)
Date: 30-12-2020
Publisher: Springer Science and Business Media LLC
Date: 12-12-2017
DOI: 10.1038/S41467-017-02139-2
Abstract: The original version of this article contained an error in the legend to Figure 4. The yellow scale bar should have been defined as ‘~600 nm’, not ‘~600 µm’. This has now been corrected in both the PDF and HTML versions of the article.
Publisher: American Physical Society (APS)
Date: 08-07-2021
Publisher: Springer Science and Business Media LLC
Date: 09-2016
DOI: 10.1038/NCOMMS12635
Abstract: Electric charge screening is a fundamental principle governing the behaviour in a variety of systems in nature. Through reconfiguration of the local environment, the Coulomb attraction between electric charges is decreased, leading, for ex le, to the creation of polaron states in solids or hydration shells around proteins in water. Here, we directly visualize the real-time creation and decay of screened magnetic charge configurations in a two-dimensional artificial spin ice system, the dipolar dice lattice. By comparing the temperature dependent occurrence of screened and unscreened emergent magnetic charge defects, we determine that screened magnetic charges are indeed a result of local energy reduction and appear as a transient minimum energy state before the system relaxes towards the predicted ground state. These results highlight the important role of emergent magnetic charges in artificial spin ice, giving rise to screened charge excitations and the emergence of exotic low-temperature configurations.
Publisher: Springer Science and Business Media LLC
Date: 21-09-2016
DOI: 10.1038/NATURE19343
Abstract: Materials that exhibit simultaneous order in their electric and magnetic ground states hold promise for use in next-generation memory devices in which electric fields control magnetism. Such materials are exceedingly rare, however, owing to competing requirements for displacive ferroelectricity and magnetism. Despite the recent identification of several new multiferroic materials and magnetoelectric coupling mechanisms, known single-phase multiferroics remain limited by antiferromagnetic or weak ferromagnetic alignments, by a lack of coupling between the order parameters, or by having properties that emerge only well below room temperature, precluding device applications. Here we present a methodology for constructing single-phase multiferroic materials in which ferroelectricity and strong magnetic ordering are coupled near room temperature. Starting with hexagonal LuFeO3-the geometric ferroelectric with the greatest known planar rumpling-we introduce in idual monolayers of FeO during growth to construct formula-unit-thick syntactic layers of ferrimagnetic LuFe2O4 (refs 17, 18) within the LuFeO3 matrix, that is, (LuFeO3)m/(LuFe2O4)1 superlattices. The severe rumpling imposed by the neighbouring LuFeO3 drives the ferrimagnetic LuFe2O4 into a simultaneously ferroelectric state, while also reducing the LuFe2O4 spin frustration. This increases the magnetic transition temperature substantially-from 240 kelvin for LuFe2O4 (ref. 18) to 281 kelvin for (LuFeO3)9/(LuFe2O4)1. Moreover, the ferroelectric order couples to the ferrimagnetism, enabling direct electric-field control of magnetism at 200 kelvin. Our results demonstrate a design methodology for creating higher-temperature magnetoelectric multiferroics by exploiting a combination of geometric frustration, lattice distortions and epitaxial engineering.
Publisher: AIP Publishing
Date: 26-02-2018
DOI: 10.1063/1.5014041
Abstract: The potential application of artificial spin ice in magnetic nanodevices provides a strong drive to investigate different lattice geometries. Here, we combine components of a recently investigated artificial spin ratchet with components of the prototypical square lattice to form a geometrically frustrated artificial spin ice system where Ising-type nanomagnets are arranged onto a two-dimensional square-kite lattice. Using synchrotron-based photoemission electron microscopy, we explore moment configurations achieved in this lattice geometry. Following thermal annealing, we image how a variation of the relevant lattice parameter affects magnetic ordering in four-island squares and four-island vertices during cooling through the Blocking temperature. Depending on lattice spacing, both nearly uniform and disordered spin configurations are accessible in our s les. We show that the relative energies of the building blocks of the system, which are typically used to classify lattice configurations, are not predictive of the low energy states adopted by the experimental system. To understand magnetic ordering in the square-kite lattice, longer range interactions must be considered.
Publisher: Springer Science and Business Media LLC
Date: 17-10-2017
DOI: 10.1038/S41467-017-01238-4
Abstract: Geometrical frustration occurs when entities in a system, subject to given lattice constraints, are hindered to simultaneously minimize their local interactions. In magnetism, systems incorporating geometrical frustration are fascinating, as their behavior is not only hard to predict, but also leads to the emergence of exotic states of matter. Here, we provide a first look into an artificial frustrated system, the dipolar trident lattice, where the balance of competing interactions between nearest-neighbor magnetic moments can be directly controlled, thus allowing versatile tuning of geometrical frustration and manipulation of ground state configurations. Our findings not only provide the basis for future studies on the low-temperature physics of the dipolar trident lattice, but also demonstrate how this frustration-by-design concept can deliver magnetically frustrated metamaterials.
Location: United States of America
No related grants have been discovered for Alan Farhan.