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Cooperativity in Spin Crossover Systems: Memory, Magnetism and Microporosity. Spin-crossover centres are a well known form of inorganic electronic switch for which variation of temperature, pressure and irradiation leads to a change in d-electron configuration and therefore changes to structure, colour and magnetism. Here we aim to synthesise and study a wide variety of new spin-crossover systems where cooperativitiy between centres, induced by careful supramolecular design, will lead to molecul ....Cooperativity in Spin Crossover Systems: Memory, Magnetism and Microporosity. Spin-crossover centres are a well known form of inorganic electronic switch for which variation of temperature, pressure and irradiation leads to a change in d-electron configuration and therefore changes to structure, colour and magnetism. Here we aim to synthesise and study a wide variety of new spin-crossover systems where cooperativitiy between centres, induced by careful supramolecular design, will lead to molecules and materials having memory retention, magnetic ordering and/or microporosity. The significance of these aims covers several fundamental questions in the science of electronic systems. We also identify a number of potential nanochemical switching applications for the unique systems proposed.Read moreRead less
Polynuclear Spin-Crossover Molecular Switches: Host-Guest Chemistry, Magnetism and Memory. The generation of advanced nanomaterials requires both a control of nanoscale structure and the incorporation of specific properties into that structure. This project will lead to significant new developments in this area, with the assembly of complex molecular systems containing electronic switches. The unique combination of nanoscale switching and guest-binding and/or magnetic ordering in these systems ....Polynuclear Spin-Crossover Molecular Switches: Host-Guest Chemistry, Magnetism and Memory. The generation of advanced nanomaterials requires both a control of nanoscale structure and the incorporation of specific properties into that structure. This project will lead to significant new developments in this area, with the assembly of complex molecular systems containing electronic switches. The unique combination of nanoscale switching and guest-binding and/or magnetic ordering in these systems will lead to entirely new materials properties, leading in turn to fundamental advances in the science of molecular electronics and nanomaterials. Benefits of the research are wide-ranging, and include the development of innovative new technologies for molecular sensing, molecular separations, data storage and visual displays.Read moreRead less
Cooperativity in Spin-Crossover Systems: Memory, Magnetism and Microporosity. Spin-crossover centres are a well known form of inorganic electronic switch for which variation of temperature, pressure and irradiation leads to a change in d-electron configuration and therefore changes to structure, colour and magnetism. Here we aim to synthesise and study a wide variety of new spin-crossover systems where cooperativity between centres, induced by careful supramolecular design, will lead to molecule ....Cooperativity in Spin-Crossover Systems: Memory, Magnetism and Microporosity. Spin-crossover centres are a well known form of inorganic electronic switch for which variation of temperature, pressure and irradiation leads to a change in d-electron configuration and therefore changes to structure, colour and magnetism. Here we aim to synthesise and study a wide variety of new spin-crossover systems where cooperativity between centres, induced by careful supramolecular design, will lead to molecules and materials having memory retention, magnetic ordering and/or microporosity. The significance of these aims covers several fundamental questions in the science of electronic systems. We also identify a number of potential nanochemical switching applications for the unique systems proposed.Read moreRead less
Spin Switching in Nanoporous, Nanomolecular and Multifunctional Hybrid Systems. The generation of molecular nanomaterials with advanced chemical and physical properties requires both the control of nanoscale structure and the incorporation of specific function into that structure. This project will lead to significant new advances in this area through the generation of molecules and materials in which nanoscale switching is combined with guest-binding, magnetic ordering, and multiple other prope ....Spin Switching in Nanoporous, Nanomolecular and Multifunctional Hybrid Systems. The generation of molecular nanomaterials with advanced chemical and physical properties requires both the control of nanoscale structure and the incorporation of specific function into that structure. This project will lead to significant new advances in this area through the generation of molecules and materials in which nanoscale switching is combined with guest-binding, magnetic ordering, and multiple other properties. Entirely new materials functionalities will emerge, leading in turn to fundamental advances in the science of molecular electronics and nanomaterials and to the development of innovative new technologies for molecular sensing, molecular separations and data storage.Read moreRead less
Polynuclear Spin-Crossover Molecular Switches: Host-Guest Chemistry, Magnetism and Memory. The generation of advanced nanomaterials requires both a control of nanoscale structure and the incorporation of specific properties into that structure. This project will lead to significant new developments in this area, with the assembly of complex molecular systems containing electronic switches. The unique combination of nanoscale switching and guest-binding and/or magnetic ordering in these system ....Polynuclear Spin-Crossover Molecular Switches: Host-Guest Chemistry, Magnetism and Memory. The generation of advanced nanomaterials requires both a control of nanoscale structure and the incorporation of specific properties into that structure. This project will lead to significant new developments in this area, with the assembly of complex molecular systems containing electronic switches. The unique combination of nanoscale switching and guest-binding and/or magnetic ordering in these systems will lead to entirely new materials properties, leading in turn to fundamental advances in the science of molecular electronics and nanomaterials. Benefits of the research are wide-ranging, and include the development of innovative new technologies for molecular sensing, molecular separations, data storage and visual displays.Read moreRead less
An Innovative Solid-State Approach to Enhanced Solar-Hydrogen Production. The project will make a major step towards the development of solar-hydrogen technology, which promises to deliver a clean and renewable fuel - hydrogen - from water (seawater or other) using sunlight and a suitable photo-catalytic material. Not only will solar-hydrogen assist Australia to reduce its dependence on imported energy, but will also reduce Australia's carbon emissions and overall contribution to climate change. ....An Innovative Solid-State Approach to Enhanced Solar-Hydrogen Production. The project will make a major step towards the development of solar-hydrogen technology, which promises to deliver a clean and renewable fuel - hydrogen - from water (seawater or other) using sunlight and a suitable photo-catalytic material. Not only will solar-hydrogen assist Australia to reduce its dependence on imported energy, but will also reduce Australia's carbon emissions and overall contribution to climate change. When commercialized, solar-hydrogen technology may also enable Australia to become a global leader in the export of clean fuel, which will have very positive, far-reaching consequences for the economy.Read moreRead less
Platinum-group Metal Oxides with Modulated Crystal Structures: Flexible Frameworks Designed for Geometrically Frustrated Magnetism. Magnetic materials are of huge importance to modern society because of the key roles they play in devices such as hard disks, sensors, switches and permanent magnets. This project will focus on the chemical design and synthesis of novel, flexible and unconventional magnetic materials. Their study will lead to improved theories of magnetism and superconductivity, and ....Platinum-group Metal Oxides with Modulated Crystal Structures: Flexible Frameworks Designed for Geometrically Frustrated Magnetism. Magnetic materials are of huge importance to modern society because of the key roles they play in devices such as hard disks, sensors, switches and permanent magnets. This project will focus on the chemical design and synthesis of novel, flexible and unconventional magnetic materials. Their study will lead to improved theories of magnetism and superconductivity, and ultimately to technologies such as new data-storage media. The project will also help introduce Australian scientists to their new research reactor and synchrotron, which will play critical roles by allowing exceptionally thorough and systematic studies to be carried out.Read moreRead less
Porous and Magnetic Networks: Functional materials by form and design. The importance of obtaining smart materials to meet the increasingly stringent demands of modern technology and society, necessitates a determined effort by the research community. Three examples of such demands are the drive towards a hydrogen-based economy, sequestration technologies and green catalysis. Specifically designed meso- or highly porous materials have a central role to play in these extremely topical societal ....Porous and Magnetic Networks: Functional materials by form and design. The importance of obtaining smart materials to meet the increasingly stringent demands of modern technology and society, necessitates a determined effort by the research community. Three examples of such demands are the drive towards a hydrogen-based economy, sequestration technologies and green catalysis. Specifically designed meso- or highly porous materials have a central role to play in these extremely topical societal demands. The inclusion of functionality by design into such materials is central to them fulfilling their considerable potential. By researching novel materials technologies today, we aim to deliver practical solutions to market tomorrow, to the benefit of Australian industry.Read moreRead less
Linkage Infrastructure, Equipment And Facilities - Grant ID: LE0668302
Funder
Australian Research Council
Funding Amount
$210,000.00
Summary
Floating-zone Crystal Growth Facility. Optical floating-zone furnaces are powerful and efficient tools for the discovery and characterisation of new materials. They are widely used in the solid-state chemistry, condensed-matter physics, materials science, and engineering communities. This optical floating-zone furnace, the first in Australia, will support and encourage the growing number of local researchers in these fields. It will allow them to take much better advantage of the new research re ....Floating-zone Crystal Growth Facility. Optical floating-zone furnaces are powerful and efficient tools for the discovery and characterisation of new materials. They are widely used in the solid-state chemistry, condensed-matter physics, materials science, and engineering communities. This optical floating-zone furnace, the first in Australia, will support and encourage the growing number of local researchers in these fields. It will allow them to take much better advantage of the new research reactor and synchrotron being constructed in Australia by maximising their ability to grow crystals of technologically and scientifically important materials, particularly electronic and magnetic materials, for fundamental and applied research at those facilities.Read moreRead less
Linkage Infrastructure, Equipment And Facilities - Grant ID: LE0775771
Funder
Australian Research Council
Funding Amount
$280,000.00
Summary
Physical Property Measurement System for Materials Characterisation. The Physical Property Measurement System (PPMS) is a versatile, state-of-the-art instrument that is capable of measuring a broad range of magnetic, electronic and thermodynamic materials properties. The instrument will greatly extend materials characterisation capabilities in the Sydney region, leading to major advances in fundamental and applied research and to essential postgraduate training in chemistry, physics and enginee ....Physical Property Measurement System for Materials Characterisation. The Physical Property Measurement System (PPMS) is a versatile, state-of-the-art instrument that is capable of measuring a broad range of magnetic, electronic and thermodynamic materials properties. The instrument will greatly extend materials characterisation capabilities in the Sydney region, leading to major advances in fundamental and applied research and to essential postgraduate training in chemistry, physics and engineering. The importance of materials discovery and characterisation is vital to the development of new technologies over the next decade, as recognised in the national priority area 'Frontier Technologies for Building and Transforming Australian Industries'. Read moreRead less