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Energy transforming polymers: from single molecules to devices. Climate control and the rapidly increasing demand for energy is driving the search for alternative sustainable energy sources. Flexible plastics will be a primary component of the new generation of solar harvesting and energy conversion materials. The objective of this project is to gain an understanding of the way polymers interact with light and can convert absorbed solar energy into electrical power and other useful forms of ene ....Energy transforming polymers: from single molecules to devices. Climate control and the rapidly increasing demand for energy is driving the search for alternative sustainable energy sources. Flexible plastics will be a primary component of the new generation of solar harvesting and energy conversion materials. The objective of this project is to gain an understanding of the way polymers interact with light and can convert absorbed solar energy into electrical power and other useful forms of energy. The outcomes of the project will allow the improved design of plastics for applications in solar energy conversion.Read moreRead less
Polyoxometalate Clusters: Catalytic Chemistry in Solution and Condensed States. Polyoxometalate cluster anions are soluble metal-oxygen clusters that are cheap, robust and non-toxic.
Conditions for systematic tuning of redox potentials over the range +2 to -3 V have become accessible via certain photo-active polyoxometalates. The same system can provide powerful oxidants (that rival chlorine) and powerful reductants (that rival potassium).
The program will take advantage of this unique ....Polyoxometalate Clusters: Catalytic Chemistry in Solution and Condensed States. Polyoxometalate cluster anions are soluble metal-oxygen clusters that are cheap, robust and non-toxic.
Conditions for systematic tuning of redox potentials over the range +2 to -3 V have become accessible via certain photo-active polyoxometalates. The same system can provide powerful oxidants (that rival chlorine) and powerful reductants (that rival potassium).
The program will take advantage of this unique range of properties to explore:-
(i) coupling of photo- and electro-chemical processes into effective catalytic cycles;
(ii) photo- and electro-chemical processes in ionic liquid solvents;
(iii) synthesis and redox reactivity of nanoparticles stabilised by polyoxometalates.
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PROCESSING OF REDUCED-BAND-GAP TITANIA FOR SOLAR-HYDROGEN. The present project involves the development of materials and devices for solar-hydrogen using photo-assisted water decomposition. The research focusses on the processing of titanium dioxide (titania) with substantially enhanced photo-sensitivity and, consequently, increased efficiency of the conversion of solar energy into chemical energy (hydrogen) through imposition of the optimal Ti/O ratio. Significance: processing technology of tit ....PROCESSING OF REDUCED-BAND-GAP TITANIA FOR SOLAR-HYDROGEN. The present project involves the development of materials and devices for solar-hydrogen using photo-assisted water decomposition. The research focusses on the processing of titanium dioxide (titania) with substantially enhanced photo-sensitivity and, consequently, increased efficiency of the conversion of solar energy into chemical energy (hydrogen) through imposition of the optimal Ti/O ratio. Significance: processing technology of titania for photo-electrochemical devices for hydrogen generation and water decontamination. Innovation: processing of titania with reduced band-gap to be achieved through optimised oxygen nonstoichiometry. Outcome: processing technology of titania with outstanding photo-sensitivity.Read moreRead less
Flexible dye-sensitised solar cells on polymer substrates. The expected outcomes of the project are the preparation and development of flexible solar cells. The resulting portable and compact solar cells could be incorporated in fabrics opening the solar cell market to the clothing industry. The products and mechanisms developed are envisaged to be amenable to large scale-up in industry. Hence, at a future date, there is the potential to fabricate the cells in Australia and then export the mater ....Flexible dye-sensitised solar cells on polymer substrates. The expected outcomes of the project are the preparation and development of flexible solar cells. The resulting portable and compact solar cells could be incorporated in fabrics opening the solar cell market to the clothing industry. The products and mechanisms developed are envisaged to be amenable to large scale-up in industry. Hence, at a future date, there is the potential to fabricate the cells in Australia and then export the materials and technology. This will benefit the Australian economy through employment of Australians and income generated through exports.Read moreRead less
ARC Centre of Excellence - Australian Centre for Electromaterials Science. The Centre will tackle some of the biggest challenges facing society: those of renewable energy, sustainable industries and enhancing human health. Improvements in all these areas are possible by developing electromaterials with improved efficiency in the generation and transfer of electrical charge. By developing new nano-materials and new theories to explain their behaviour, the Centre will make advances in the areas ....ARC Centre of Excellence - Australian Centre for Electromaterials Science. The Centre will tackle some of the biggest challenges facing society: those of renewable energy, sustainable industries and enhancing human health. Improvements in all these areas are possible by developing electromaterials with improved efficiency in the generation and transfer of electrical charge. By developing new nano-materials and new theories to explain their behaviour, the Centre will make advances in the areas of human health through the regeneration of damaged nerves (eg. in spinal injury) and development of artificial muscles; in renewable energy (plastic solar cells, lightweight batteries and electronic textiles) and in sustainable industries (recovery of precious metals and new corrosion protection technologies).Read moreRead less
Computational approaches to selection and design of ionic materials. Advanced batteries, fuel cells and solar cell technologies are beginning to use ionic liquids/plastic crystals as electrolytes due to their superb stability and valuable properties. As a broad class these ionic materials have only been known for the last 10 years or so and there is much to learn about their structure and properties. The project will develop and advance quantum chemical techniques for selection and design of ion ....Computational approaches to selection and design of ionic materials. Advanced batteries, fuel cells and solar cell technologies are beginning to use ionic liquids/plastic crystals as electrolytes due to their superb stability and valuable properties. As a broad class these ionic materials have only been known for the last 10 years or so and there is much to learn about their structure and properties. The project will develop and advance quantum chemical techniques for selection and design of ionic materials with the goal of developing electrolytes for a range of applications from advanced metal batteries, solar cells to fuel cells. These applications will have impact on energy efficiency and energy conservation by enabling CO2 replacing technologies. Read moreRead less
Fully ab initio, large-scale calculations of thermodynamic and transport properties of ionic materials. Advanced batteries, fuel cells, and photonic device technologies are beginning to use ionic materials as electrolytes due to their superb stability and technologically valuable properties. As a broad class these materials have only been known for just over a decade and there is still more unknown than known about their structure and properties. The project will develop new advanced computation ....Fully ab initio, large-scale calculations of thermodynamic and transport properties of ionic materials. Advanced batteries, fuel cells, and photonic device technologies are beginning to use ionic materials as electrolytes due to their superb stability and technologically valuable properties. As a broad class these materials have only been known for just over a decade and there is still more unknown than known about their structure and properties. The project will develop new advanced computational methods as a basis for understanding their properties and thereby allowing us to design-in desired features. Ultimately these advances will have support the development of energy efficient CO2 replacement technologies.Read moreRead less
Novel Materials for Dye Sensitised Solar Cells. Solar energy is the most attractive renewable energy source. Dye sensitised solar cells (DSSCs) are one type of device that can harvest this energy, offering advantages of low materials cost and ease of fabrication when compared to alternative devices. This project aims to develop efficient, flexible DSSCs by using polymer substrates in place of glass. Novel surface modification approaches and microwave processing will be employed to fabricate the ....Novel Materials for Dye Sensitised Solar Cells. Solar energy is the most attractive renewable energy source. Dye sensitised solar cells (DSSCs) are one type of device that can harvest this energy, offering advantages of low materials cost and ease of fabrication when compared to alternative devices. This project aims to develop efficient, flexible DSSCs by using polymer substrates in place of glass. Novel surface modification approaches and microwave processing will be employed to fabricate the nanporous semiconductor electrodes on polymer substrates and to improve cell efficiency. Improved dyes and new electrolyte systems, such as plastic crystals, will be incorporated into the cell to improve efficiency, durability and stability.Read moreRead less
MICROWAVE PROCESSING OF FLEXIBLE DYE SENSITISED SOLAR CELLS. Solar energy is the most attractive renewable and environmentally sustainable energy source. Dye sensitised solar cells (DSSCs) are one type of device that can harvest this energy, offering advantages of low materials cost and ease of fabrication when compared to silicon-based solar cells. This project aims to develop efficient, flexible DSSCs by using polymer substrates in place of glass. Microwave processing will be employed to fabr ....MICROWAVE PROCESSING OF FLEXIBLE DYE SENSITISED SOLAR CELLS. Solar energy is the most attractive renewable and environmentally sustainable energy source. Dye sensitised solar cells (DSSCs) are one type of device that can harvest this energy, offering advantages of low materials cost and ease of fabrication when compared to silicon-based solar cells. This project aims to develop efficient, flexible DSSCs by using polymer substrates in place of glass. Microwave processing will be employed to fabricate the semiconductor layers on polymer substrates. Novel surface modification approaches will be examined to facilitate microwave processing and improve cell efficienRead moreRead less
Ionic Liquids and Solids - New Designs, Insights and Applications. Ionic Materials in the form of liquid salts and plastic crystals are of interest in a wide range of applications including environmentally benign synthesis of chemicals and high stability electrolytes for batteries, capacitors and other devices. These materials represent some of the most stable chemicals known, making them attractive for any application where complete stability and recycling are issues. Building on our recent wor ....Ionic Liquids and Solids - New Designs, Insights and Applications. Ionic Materials in the form of liquid salts and plastic crystals are of interest in a wide range of applications including environmentally benign synthesis of chemicals and high stability electrolytes for batteries, capacitors and other devices. These materials represent some of the most stable chemicals known, making them attractive for any application where complete stability and recycling are issues. Building on our recent work, this project will design, prepare and characterize novel materials of this type for a number of target applications. Collaborators in Europe and USA will be involved in the analysis and testing of the materials.Read moreRead less