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Discovery Early Career Researcher Award - Grant ID: DE240100068
Funder
Australian Research Council
Funding Amount
$417,237.00
Summary
Original metal-based catalysts for enzyme-inspired CO2 activation. The chemical utilisation of CO2 is one of two major strategies in achieving net negative CO2 emissions mitigating the environmental and socioeconomic damage of global warming. Inspired by the ability of natural enzymes to efficiently utilise molecules like CO2, this project aims to develop original metal-based catalysts as enzyme mimics for the efficient transformation of CO2. It will deliver practical strategies to transform CO2 ....Original metal-based catalysts for enzyme-inspired CO2 activation. The chemical utilisation of CO2 is one of two major strategies in achieving net negative CO2 emissions mitigating the environmental and socioeconomic damage of global warming. Inspired by the ability of natural enzymes to efficiently utilise molecules like CO2, this project aims to develop original metal-based catalysts as enzyme mimics for the efficient transformation of CO2. It will deliver practical strategies to transform CO2 into value-added materials permanently removing it from the atmosphere. Project outcomes are expected to enhance industry’s capacity to use CO2 as a feedstock chemical for the production of fuels and materials, providing significant economic and environmental benefits through CO2 upcycling and recycling.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE140101137
Funder
Australian Research Council
Funding Amount
$389,470.00
Summary
Synthesis, Structure and Utility of Novel P-chiral and C-chiral Organophosphido Metal Complexes . The formation of new molecules requires original methods to achieve their synthesis with greatest efficiency. Organometallic chemistry remains crucial for establishing novel reagents and processes. Driven by advances in organo-multi-metallic chemistry this project will build upon fundamental concepts in main group and transition metal chemistry to establish the area of phosphorous-chiral and carbon- ....Synthesis, Structure and Utility of Novel P-chiral and C-chiral Organophosphido Metal Complexes . The formation of new molecules requires original methods to achieve their synthesis with greatest efficiency. Organometallic chemistry remains crucial for establishing novel reagents and processes. Driven by advances in organo-multi-metallic chemistry this project will build upon fundamental concepts in main group and transition metal chemistry to establish the area of phosphorous-chiral and carbon-chiral organophosphido metal chemistry. By rationally designing and integrating new chiral phosphido ligands into mono- and mixed-metal organometallic complexes, chemists will have access to a suite of new tools for application in asymmetric synthesis and catalysis, all relevant to the fields of structural, sustainable and biological chemistry.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE230100978
Funder
Australian Research Council
Funding Amount
$406,818.00
Summary
A new Iron Age! Making Iron complexes fit for C-C cross-coupling catalysis. This project aims to develop new iron catalysts as alternatives to the expensive and increasingly rare noble metals currently used in C-C bond forming reactions, the most important single-step in the fine-chemicals sector.
This project expects to create a flexible yet robust framework by introducing a hemilabile ligand into the backbone of the iron complex to control the number of vacant coordination sites.
Expected outc ....A new Iron Age! Making Iron complexes fit for C-C cross-coupling catalysis. This project aims to develop new iron catalysts as alternatives to the expensive and increasingly rare noble metals currently used in C-C bond forming reactions, the most important single-step in the fine-chemicals sector.
This project expects to create a flexible yet robust framework by introducing a hemilabile ligand into the backbone of the iron complex to control the number of vacant coordination sites.
Expected outcomes of this project are 1) iron complexes able to catalyse biaryl couplings from sustainable substrates and 2) knowledge on structure-property relationships of iron-based catalytic processes.
Australia will benefit by applying its own resources and help preserving the valuable noble metals for processes relying on them.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE190100524
Funder
Australian Research Council
Funding Amount
$422,574.00
Summary
Heterometallic iron-molybdenum complexes for nitrogen activation. This project aims to develop a range of bio-inspired, mixed metal iron-molybdenum complexes that are capable of activating molecular nitrogen, N2, at ambient pressure and temperature. The activation of atmospheric N2 is performed on a multi-million tonne scale each year and is key to a number of industrial processes. The project expects to generate new knowledge in the area of organometallic chemistry, specifically with regards to ....Heterometallic iron-molybdenum complexes for nitrogen activation. This project aims to develop a range of bio-inspired, mixed metal iron-molybdenum complexes that are capable of activating molecular nitrogen, N2, at ambient pressure and temperature. The activation of atmospheric N2 is performed on a multi-million tonne scale each year and is key to a number of industrial processes. The project expects to generate new knowledge in the area of organometallic chemistry, specifically with regards to molecular metal-metal bonding and subsequent reactivity towards the activation of N2. Expected outcomes include new and improved catalysts, which will provide significant financial benefits to industry, as well as benefiting the environment by reducing energy demand.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE200100450
Funder
Australian Research Council
Funding Amount
$425,398.00
Summary
Cooperativity by Design: Unlocking Metal-Metal-Ligand Cooperativity. This proposal aims to deliver efficient chemical hydrogen storage by designing new catalysts to facilitate the storage and release of hydrogen fuel. Hydrogen is an important zero-emission fuel for the low carbon energy future. However, to realise the potential of the hydrogen economy, efficient, cost-effective solutions are required for storage and transportation. This project seeks to provide technological and intellectual adv ....Cooperativity by Design: Unlocking Metal-Metal-Ligand Cooperativity. This proposal aims to deliver efficient chemical hydrogen storage by designing new catalysts to facilitate the storage and release of hydrogen fuel. Hydrogen is an important zero-emission fuel for the low carbon energy future. However, to realise the potential of the hydrogen economy, efficient, cost-effective solutions are required for storage and transportation. This project seeks to provide technological and intellectual advances in chemical hydrogen storage methods. These outcomes are expected to provide environmental and economic benefits for Australia’s developing hydrogen economy, both in the energy export market and locally in utilisation of hydrogen as a sustainable fuel.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE170100540
Funder
Australian Research Council
Funding Amount
$360,000.00
Summary
Site-specific modification of proteins with radioactive technetium. This project aims to produce homogeneous and fully functional constructs that may be used as imaging agents. Most techniques for incorporating radioactive isotopes into proteins adversely influence biological behaviour and the quality of the image. This project will develop technology for the benign modification of proteins with the radioactive isotope technetium for nuclear imaging. Development of the fundamental chemistry in t ....Site-specific modification of proteins with radioactive technetium. This project aims to produce homogeneous and fully functional constructs that may be used as imaging agents. Most techniques for incorporating radioactive isotopes into proteins adversely influence biological behaviour and the quality of the image. This project will develop technology for the benign modification of proteins with the radioactive isotope technetium for nuclear imaging. Development of the fundamental chemistry in this project may lead to future applications in imaging and therapy. Creation of intellectual property could lead to joint ventures with hospitals and industry.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE160100732
Funder
Australian Research Council
Funding Amount
$359,544.00
Summary
Electrostatic Catalysis: guiding reactive interfaces using electric fields. This project seeks to gain quantitative understanding of the role of electrostatics over chemical processes. Chemical transformations of organic compounds at interfaces underpin some of the most important processes, from the production of fine chemicals for pharmaceuticals to assisting bio-degradation of pollutants in clean technologies. Recent computational studies suggest that by applying oriented electric fields at in ....Electrostatic Catalysis: guiding reactive interfaces using electric fields. This project seeks to gain quantitative understanding of the role of electrostatics over chemical processes. Chemical transformations of organic compounds at interfaces underpin some of the most important processes, from the production of fine chemicals for pharmaceuticals to assisting bio-degradation of pollutants in clean technologies. Recent computational studies suggest that by applying oriented electric fields at interfaces, the rate and the selectivity of chemical processes can be altered at will. The project intends to test these theoretical findings. The knowledge generated by this research may translate into new technologies for the fine-chemical and biotechnology industries.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE180100462
Funder
Australian Research Council
Funding Amount
$364,975.00
Summary
Molecular complexity through multi-bond forming reactions. This project aims to develop techniques for the synthesis of many, highly valuable natural and designed molecules which are too complex to be synthesised on scale with current methodologies. The project aims to develop new strategies for the simultaneous construction of several chemical bonds, with a focus on molecular scaffolds that can be readily converted into pharmaceuticals, potential drug candidates, chiral ligands, and agrochemica ....Molecular complexity through multi-bond forming reactions. This project aims to develop techniques for the synthesis of many, highly valuable natural and designed molecules which are too complex to be synthesised on scale with current methodologies. The project aims to develop new strategies for the simultaneous construction of several chemical bonds, with a focus on molecular scaffolds that can be readily converted into pharmaceuticals, potential drug candidates, chiral ligands, and agrochemicals. This will ultimately lead to advancements in both the production and application of organic molecules in these fields.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE220101471
Funder
Australian Research Council
Funding Amount
$441,100.00
Summary
Controlling uranium species to its long-term stability in bioremediation. This project aims to reveal the mechanisms of uranium transformation and immobilisation in both aerobic and anaerobic conditions of bioremediation with the emphasis on elucidating stable uranium immobilised under different pathways and conditions. This project expects to generate new knowledge regarding the relationship between uranium speciation and stability with the matrix mineral, microbiota, and environmental conditio ....Controlling uranium species to its long-term stability in bioremediation. This project aims to reveal the mechanisms of uranium transformation and immobilisation in both aerobic and anaerobic conditions of bioremediation with the emphasis on elucidating stable uranium immobilised under different pathways and conditions. This project expects to generate new knowledge regarding the relationship between uranium speciation and stability with the matrix mineral, microbiota, and environmental conditions. Expected outcomes from this project include new strategies for preferential immobilisation of uranium to stable species that are resistant to air and acid. The anticipated benefits of this project include mitigating uranium contamination and promoting the sustainable development of the uranium industry in Australia.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE150100263
Funder
Australian Research Council
Funding Amount
$373,536.00
Summary
Halogen Bonding for Assembly and Separation in Solution. The properties of substances we experience in our daily lives owe much to very weak interactions taking place between molecules. Consider a cup of coffee: very weak interactions hold the water together as a liquid, and result in the biological action of caffeine within the body. The project aims to develop new materials based on an underexplored class of weak interactions known as halogen bonds. These interactions will be used to assemble ....Halogen Bonding for Assembly and Separation in Solution. The properties of substances we experience in our daily lives owe much to very weak interactions taking place between molecules. Consider a cup of coffee: very weak interactions hold the water together as a liquid, and result in the biological action of caffeine within the body. The project aims to develop new materials based on an underexplored class of weak interactions known as halogen bonds. These interactions will be used to assemble large molecules in solution, probe the presence of pollutants in water, and to separate active and inactive forms of pharmaceuticals. The development of health and environmental applications in the course of this project aim to significantly enhance our fundamental understanding of these weak interactions.Read moreRead less