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Using natural products to inspire discoveries in synthesis and biosynthesis. This project aims to understand the organic chemistry that occurs in the biosynthesis of unusual antibiotic natural products by marine microorganisms. In an interdisciplinary approach, proposed biosynthetic intermediates will be synthesised and screened against newly isolated enzymes from the microorganisms of interest. This will allow the elucidation of biosynthetic pathways, and aid the discovery of new chemoenzymatic ....Using natural products to inspire discoveries in synthesis and biosynthesis. This project aims to understand the organic chemistry that occurs in the biosynthesis of unusual antibiotic natural products by marine microorganisms. In an interdisciplinary approach, proposed biosynthetic intermediates will be synthesised and screened against newly isolated enzymes from the microorganisms of interest. This will allow the elucidation of biosynthetic pathways, and aid the discovery of new chemoenzymatic reactivity that may be broadly useful in organic synthesis. Non-enzymatic, predisposed organic reactions will also be uncovered during the project. The benefit of this project will be an improvement in our ability to synthesise potential antibiotics using a combined synthetic organic and chemoenzymatic approach. This could lead to useful new antibiotics in the future.Read moreRead less
Internally decorated discrete Metallo-supramolecular Assemblies and infinite Metal-Organic Frameworks as molecular containers. In the macroscopic world, containers are used to hold, provide physical protection, or create a modified environment for their contents. This project will result in the synthesis of novel molecular container materials that provide decorated internal surfaces capable of selectively binding chemical species. In addition to the breakthrough scientific benefits of establish ....Internally decorated discrete Metallo-supramolecular Assemblies and infinite Metal-Organic Frameworks as molecular containers. In the macroscopic world, containers are used to hold, provide physical protection, or create a modified environment for their contents. This project will result in the synthesis of novel molecular container materials that provide decorated internal surfaces capable of selectively binding chemical species. In addition to the breakthrough scientific benefits of establishing the fundamentals of these systems, the binding of chemicals, which are environmental contaminants, will provide the grounding for applications that will contribute to the national priority of 'Frontier technologies'. Furthermore, this research will lead to the training of the next generation of Australian scientists by quality international researchers.Read moreRead less
Solar-Driven C-H Functionalization Reactions. This project aims to investigate the functionalization reaction of unreactive C-H bonds using light as the source of energy. Light is a transformative change to synthesis as thermal activation is exchanged to solar activation. The latter gives access to excited state chemistry and enables reaction steps that are thermally inaccessible. It is a key strategy to leverage synthesis to the demands of the 21st century and to minimise its ecologic footprint ....Solar-Driven C-H Functionalization Reactions. This project aims to investigate the functionalization reaction of unreactive C-H bonds using light as the source of energy. Light is a transformative change to synthesis as thermal activation is exchanged to solar activation. The latter gives access to excited state chemistry and enables reaction steps that are thermally inaccessible. It is a key strategy to leverage synthesis to the demands of the 21st century and to minimise its ecologic footprint. At the same time this strategy provides a lever to profoundly impact and drive new concepts in synthesis. Significant benefits are expected, such as increase in fundamental knowledge on photochemical processes, but also the access to new materials for applications as drugs or OLEDs.Read moreRead less
Sulfur-based materials for infrared optics and thermal imaging. This project aims to investigate novel sulfur polymers for use in infrared optics and thermal imaging. Current thermal imaging lenses are made in energy-intensive processes from expensive semiconductors and toxic chalcogenide glasses. In contrast, highly abundant elemental sulfur can be converted into polymers that are highly transparent to mid- and long-wave infrared light, providing a promising low-cost alternative. In developing ....Sulfur-based materials for infrared optics and thermal imaging. This project aims to investigate novel sulfur polymers for use in infrared optics and thermal imaging. Current thermal imaging lenses are made in energy-intensive processes from expensive semiconductors and toxic chalcogenide glasses. In contrast, highly abundant elemental sulfur can be converted into polymers that are highly transparent to mid- and long-wave infrared light, providing a promising low-cost alternative. In developing this technology, expected outcomes include novel methods to manufacture polymers from low-cost sulfur and their use as lenses for thermal imaging. Significant benefits are expected, such as access to low-cost, recyclable materials for thermal imaging required in surveillance, diagnostics, and spectroscopy.Read moreRead less
Light driven degradation of persistent organic pollutants. This project aims to address the accumulation of pollutants in our environment by developing and optimising materials that utilise light energy to breakdown these persistent chemicals. Combining novel techniques and approaches, this project expects to generate new knowledge in the field of materials science and photochemistry. The anticipated outcomes of this project include an advancement of environmental remediation methods and the cap ....Light driven degradation of persistent organic pollutants. This project aims to address the accumulation of pollutants in our environment by developing and optimising materials that utilise light energy to breakdown these persistent chemicals. Combining novel techniques and approaches, this project expects to generate new knowledge in the field of materials science and photochemistry. The anticipated outcomes of this project include an advancement of environmental remediation methods and the capture of pollutants at their source. This should provide significant benefits to both humans and the environment through preventing the adverse impacts of pollutant exposure.Read moreRead less
Improving anti-salt crystallisation for solar-steam desalination. This project aims to solve a critical issue of solar-steam desalination by fundamental research. The solar-steam desalination technology offers an ideal strategy to utilize solar light as the energy source for desalination and water purification to produce affordable clean water. Photothermal materials play a key role in the desalination system to convert sunlight to heat and subsequently evaporate the saline water to generate ste ....Improving anti-salt crystallisation for solar-steam desalination. This project aims to solve a critical issue of solar-steam desalination by fundamental research. The solar-steam desalination technology offers an ideal strategy to utilize solar light as the energy source for desalination and water purification to produce affordable clean water. Photothermal materials play a key role in the desalination system to convert sunlight to heat and subsequently evaporate the saline water to generate steam as clean water. However, salt crystallization on the photothermal material surfaces severely limits the performance of the materials and clean water production. Solving this problem could accelerate the commercialisation and application of this technology, which will benefit millions of people worldwide.Read moreRead less
Defining and controlling seawater intrusion in threatened coastal aquifers. This project aims to improve knowledge of coastal aquifer processes and management practices in order to increase the security of highly vulnerable freshwater. In particular, it aims to address critical barriers to the regional-scale investigation of coastal aquifers, including island lenses – the most vulnerable freshwater resources on earth. Threats to coastal aquifers are intensifying globally, and key knowledge gaps ....Defining and controlling seawater intrusion in threatened coastal aquifers. This project aims to improve knowledge of coastal aquifer processes and management practices in order to increase the security of highly vulnerable freshwater. In particular, it aims to address critical barriers to the regional-scale investigation of coastal aquifers, including island lenses – the most vulnerable freshwater resources on earth. Threats to coastal aquifers are intensifying globally, and key knowledge gaps prevail in our current understanding and representation of transient, regional-scale seawater intrusion. The project plans to use coastal aquifer case studies from Australia and overseas to evaluate seawater intrusion reversibility, intermittent pumping effects, offshore aquifer processes, and management approaches. The project may improve coastal aquifer practices globally by unravelling the driving forces of transient seawater intrusion and developing new seawater intrusion models.Read moreRead less
Novel CO2-stable oxygen transporting membranes for oxyfuel-based CO2 capture and utilization. Industrial carbon dioxide (CO2) emission is considered the main contribution to global warming. This project aims to develop a new class of oxygen transporting membrane (OTM) for CO2 capture and utilisation. To achieve this objective, the formation process and the unique characteristic of the membrane, as well as the oxygen transportation mechanism through the membrane will be investigated, experimental ....Novel CO2-stable oxygen transporting membranes for oxyfuel-based CO2 capture and utilization. Industrial carbon dioxide (CO2) emission is considered the main contribution to global warming. This project aims to develop a new class of oxygen transporting membrane (OTM) for CO2 capture and utilisation. To achieve this objective, the formation process and the unique characteristic of the membrane, as well as the oxygen transportation mechanism through the membrane will be investigated, experimentally and theoretically. This will advance the membrane technology in economically viable and efficient, clean energy applications.Read moreRead less
Engineered redox polymers for catalytic water purification. This project aims to develop a novel family of chemically and structurally controlled redox polymer as metal-free catalysts for wastewater micropollutant treatment. Innovations lie in the synthesis of high-performance and nanostructured carbon-based materials, multiscale modeling, and in situ characterizations for understanding structure-property relationship in carbon catalysis. Expected outcomes will deliver innovations in functional ....Engineered redox polymers for catalytic water purification. This project aims to develop a novel family of chemically and structurally controlled redox polymer as metal-free catalysts for wastewater micropollutant treatment. Innovations lie in the synthesis of high-performance and nanostructured carbon-based materials, multiscale modeling, and in situ characterizations for understanding structure-property relationship in carbon catalysis. Expected outcomes will deliver innovations in functional materials, mechanism, catalytic engineering, and sustainable separation processes. This project will provide significant benefits in renovating smart nanomaterials in advanced manufacturing and clean environmental technologies, promoting Australia’s economic development and environment protection.Read moreRead less
Deciphering Electron Transfer Pathways in Bacteria. Enzyme catalysed oxidation reactions are key players in the production of naturally occurring biologically active molecules. These processes are tightly regulated by their electron transfer partners. This project aims to characterise new electron transfer ferredoxin proteins from a metabolically diverse bacterium. These ferredoxins, important in many bacteria, contain different non-cysteine amino acids in their iron-sulfur cluster binding motif ....Deciphering Electron Transfer Pathways in Bacteria. Enzyme catalysed oxidation reactions are key players in the production of naturally occurring biologically active molecules. These processes are tightly regulated by their electron transfer partners. This project aims to characterise new electron transfer ferredoxin proteins from a metabolically diverse bacterium. These ferredoxins, important in many bacteria, contain different non-cysteine amino acids in their iron-sulfur cluster binding motifs and are poorly defined. The outcomes will advance understandings of electron transfer, a fundamental process. This will allow strategies to combat human and plant pathogens and unlock the potential of these systems as biocatalysts for the green chemical synthesis of complex and valuable chemicals.Read moreRead less