ORCID Profile
0000-0002-4624-054X
Current Organisation
University of Wollongong
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Publisher: Wiley
Date: 17-01-2022
Abstract: The exploration of facile, low‐cost, and universal synthetic strategies for high‐performance aqueous energy storage is extremely urgent. The electrochemical activation tactic is an emerging synthetic technique that can turn inert or weakly active substances into highly active materials for aqueous energy storage via in situ or ex situ electrochemical treatment, which is receiving increasing attention due to its advantages of facile operation, variable control, high efficiency, flexibility, and wide applicability. This review first discusses the definition and general implementing methods of the electrochemical activation tactic, as well as the fundamental activation mechanisms, and then summarizes its applications in various aqueous systems, including rechargeable batteries and electrochemical capacitors with different charge carriers. The remaining challenges, potential solutions, and further perspectives are discussed finally. It is believed that this review will provide a timely summary and new inspiration for cutting‐edge research on advanced aqueous energy storage devices.
Publisher: MDPI AG
Date: 21-07-2023
DOI: 10.3390/MOLECULES28145563
Abstract: The development of a stable and highly active photocatalyst has garnered significant attention in the field of wastewater treatment. In this study, a novel technique involving a facile stirring method was devised to fabricate an array of g-C3N4/ZnO nanowire (ZnO NW) composites. Through the introduction of g-C3N4 to augment the generation of electron-hole pairs upon exposure to light, the catalytic efficacy of these composites was found to surpass that of the pristine ZnO NWs when subjected to simulated sunlight. The photocatalytic performance of a 20 mg·L−1 methylene blue solution was found to be highest when the doping rate was 25 wt%, resulting in a degradation rate of 99.1% after 60 min. The remarkable enhancement in catalytic efficiency can be ascribed to the emergence of a captivating hetero-junction at the interface of g-C3N4 and ZnO NWs, characterized by a harmoniously aligned band structure. This alluring arrangement effectively curtailed charge carrier recombination, lified light absorption, and augmented the distinct surface area, culminating in a notable boost to the photocatalytic prowess. These findings suggest that the strategic engineering of g-C3N4/ZnO NW heterostructures holds tremendous promise as a pioneering avenue for enhancing the efficacy of wastewater treatment methodologies.
Publisher: Wiley
Date: 17-05-2023
Abstract: Sodium (Na) metal anodes are promising candidates for various batteries with high energy density and high‐power density, however, the dendrite growth of Na metal is impeding their practical applications. The binary alloy Na–K is in the liquid state at room temperature with a wide composition range, which renders it inherently free from solid dendrite growth. Whereas the application of Na–K alloy is plagued by the lack of a wettable matrix to immobilize the liquid metal. Herein, a facile method is reported to introduce oxygen‐rich functional groups into carbon fiber cloth (O‐CFC), which is initially Na–K phobic yet turns into superwetting after the treatment. The superwetting behavior of the O‐CFC can be attributed to the favorable enthalpy changes as a result of the introduction of O‐rich functional groups. The superwetting property of the O‐CFC exhibits good universality, which can be extended to melting Na and K metals. By adopting the superwetting O‐CFC as a host for liquid Na–K alloy, the liquid metal can be well retained in the matrix and deliver a stable cycling for h. The concept of enthalpy‐driven wettability regulation can be enlightening for the host material design of other liquid metals and alloys.
Publisher: MDPI AG
Date: 29-06-2021
Abstract: The hybrid ion capacitor (HIC) is a hybrid electrochemical energy storage device that combines the intercalation mechanism of a lithium-ion battery anode with the double-layer mechanism of the cathode. Thus, an HIC combines the high energy density of batteries and the high power density of supercapacitors, thus bridging the gap between batteries and supercapacitors. Two-dimensional (2D) carbon materials (graphite, graphene, carbon nanosheets) are promising candidates for hybrid capacitors owing to their unique physical and chemical properties, including their enormous specific surface areas, abundance of active sites (surface and functional groups), and large interlayer spacing. So far, there has been no review focusing on the 2D carbon-based materials for the emerging post-lithium hybrid capacitors. This concept review considers the role of 2D carbon in hybrid capacitors and the recent progress in the application of 2D carbon materials for post-Li (Na+, K+, Zn2+) hybrid capacitors. Moreover, their challenges and trends in their future development are discussed.
Publisher: Wiley
Date: 24-04-2021
Abstract: Structural engineering and creating atomic disorder in electrodes are promising strategies for highly efficient and rapid charge storage in advanced batteries. Herein, a nanohybrid architecture is presented with amorphous vanadium oxide conformally coated on layered V 2 C MXene ( a ‐VO x /V 2 C) via tunable anodic oxidation, which exhibits a high reversible capacity of 307 mAh g –1 at 50 mA g –1 , decent rate capability with capacity up to 96 mAh g –1 at 2000 mA g –1 , and good cycling stability as a cathode for sodium‐ion batteries. The a‐ VO x layer enables reversible and fast Na + insertion/extraction by providing sufficient vacancies and open pathways in the amorphous framework, unlike the irreversible phase transition in its crystalline counterpart, while layered V 2 C MXene offers abundant electron/ion transfer channels, which are joined together to boost the electrochemical performance. Notably the improved reversibility and structural superiority of the a ‐VO x /V 2 C nanohybrid are clearly revealed by in situ Raman, in situ transmission electron microscopy, in situ synchrotron X‐ray absorption spectroscopy, and density functional theory calculations, demonstrating a reversible V–O vibration and valence oscillation between V 4+ and V 5+ in the disordered framework, with robust structural stability and unobstructed Na + diffusion. This work provides a meaningful reference for the elaborate design of MXene‐based nanostructured electrodes toward advanced rechargeable batteries.
Publisher: American Chemical Society (ACS)
Date: 27-04-2017
Publisher: Royal Society of Chemistry (RSC)
Date: 2020
DOI: 10.1039/D0RA03490H
Publisher: Wiley
Date: 20-01-2022
Publisher: Royal Society of Chemistry (RSC)
Date: 2017
DOI: 10.1039/C7TA06194C
Publisher: American Chemical Society (ACS)
Date: 16-07-2020
Publisher: Wiley
Date: 10-10-2019
Publisher: American Chemical Society (ACS)
Date: 29-04-2021
Publisher: Wiley
Date: 28-08-2021
Publisher: Wiley
Date: 07-2020
Publisher: American Chemical Society (ACS)
Date: 05-07-2018
Publisher: American Chemical Society (ACS)
Date: 23-06-2023
Publisher: American Chemical Society (ACS)
Date: 17-06-2022
Abstract: Improving the electrochemical kinetics and the intrinsic poor conductivity of transition metal dichalcogenide (TMD) electrodes is meaningful for developing next-generation energy storage systems. As one of the most promising TMD anode materials, ReS
Publisher: American Chemical Society (ACS)
Date: 28-01-2022
DOI: 10.1021/ACS.NANOLETT.1C04492
Abstract: For practical sodium-ion batteries, both high electrochemical performance and cost efficiency of the electrode materials are considered as two key parameters. Prussian blue analogues (PBAs) are broadly recognized as promising cathode materials due to their low cost, high theoretical capacity, and cycling stability, although they suffer from low-crystallinity-induced performance deterioration. Herein, a facile "ice-assisted" strategy is presented to prepare highly crystallized PBAs without any additives. By suppressing structure defects, the cathode exhibits a high capacity of 123 mAh g
Publisher: American Chemical Society (ACS)
Date: 10-12-2018
Publisher: American Chemical Society (ACS)
Date: 09-06-2021
Publisher: American Chemical Society (ACS)
Date: 26-04-2018
Publisher: Elsevier BV
Date: 03-2021
Publisher: Wiley
Date: 04-12-2020
Publisher: World Scientific Pub Co Pte Ltd
Date: 10-06-2011
Publisher: American Chemical Society (ACS)
Date: 20-08-2021
Publisher: American Chemical Society (ACS)
Date: 24-07-2017
Publisher: Wiley
Date: 27-04-2023
Publisher: Royal Society of Chemistry (RSC)
Date: 2021
DOI: 10.1039/D0TA11496K
Abstract: Potassium-ion batteries (PIBs) have attracted great attention due to the abundance and low cost of potassium resources.
Publisher: American Chemical Society (ACS)
Date: 17-10-2022
Abstract: Increasing generation of permanent magnet waste has resulted in an urgent need to preserve finite resources. Reforming these wastes as feedstock to produce renewables is an ideal strategy for addressing waste and energy challenges. Herein, our work reports a smart and sustainable strategy to convert iron in magnet wastes into Prussian blue analogues that can serve as cathode materials for sodium-ion batteries. Moreover, a method to control feed rates is proposed to generate high-quality materials with fewer [Fe(CN)
Publisher: Royal Society of Chemistry (RSC)
Date: 2023
DOI: 10.1039/D3CC01548C
Abstract: This review summarizes the recent progress and presents the challenges and strategies of Fe-based and Mn-based Prussian blue analogues for metal-ion batteries.
Publisher: Elsevier BV
Date: 2020
Publisher: American Chemical Society (ACS)
Date: 28-04-2022
Abstract: Poly(ethylene oxide) (PEO)-based polymer electrolytes have been widely studied as a result of their flexibility, excellent interface contact, and high compatibility with a lithium metal anode. Owing to the poor oxidation resistance of ethers, however, the PEO-based electrolytes are only compatible with low-voltage cathodes, which limits their energy density. Here, a high-voltage stable solid-state interface layer based on polyfluoroalkyl acrylate was constructed via
Publisher: American Chemical Society (ACS)
Date: 24-04-2018
Publisher: Wiley
Date: 05-12-2022
DOI: 10.1002/CEY2.298
Abstract: The crystal plane plays a very important role in the properties of Ni‐rich cathodes. [003] crystallographic texture regulation has been proven to improve structural stability, and yet, the discrepancy of particles with different exposed ratios of [003] in structural attenuation has not been clarified. Herein, we have unraveled comprehensively the structural decay difference for Ni‐rich cathodes’ primary particles with the different percentages of exposed [003] by regulating the precursor coprecipitation process. The findings based on structural characterization, first‐principles calculations, finite element analysis, and electrochemical test reveal that the length and width of particles represent and [003] directions, respectively, and show that cathode particles with a higher /[003] ratio can effectively inhibit structure degradation and intergranular/intragranular crack formation owing to the low oxygen vacancy formation energy on (003) planes and the small local stress on secondary rimary particles. This study may provide guidance for the structural design of layered cathodes.
Publisher: Wiley
Date: 05-2023
Abstract: The development of large‐scale energy storage systems (ESSs) aimed at application in renewable electricity sources and in smart grids is expected to address energy shortage and environmental issues. Sodium‐ion batteries (SIBs) exhibit remarkable potential for large‐scale ESSs because of the high richness and accessibility of sodium reserves. Using low‐cost and abundant elements in cathodes with long cycling stability is preferable for lowering expenses on cathodes. Many investigated cathodes for SIBs are dogged by structural and morphology changes, unstable interphases between the cathode and the electrolyte, and air sensitivity, causing unsatisfactory cycling performance. Therefore, understanding the mechanism of capacity degeneration in depth and developing precise solutions are critical for designing low‐cost cathodes that are highly stable under cycling. Herein, recent progress in long‐cycle‐life and low‐cost cathodes for SIBs is focused on, and a comprehensive discussion of the key points in SIBs toward large‐scale applications is provided. The roots of the unstable cycling performance of low‐cost cathodes are discussed. Also, effective strategies are summarized from the recent progress on long‐cycle‐life and low‐cost cathodes. This review is expected to encourage deeper investigation of long‐lifespan cathodes for SIBs, particularly for potential large‐scale industrialization.
Publisher: Wiley
Date: 02-01-2023
Abstract: Sodium‐ion batteries (SIBs) with fast‐charge capability and long lifespan could be applied in various sustainable energy storage systems, from personal devices to grid storage. Inspired by the disordered Rubik's cube, here, we report that the high‐entropy (HE) concept can lead to a very substantial improvement in the sodium storage properties of hexacyanoferrate (HCF). An ex le of HE‐HCF has been synthesized as a proof of concept, which has achieved impressive cycling stability over 50 000 cycles and an outstanding fast‐charging capability up to 75 C. Remarkable air stability and all‐climate performance are observed. Its quasi‐zero‐strain reaction mechanism and high sodium diffusion coefficient have been measured and analyzed by multiple in situ techniques and density functional theory calculations. This strategy provides new insights into the development of advanced electrodes and provides the opportunity to tune electrochemical performance by tailoring the atomic composition.
Publisher: Wiley
Date: 05-01-2023
Publisher: Wiley
Date: 05-05-2021
Abstract: Most of the cathode materials for potassium ion batteries (PIBs) suffer from poor structural stability due to the large ionic radius of K + , resulting in poor cycling stability. Here we report a low‐strain potassium‐rich K 1.84 Ni[Fe(CN) 6 ] 0.88 ⋅0.49 H 2 O (KNiHCF) as a cathode material for PIBs. The as‐prepared KNiHCF cathode can deliver reversible discharge capacity of 62.8 mAh g −1 at 100 mA g −1 , with a high discharge voltage of 3.82 V. It can also achieve a superior rate performance of 45.8 mAh g −1 at 5000 mA g −1 , with a capacity retention of 88.6 % after 100 cycles. The superior performance of KNiHCF cathode results from low‐strain de‐/intercalation mechanism, intrinsic semiconductor property and low potassium diffusion energy barrier. The high power density and long‐term stability of KNiHCF//graphite full cell confirmed the feasibility of K‐rich KNiHCF cathode in PIBs. This work provides guidance to develop Prussian blue analogues as cathode materials for PIBs.
Publisher: American Chemical Society (ACS)
Date: 31-07-2019
Publisher: Wiley
Date: 05-11-2021
Abstract: Prussian blue analogs (PBAs), as promising cathode materials for sodium‐ion batteries (SIBs), have received extensive research interest due to their appealing characteristics, e.g., the low cost of their raw materials, easy manufacturing, open frameworks, and high theoretical specific capacity. There are some challenges for PBAs cathodes, however, hindering their performance output, making them currently unacceptable for practical applications. To improve the performance and cycling stability of PBAs, a clear in‐depth understanding of the relationship of their electrochemical reaction process to their ion insertion/extraction mechanisms and structural evolution is extremely important. Nowadays, advanced characterization techniques have become an important tool to guide the construction of high‐performance PBAs cathodes. In this review, the various advances by using advanced characterization techniques to reveal the reaction mechanisms for PBAs cathodes are summarized and discussed. By appreciating how the advanced characterization techniques to guide fabrication of high‐performance PBAs or reveal their detailed reaction mechanisms, it is hoped that this review can assist readers to find more valuable and advanced technologies to help to resolve some key problems and enhance their performance so as to accelerate the practical application of PBAs cathode for SIBs.
Publisher: Wiley
Date: 24-02-2022
Abstract: Prussian blue analogues (PBAs) have attracted wide attention for their application in the energy storage and conversion field due to their low cost, facile synthesis, and appreciable electrochemical performance. At the present stage, most research on PBAs is focused on their material‐level optimization, whereas their properties in practical battery systems are seldom considered. This review aims to first provide an overview of the history and parameters of PBA materials and analyze the fundamental principles toward rational design of PBAs, and then evaluate the prospects and challenges for PBAs for practical sodium‐ion batteries, hoping to bridge the gap between laboratory research and commercial reality.
Publisher: Elsevier BV
Date: 09-2020
Publisher: Wiley
Date: 23-06-2022
Abstract: With a series of merits, Prussian blue analogs (PBAs) have been considered as superior cathode materials for sodium‐ion batteries (SIBs). Their commercialization, however, still suffers from inferior stability, considerable [Fe(CN) 6 ] defects and interstitial water in the framework, which are related to the rapid crystal growth. Herein, a “water‐in‐salt” nanoreactor is proposed to synthesize highly crystallized PBAs with decreased defects and water, which show both superior specific capacity and rate capability in SIBs. The air‐stability, all‐climate, and full‐cell properties of our PBA have also been evaluated, and it exhibits enhanced electrochemical performance and higher volume yield than its counterpart synthesized via the water‐based co‐precipitation method. Furthermore, their highly reversible sodium‐ion storage behavior has been measured and identified via multiple in situ techniques. This work could pave the way for the PBA‐based SIBs in grid‐scale energy‐storage systems.
Publisher: Wiley
Date: 04-01-2018
Publisher: Elsevier BV
Date: 02-2017
Publisher: Wiley
Date: 09-06-2022
Abstract: Transition‐metal alloys are currently drawing increasing attention as promising electrocatalysts for the alkaline hydrogen evolution reaction (HER). However, traditional density‐functional‐theory‐derived d ‐band theory fails to describe the hydrogen adsorption energy (Δ G H ) on hollow sites. Herein, by studying the Δ G H for a series of Ni−M (M=Ti, V, Cr, Mn, Fe, Co, Cu, Zn, Mo, W) bimetallic alloys, an improved d ‐band center was provided and a potential NiCu electrocatalyst with a near‐optimal Δ G H was discovered. Moreover, oxygen atoms were introduced into Ni−M (O−NiM) to balance the adsorption/desorption of hydroxyl species. The tailored electrocatalytic sites for water dissociation can synergistically accelerate the multi‐step alkaline HER. The prepared O−NiCu shows the optimum HER activity with a low overpotential of 23 mV at 10 mA cm −2 . This work not only broadens the applicability of d ‐band theory, but also provides crucial understanding for designing efficient HER electrocatalysts.
Publisher: Wiley
Date: 13-10-2021
Abstract: To reach a closed‐loop material system and meet the urgent requirement of sustainable energy storage technologies, it is essential to incorporate efficient waste management into designing new energy storage materials. Here, a “two birds with one stone” strategy to transform rusty iron products into Prussian blue as high‐performance cathode materials, and recover the rusty iron products to their original status, is reported. Owing to the high crystalline and Na + content, the rusty iron derived Prussian blue shows a high specific capacity of 145 mAh g −1 and excellent cycling stability over 3500 cycles. Through the in situ X‐ray diffraction and in situ Raman spectra, it is found that the impressive ion storage capability and stability are strongly related to the suppressed structure distortion during the charge/discharge process. The ion migration mechanism and the possibility to serve as a universal host for other kinds of ions are further illuminated by density functional theory calculations. This work provides a new strategy for recycling wasted materials into high value‐added materials for sustainable battery systems, and is adaptable in the nanomedicine, catalysis, sensors, and gas storage applications.
Publisher: American Geophysical Union (AGU)
Date: 27-01-2004
DOI: 10.1029/2002TC001452
Publisher: Wiley
Date: 03-12-2018
Publisher: Elsevier BV
Date: 03-2019
Publisher: Elsevier BV
Date: 07-2019
Publisher: MDPI AG
Date: 02-12-2022
DOI: 10.3390/MOLECULES27238476
Abstract: Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C3N4)/ZnO photocatalysts were facilely synthesized through a grinding method using ZnO nanoparticles and g-C3N4 as the starting materials. According to the results, the photocatalytic performance of 10 wt.% CN-200/Z-500 (CN-200, which g-C3N4 was 200 kGy, referred to the irradiation metering. Z-500, which ZnO was 500 °C, referred to the calcination temperature) with the CN-200 exposed to electron beam radiation was better than those of either Z-500 or CN-200 alone. This material displayed a 98.9% degradation rate of MB (20 mg/L) in 120 min. The improvement of the photocatalytic performance of the 10 wt.% CN-200/Z-500 composite material was caused by the improvement of the separation efficiency of photoinduced electron–hole pairs, which was, in turn, due to the formation of heterojunctions between CN-200 and Z-500 interfaces. Thus, this study proposes the application of electron-beam irradiation technology for the modification of photocatalytic materials and the improvement of photocatalytic performance.
Publisher: Wiley
Date: 17-11-2021
Abstract: The safety of energy storage equipment has always been a stumbling block to the development of battery, and sodium ion battery is no exception. However, as an ultimate solution, the use of non‐flammable electrolyte is susceptible to the side effects, and its poor compatibility with electrode, causing failure of batteries. Here, we report a non‐flammable electrolyte design to achieve high‐performance sodium ion battery, which resolves the dilemma via regulating the solvation structure of electrolyte by hydrogen bonds and optimizing the electrode–electrolyte interphase. The reported non‐flammable electrolyte allows stable charge‐discharge cycling of both sodium vanadium phosphate@hard carbon and Prussian blue@hard carbon full pouch cell for more than 120 cycles with a capacity retention of % and high cycling Coulombic efficiency (99.7 %).
Publisher: Royal Society of Chemistry (RSC)
Date: 2019
DOI: 10.1039/C9TA04503A
Publisher: Wiley
Date: 15-01-2018
Publisher: Wiley
Date: 20-07-2022
Abstract: Sodium metal batteries are recognized as promising candidates for next‐generation energy storage devices, as a result of their high energy density, low redox potential, and cheap material price. Na metal anodes, however, generally exhibit notorious problems, including progressively thickened interfaces with active Na loss and Na metal dendrite growth with safety hazards. Herein, a lightweight aerogel consisting of MgF 2 nanocrystals grown on a reduced graphene oxide (RGO) aerogel matrix (MgF 2 @RGO) is rationally designed as a multifunctional host material for Na metal anodes. The MgF 2 nanocrystals can be electrochemically converted in situ into Mg and NaF nanograins during the first Na plating process, in which the Mg works as sodiophilic nucleation seeds for Na plating and NaF plays a key role in suppressing Na dendrite growth. Significantly, the Na metal anodes with the MgF 2 @RGO aerogel host deliver significantly enhanced Coulombic efficiency and dramatically improved cycling stability for more than 1600 h. The morphology evolution confirms the advantages of the Na metal anode with the MgF 2 @RGO host, which exhibits dense and flat interfaces. By pairing with the Na 3 V 2 (PO 4 ) 3 cathode, the Na metal batteries achieve stable cycling and good rate capability, suggesting the potential of the Na/MgF 2 @RGO anode for practical applications.
Publisher: Elsevier BV
Date: 08-2021
Publisher: Wiley
Date: 22-06-2022
Abstract: Prussian blue analogues (PBAs) have attracted extensive attention as cathode materials in sodium-ion batteries (SIBs) due to their low cost, high theoretical capacity, and facile synthesis process. However, it is of great challenge to control the crystal vacancies and interstitial water formed during the aqueous co-precipitation method, which are also the key factors in determining the electrochemical performance. Herein, an antioxidant and chelating agent co-assisted non-aqueous ball-milling method to generate highly-crystallized Na
Publisher: Royal Society of Chemistry (RSC)
Date: 2021
DOI: 10.1039/D1EE00087J
Abstract: The guest-ion disordered and quasi-zero-strain nonequilibrium solid–solution reaction mechanism provides an effective guarantee for realizing long-cycle life and high-rate capability electrode materials.
Publisher: Wiley
Date: 30-11-2020
Abstract: Hard carbon (HC) is recognized as a promising anode material with outstanding electrochemical performance for alkali metal‐ion batteries including lithium‐ion batteries (LIBs), as well as their analogs sodium‐ion batteries (SIBs) and potassium‐ion batteries (PIBs). Herein, a comprehensive review of the recent research is presented to interpret the challenges and opportunities for the applications of HC anodes. The ion storage mechanisms, materials design, and electrolyte optimizations for alkali metal‐ion batteries are illustrated in‐depth. HC is particularly promising as an anode material for SIBs. The solid‐electrolyte interphase, initial Coulombic efficiency, safety concerns, and all‐climate performances, which are vital for practical applications, are comprehensively discussed. Furthermore, commercial prototypes of SIBs based on HC anodes are extensively elaborated. The remaining challenges and research perspectives are provided, aiming to shed light on future research and early commercialization of HC‐based SIBs.
Publisher: Wiley
Date: 24-05-2023
Abstract: Prussian blue analogues (PBAs) have been regarded as promising cathode materials for alkali‐ion batteries owing to their high theoretical energy density and low cost. However, the high water and vacancy content of PBAs lower their energy density and bring safety issues, impeding their large‐scale application. Herein, a facile “potassium‐ions assisted” strategy is proposed to synthesize highly crystallized PBAs. By manipulating the dominant crystal plane and suppressing vacancies, the as‐prepared PBAs exhibit increased redox potential resulting in high energy density up to ≈450 Wh kg −1 , which is at the same level of the well‐known LiFePO 4 cathodes for lithium‐ion batteries. Remarkably, unconventional highly‐reversible phase evolution and redox‐active pairs were identified by multiple in situ techniques for the first time. The preferred guest‐ion storage sites and migration mechanism were systematically analysed through theoretical calculations. We believe these results could inspire the design of safe with high energy density.
Publisher: American Chemical Society (ACS)
Date: 19-10-2021
DOI: 10.1021/JACS.1C06727
No related grants have been discovered for Jian Peng.