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Polynuclear Metal Complexes as Molecular Nanomagnets. Computer hard drives and other devices use tiny particles of magnetic materials to store digital information. Technological advances require an increase in the density of information storage and therefore even smaller magnetic particles. This project has the potential to synthesise materials where a single molecule could act as the smallest possible unit of magnetic memory. The future application of these materials may provide an increase ....Polynuclear Metal Complexes as Molecular Nanomagnets. Computer hard drives and other devices use tiny particles of magnetic materials to store digital information. Technological advances require an increase in the density of information storage and therefore even smaller magnetic particles. This project has the potential to synthesise materials where a single molecule could act as the smallest possible unit of magnetic memory. The future application of these materials may provide an increase of three orders of magnitude in information storage density. In addition, they may find employment in quantum computers, which can perform calculations exponentially faster than conventional computers.Read moreRead less
An Integrated Synthetic and NMR Spectroscopic Study of Photochemical Organometallic Bond Activation. Modifications of alkanes and related processes under study will occupy the heart of next generation catalysed chemical processes that may ultimately be used globally on a vast scale. A detailed knowledge of mechanism is the precursor to rational design and improvement of catalysed processes, making them more efficient and greener. This will allow better usage of Australia's natural gas and preci ....An Integrated Synthetic and NMR Spectroscopic Study of Photochemical Organometallic Bond Activation. Modifications of alkanes and related processes under study will occupy the heart of next generation catalysed chemical processes that may ultimately be used globally on a vast scale. A detailed knowledge of mechanism is the precursor to rational design and improvement of catalysed processes, making them more efficient and greener. This will allow better usage of Australia's natural gas and precious metal resources and benefit local chemical companies. Specialized new NMR technology that will greatly aid a wide range of local researchers will be developed to facilitate these studies. The researchers of the future will also be trained.Read moreRead less
Smart Molecular Materials for Sensors, Displays and Nanodevices. The aims of this project are to synthesise new smart molecular materials and elucidate the chemical origin of the physical properties they exhibit. Exposure of these transition metal-based compounds to heat or light will induce changes in colour and magnetic behaviour, affording potential roles as the smallest possible electronic components or addressable entities for high density data storage. It is expected that the materials wil ....Smart Molecular Materials for Sensors, Displays and Nanodevices. The aims of this project are to synthesise new smart molecular materials and elucidate the chemical origin of the physical properties they exhibit. Exposure of these transition metal-based compounds to heat or light will induce changes in colour and magnetic behaviour, affording potential roles as the smallest possible electronic components or addressable entities for high density data storage. It is expected that the materials will also exhibit tunable thermochromic and photochromic properties, which are important for applications in photoresponsive devices or temperature sensors. The structure-function relationships determined will inform the development of molecular materials for future nanodevices, sensors or displays.Read moreRead less
New platforms for molecular electronics. Molecular electronics involves the integration of molecules with solid-state electronics and is seen as an answer to the growing need for ultradense and ultrafast computation. This project will design molecular-based components specifically intended for solid-state applications, such as molecular-based memory.
Harnessing redox-active ligands in functional metal complexes. This project aims to synthesise and investigate metal-based molecules that can be reversibly switched between forms with different physical properties, such as colour or electrical conductivity, upon exposure to heat, light or electrical potential. The project expects to develop compounds that offer physical properties relevant for deployment in advanced materials or nanodevices. Expected outcomes of this project include elucidation ....Harnessing redox-active ligands in functional metal complexes. This project aims to synthesise and investigate metal-based molecules that can be reversibly switched between forms with different physical properties, such as colour or electrical conductivity, upon exposure to heat, light or electrical potential. The project expects to develop compounds that offer physical properties relevant for deployment in advanced materials or nanodevices. Expected outcomes of this project include elucidation of chemical routes to tuning the switchability and candidate compounds for future applications. As well as achieving important advances in fundamental chemistry, this project should provide significant benefits, such as novel materials for molecular electronics/spintronics, photoresponsive devices or sensors.Read moreRead less
Mixed valence coordination polymers and their electronic properties. The project aims to synthesise and examine the properties of crystalline coordination polymers that exhibit unusual and technologically useful properties arising from long-range electronic communication. The focus will be on materials in which the modular components (ligands, metals and counterions) are present in mixed valence states. The experimental investigation will be supported by dispersion-corrected, periodic-boundary D ....Mixed valence coordination polymers and their electronic properties. The project aims to synthesise and examine the properties of crystalline coordination polymers that exhibit unusual and technologically useful properties arising from long-range electronic communication. The focus will be on materials in which the modular components (ligands, metals and counterions) are present in mixed valence states. The experimental investigation will be supported by dispersion-corrected, periodic-boundary DFT calculations which will be employed to both rationalise behaviour and provide direction for the generation of new materials.Read moreRead less
Synthetic Molybdenum Enzymes. This project aims to produce synthetic molybdenum (Mo) enzymes, small molecules that share structural and functional attributes with the crucially important molybdopterin?Mo enzymes. These ubiquitous enzymes are essential for plant and animal health, natural cycles involving carbon, nitrogen and sulfur, and global climate control and atmospheric albedo (reflectance); consequently, they impact heavily on commerce, the environment and society. The study will provid ....Synthetic Molybdenum Enzymes. This project aims to produce synthetic molybdenum (Mo) enzymes, small molecules that share structural and functional attributes with the crucially important molybdopterin?Mo enzymes. These ubiquitous enzymes are essential for plant and animal health, natural cycles involving carbon, nitrogen and sulfur, and global climate control and atmospheric albedo (reflectance); consequently, they impact heavily on commerce, the environment and society. The study will provide urgently needed insights into the fundamental Mo?sulfur chemistry of the enzyme active sites and inform efforts to reduce the negative impacts of enzyme dysfunction and the design of new commercial catalysts.Read moreRead less
Bioinorganic Chemistry of Molybdenum. Enzymes containing the trace element molybdenum play crucial roles in plant, animal and human health, drug metabolism, environmental processes and climate. This international, multidisciplinary project will advance our understanding of the structure and function of these enzymes at the atomic level and inform strategies to reduce the impact of crop, livestock and human diseases and adverse environmental (e.g. algal blooms, leaching of toxic arsenic) and clim ....Bioinorganic Chemistry of Molybdenum. Enzymes containing the trace element molybdenum play crucial roles in plant, animal and human health, drug metabolism, environmental processes and climate. This international, multidisciplinary project will advance our understanding of the structure and function of these enzymes at the atomic level and inform strategies to reduce the impact of crop, livestock and human diseases and adverse environmental (e.g. algal blooms, leaching of toxic arsenic) and climatic events. Effective strategies would be of enormous social and economic benefit to Australia. The training of skilled scientists and access to major overseas facilities are additional benefits of the project.Read moreRead less
New molecular architectures: synthesis, structure and properties. Through the implementation of rational design principles we intend to generate new types of nanoporous materials by bringing together molecular building blocks of appropriate size, shape and functionality. With such systems able to act as hosts for small molecules we expect that novel and technologically useful properties will arise.
X-ray snapshots of chemical transformations in open framework materials. The aim of this project is to unearth structural insights into the chemistry of coordinatively unsaturated metal complexes – reactive species lacking their full complement of binding groups – by isolating them within a carefully designed metal-organic framework and examining them via single crystal X-ray diffraction. Such intrinsically reactive species play an important role in metal-based catalysis, but their definitive st ....X-ray snapshots of chemical transformations in open framework materials. The aim of this project is to unearth structural insights into the chemistry of coordinatively unsaturated metal complexes – reactive species lacking their full complement of binding groups – by isolating them within a carefully designed metal-organic framework and examining them via single crystal X-ray diffraction. Such intrinsically reactive species play an important role in metal-based catalysis, but their definitive structural characterisation remains a significant challenge. This project aims to facilitate a detailed understanding of how these species bind and activate substrates and thus provide important first steps towards developing novel adsorbents for separations and efficient catalysts.Read moreRead less