ORCID Profile
0000-0001-9023-5134
Current Organisation
Xi'an University of Science and Technology
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Publisher: Elsevier BV
Date: 02-2011
DOI: 10.1016/J.BIORTECH.2010.10.120
Abstract: The thermal decomposition behavior of ramie residue (RR) and the characteristics of fuel gas produced in a cyclone furnace were studied. The pyrolysis kinetics was investigated using thermogravimetric analysis (TGA) at heating rates of 5-20°C/min. The results showed that RR mainly decomposed between 250 and 390°C, and the apparent activation energy ranged from 200 to 258 kJ/mol. In the cyclone furnace, fast pyrolysis, partial combustion and gasification occurred almost simultaneously, and the thermal energy was supplied by partial combustion of RR powder at the hypo stoichiometric amount of air. Higher effect of equivalence ratio (ER) led to higher reaction temperature and fewer contents of tar and char, but too high ER lowered fuel gas content and degraded fuel gas quality. Over the ranges of the experimental conditions, the gas yield varied between 1.07 and 2.08 N m(3)/kg and the LHV was between 3350 and 4798 kJ/Nm(3).
Publisher: Elsevier BV
Date: 09-2019
Publisher: Walter de Gruyter GmbH
Date: 15-08-2023
Abstract: Coal and biomass are important feedstocks for carbon energy from thermochemical conversion process. Fully understanding the analytical technology that characterizes the changes in physicochemical properties and structural characteristics of coal and biomass during the thermochemical reactions is a key prerequisite for the realization of appropriate utilization of energy fuels. Modern in-situ process analysis technology can accomplish the in-situ detection of the experimental process, and therefore reflect the experimental process more accurately. Moreover, it is developing towards automation, intelligentization, and comprehensive detection. Based on the characteristics of each detection technology, this paper summarizes the basic principles, application scope and performance characteristics of the three advanced in-situ process analysis technologies: hyphenated technology, synchrotron radiation, and online analysis. The practicability and accuracy of each detection technology in coal and biomass research are compared and analyzed, and its latest application and development trend are elucidated. These tools not only make up for the shortcomings of traditional detection techniques in characterizing the in-situ reaction, but also provide complementary information on molecular microscopic changes during fuel thermal conversion. This review paper can provide insights for relevant researchers in the selection of analytical techniques, and promote in-depth study on microcosmic mechanism of fuel conversion.
Publisher: Elsevier BV
Date: 12-2018
Publisher: American Chemical Society (ACS)
Date: 27-06-2019
Publisher: Elsevier BV
Date: 08-2022
Publisher: Elsevier BV
Date: 09-2017
Publisher: Elsevier BV
Date: 10-2010
Publisher: MDPI AG
Date: 21-01-2022
Abstract: The potential of catalytic pyrolysis of biomass for hydrogen and bio-oil production has drawn great attention due to the concern of clean energy utilization and decarbonization. In this paper, the catalytic pyrolysis of pine sawdust with calcined dolomite was carried out in a novel moving bed reactor with a two-stage screw feeder. The effects of pyrolysis temperature (700–900 °C) and catalytic temperature (500–800 °C) on pyrolysis performance were investigated in product distribution, gas composition, and gas properties. The results showed that with the temperature increased, pyrolysis gas yield increased, but the yield of solid and liquid products decreased. With the increase in temperature, the CO and H2 content increased significantly, while the CO2 and CH4 decreased correspondingly. The calcined dolomite can remove the tar by 44% and increased syngas yield by 52.9%. With the increasing catalytic temperature, the catalytic effect of calcined dolomite was also enhanced.
Publisher: Elsevier BV
Date: 11-2016
Publisher: Elsevier BV
Date: 08-2019
Publisher: MDPI AG
Date: 24-02-2022
Abstract: Hydrogen production from biomass pyrolysis is economically and technologically attractive from the perspectives of energy and the environment. The two-stage catalytic pyrolysis of pine sawdust for hydrogen-rich gas production is investigated using nano-NiO/Al2O3 as the catalyst at high temperatures. The influences of residence time (0–30 s) and catalytic temperature (500–800 °C) on pyrolysis performance are examined in the distribution of pyrolysis products, gas composition, and gas properties. The results show that increasing the residence time decreased the solid and liquid products but increased gas products. Longer residence times could promote tar cracking and gas-phase conversion reactions and improve the syngas yield, H2/CO ratio, and carbon conversion. The nano-NiO/A12O3 exhibits excellent catalytic activity for tar removal, with a tar conversion rate of 93% at 800 °C. The high catalytic temperature could significantly improve H2 and CO yields by enhancing the decomposition of tar and gas-phase reactions between CO2 and CH4. The increasing catalytic temperature increases the dry gas yield and carbon conversion but decreases the H2/CO ratio and low heating value.
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