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Reactions of Coordinated Dinitrogen. The program will develop novel metal-based catalysts and reagents that will transform nitrogen gas into ammonia and other nitrogen-containing compounds (nitrogen fixation). This fundamental chemical transformation underpins major chemical industries and this new approach using organometallic catalysts will significantly improve the efficiency of ammonia production and reduce the energy and harsh reaction conditions currently required. This program will desi ....Reactions of Coordinated Dinitrogen. The program will develop novel metal-based catalysts and reagents that will transform nitrogen gas into ammonia and other nitrogen-containing compounds (nitrogen fixation). This fundamental chemical transformation underpins major chemical industries and this new approach using organometallic catalysts will significantly improve the efficiency of ammonia production and reduce the energy and harsh reaction conditions currently required. This program will design catalysts with multiple complementary metal centres tailored to bind and activate nitrogen gas to facilitate its reaction with hydrogen or other reagents.Read moreRead less
Cyclophane Carbene Complexes as Catalysts: An Integrated Synthetic, Structural, and Mechanistic Approach. Metal-carbene complexes are emerging as efficient catalysts for chemical processes of immense importance to the pharmaceutical and fine chemicals industries. This project will build on the recent discovery of a family of complexes that exhibits the highest activity yet reported for metal-carbene catalysts in carbon-carbon bond-forming reactions. Insights into the ways the new catalysts work ....Cyclophane Carbene Complexes as Catalysts: An Integrated Synthetic, Structural, and Mechanistic Approach. Metal-carbene complexes are emerging as efficient catalysts for chemical processes of immense importance to the pharmaceutical and fine chemicals industries. This project will build on the recent discovery of a family of complexes that exhibits the highest activity yet reported for metal-carbene catalysts in carbon-carbon bond-forming reactions. Insights into the ways the new catalysts work will be gained through a combination of synthetic, mechanistic, and structural studies. This detailed investigation of structure/reactivity relationships will provide an understanding of why these catalyst are so efficient and hence give synthetic leads for the development of superior new catalysts suitable for industrial application.Read moreRead less
Arsenic speciation in Cleveland Bay, and controls on its uptake in commercial crab species. Marine organisms from the Great Barrier Reef exhibit elevated arsenic concentrations. It is not known if arsenic constitutes a human health risk since its chemical form has not been determined. The factors which control arsenic uptake in the GBR environment are unknown, making it difficult to predict how changes in water quality (such as phosphate which is chemically similar to arsenic) may alter arsenic ....Arsenic speciation in Cleveland Bay, and controls on its uptake in commercial crab species. Marine organisms from the Great Barrier Reef exhibit elevated arsenic concentrations. It is not known if arsenic constitutes a human health risk since its chemical form has not been determined. The factors which control arsenic uptake in the GBR environment are unknown, making it difficult to predict how changes in water quality (such as phosphate which is chemically similar to arsenic) may alter arsenic concentrations in these organisms. This project will determine the chemical form of arsenic in biota, sediment and water, and will test the hypothesis that the elevated arsenic levels reflect the low phosphate concentrations in the water.Read moreRead less
Studies of metal compounds containing carbon chains - approaches to novel materials. There is an increasing need to design functional devices on the molecular scale ("nanotechnology"). We are developing the chemistry of compounds which contain chains of up to 12 carbon atoms to allow electronic communication between metal centres attached to each end. This projects seeks to extend this work, to discover new and more effective compounds, and to develop the associated chemistry to provide synthese ....Studies of metal compounds containing carbon chains - approaches to novel materials. There is an increasing need to design functional devices on the molecular scale ("nanotechnology"). We are developing the chemistry of compounds which contain chains of up to 12 carbon atoms to allow electronic communication between metal centres attached to each end. This projects seeks to extend this work, to discover new and more effective compounds, and to develop the associated chemistry to provide syntheses of novel compounds of potential use in the fine chemicals industry. Extensive collaboration with French colleagues exists and will continue.Read moreRead less
All-carbon molecules in metal complexes - novel materials and intermediates. An important requirement for the future is new materials with unusual properties that can be controlled. The need for ever smaller electronic devices requires knowledge about appropriate properties (particularly electronic) of molecules designed to model devices such as wires, switches, etc. This work seeks to design, measure and evaluate such molecules, which are based on chains of carbon atoms linking metal centres ....All-carbon molecules in metal complexes - novel materials and intermediates. An important requirement for the future is new materials with unusual properties that can be controlled. The need for ever smaller electronic devices requires knowledge about appropriate properties (particularly electronic) of molecules designed to model devices such as wires, switches, etc. This work seeks to design, measure and evaluate such molecules, which are based on chains of carbon atoms linking metal centres which can gain or lose electrons readily. As the electronic structure changes, so do the physical (photo, solid-state) and chemical properties (reactivity). Improved understanding of these features will benefit development of advanced technology and new materials.Read moreRead less
Low Temperature Catlytic Wet Oxidation of Organics from Strippped Sour Water. The commercialisation of a ~$3billion Australian oil shale industry heavily depends upon environmental sustainability of its technology. One key environmental issue of this technology is a need to remove organics from an aqueous industrial stream (stripped sour water). This proposal aims to develop a method based on catalytic wet oxidation for removing organics from stripped sour water. Research will be focused to deve ....Low Temperature Catlytic Wet Oxidation of Organics from Strippped Sour Water. The commercialisation of a ~$3billion Australian oil shale industry heavily depends upon environmental sustainability of its technology. One key environmental issue of this technology is a need to remove organics from an aqueous industrial stream (stripped sour water). This proposal aims to develop a method based on catalytic wet oxidation for removing organics from stripped sour water. Research will be focused to develop and study potential catalytic systems to lower the activation energy of the rate-determining step and to increase the rate of organics oxidation. The development of such a method would be a substantial technology achievement with many applications in pollution control for wastewater treatment in many other industries.Read moreRead less
Investigation of the variation and origin of contaminants present in recycled PET. Recycling and waste management are of ever increasing concern in today's consumer society and our capacity to recycle waste is directly reliant on our ability to lower contamination levels and ensure consumer safety. Using novel analytical techniques, this project aims to characterise contaminants found in recycled PET and identify the source(s) of this contamination. Ultimately this will lead to a reduction in re ....Investigation of the variation and origin of contaminants present in recycled PET. Recycling and waste management are of ever increasing concern in today's consumer society and our capacity to recycle waste is directly reliant on our ability to lower contamination levels and ensure consumer safety. Using novel analytical techniques, this project aims to characterise contaminants found in recycled PET and identify the source(s) of this contamination. Ultimately this will lead to a reduction in recycled PET contamination levels, and allow a more complete recycling process. The global objective being to generate enough relevant scientific data to assist Visy in its endeavours to achieve higher levels of environmental performances and sustainable product development.Read moreRead less
From Nanostructured Functional Materials to Sustainable Processes. Nano-structured functional materials in the areas of catalysis and reversible hydrogen storage will be developed with the view to arrive at (a) sustainable processes and (b) the adoption of hydrogen as an energy carrier. These aims are driven by a global need to change the industrial paradigm due to environmental pressures and limited resources, particularly in terms of energy. Expected outcomes are new avenues to process intens ....From Nanostructured Functional Materials to Sustainable Processes. Nano-structured functional materials in the areas of catalysis and reversible hydrogen storage will be developed with the view to arrive at (a) sustainable processes and (b) the adoption of hydrogen as an energy carrier. These aims are driven by a global need to change the industrial paradigm due to environmental pressures and limited resources, particularly in terms of energy. Expected outcomes are new avenues to process intensification, leading to novel commercial routes, and a hydrogen storage technology which has the potential to play a strong part in the global economy.Read moreRead less
Metallographitic Discs as New Materials. Materials science plays a pivotal role in determining and improving economic performance and quality of life. While application of materials is the ultimate goal, basic understanding of a material's behaviour from the atomic/nano-level to macrostructural level is also of critical importance. This project builds upon the recent success of soluble, well-defined carbon discs in molecular electronics, through the preparation and study of metal-containing deri ....Metallographitic Discs as New Materials. Materials science plays a pivotal role in determining and improving economic performance and quality of life. While application of materials is the ultimate goal, basic understanding of a material's behaviour from the atomic/nano-level to macrostructural level is also of critical importance. This project builds upon the recent success of soluble, well-defined carbon discs in molecular electronics, through the preparation and study of metal-containing derivatives as new advanced crystalline and liquid crystalline materials. The possibility of enhanced electronic, optical and/or magnetic properties, along with good processability, make these materials potential candidates as the active component of future, technologically important devices.Read moreRead less