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Bimolecular chemistry at very low temperatures. Many chemical reactions involve short-lived and highly reactive intermediates that cannot be observed under ordinary reaction conditions. Hence, much of this chemistry is shrouded in mystery. This project aims to develop the ability to observe and monitor such reactions directly using a combination of spectroscopies at very low temperatures, where the molecules are more stable and reactions slower. These studies will give quantitative information ....Bimolecular chemistry at very low temperatures. Many chemical reactions involve short-lived and highly reactive intermediates that cannot be observed under ordinary reaction conditions. Hence, much of this chemistry is shrouded in mystery. This project aims to develop the ability to observe and monitor such reactions directly using a combination of spectroscopies at very low temperatures, where the molecules are more stable and reactions slower. These studies will give quantitative information on the nature of the reactive intermediates themselves, the nature of the products formed, and the reaction dynamics, and they are of fundamental importance for an understanding of chemical reactivity generally. The methodology developed will be applicable to the investigation of a wide range of processes.Read moreRead less
Gas phase studies of the interactions of electrons with peptide ions: structure assignment and fundamentals. Electron-induced reactions are fundamental to a wide range of processes that underlie many areas of science and technology, ranging from planetary atmospheres, industrial plasmas to living tissues. Since ionizing radiation is believed to be a major cause of damage to living cells, understanding electron interactions with biological molecules is essential to predict the consequences of ex ....Gas phase studies of the interactions of electrons with peptide ions: structure assignment and fundamentals. Electron-induced reactions are fundamental to a wide range of processes that underlie many areas of science and technology, ranging from planetary atmospheres, industrial plasmas to living tissues. Since ionizing radiation is believed to be a major cause of damage to living cells, understanding electron interactions with biological molecules is essential to predict the consequences of exposure. Structure determination of biomolecules is at the heart of identifying, diagnosing and potentially developing treatments for diseases, and thus another important reason for studying these interactions is the potential to develop new mass spectrometry based analytical methods.Read moreRead less
Development of a test bed for molecular memory and molecular photovoltaic devices. The development of nanostructured materials and the devices that utilize them is at the forefront of modern science and technology. Electrical devices whose functional units are structurally ordered single molecules dominate biochemical processes, especially pertinent ones being photosynthesis and cellular energy production; artificial devices promise new technologies in multi-$B markets such as long-term data st ....Development of a test bed for molecular memory and molecular photovoltaic devices. The development of nanostructured materials and the devices that utilize them is at the forefront of modern science and technology. Electrical devices whose functional units are structurally ordered single molecules dominate biochemical processes, especially pertinent ones being photosynthesis and cellular energy production; artificial devices promise new technologies in multi-$B markets such as long-term data storage and renewable solar-energy production. Interfacing molecules with macroscopic interconnects poses a great technological challenge, however, and in this project the underlying basic science will be determined through the formation of molecules into device-accessible functional materials.Read moreRead less
Electrochemistry of redox-active non-metal compounds. Unsaturated compounds of heavier non-metal elements can exist in multiple stable redox states. The interconversion is best assessed by electrochemical techniques, which can measure the energetics and the mechanism of the redox processes involved in both solution and solid state phases. Compounds to be studied will be prepared in the Canadian laboratories of the partner investigator. The electrochemical and spectroelectrochemical properties ....Electrochemistry of redox-active non-metal compounds. Unsaturated compounds of heavier non-metal elements can exist in multiple stable redox states. The interconversion is best assessed by electrochemical techniques, which can measure the energetics and the mechanism of the redox processes involved in both solution and solid state phases. Compounds to be studied will be prepared in the Canadian laboratories of the partner investigator. The electrochemical and spectroelectrochemical properties will initially be investigated in Australia during the visit of the partner investigator to Monash University with follow up studies in both countries. The mutual skills of synthesis and electrochemistry in the Canadian-Australian laboratories are essential to the project.Read moreRead less
Biomolecular chemical survival strategies of terrestrial extremophiles and the spectroscopic search for life on Mars. This project is aimed to place Australian research at the forefront of developments in the search for extraterrestrial life, the evolution of life on earth, and the design of new probes for the identification of microorganisms. The research will link key centres in Australia and the UK with international space agencies (NASA and the European Space Agency) in the search for cutti ....Biomolecular chemical survival strategies of terrestrial extremophiles and the spectroscopic search for life on Mars. This project is aimed to place Australian research at the forefront of developments in the search for extraterrestrial life, the evolution of life on earth, and the design of new probes for the identification of microorganisms. The research will link key centres in Australia and the UK with international space agencies (NASA and the European Space Agency) in the search for cutting edge techniques to be used in the search for extraterrestrial life forms and their links to paleo and extremophile life forms on Earth. Read moreRead less
Inhibitors of enzymes in the lysine biosynthetic pathway. Recent reports of increasing bacterial resistance to antibiotics highlight the need for continual development of new antibacterial agents. Inhibitors of the biosynthesis of the amino acid lysine - an essential component of bacterial proteins and cell wall - may provide a novel class of antibiotics. This project describes investigations of the mechanism of the first two enzymes in the lysine biosynthetic pathway and the design and synthesi ....Inhibitors of enzymes in the lysine biosynthetic pathway. Recent reports of increasing bacterial resistance to antibiotics highlight the need for continual development of new antibacterial agents. Inhibitors of the biosynthesis of the amino acid lysine - an essential component of bacterial proteins and cell wall - may provide a novel class of antibiotics. This project describes investigations of the mechanism of the first two enzymes in the lysine biosynthetic pathway and the design and synthesis of inhibitors of these enzymes.Read moreRead less
Metabolic engineering of Zymomonas mobilis for higher value fermentation products. This project will provide an opportunity to revolutionise the Australian chemical and sugar industries. Unlike the traditional methods of the petrochemical industry, bioconversion of carbohydrates to chemicals such as succinic acid via fermentation is cosiderably environmental friendly. For the sugar industry this project will provide an opportunity to produce not only conventional sugar products but also high val ....Metabolic engineering of Zymomonas mobilis for higher value fermentation products. This project will provide an opportunity to revolutionise the Australian chemical and sugar industries. Unlike the traditional methods of the petrochemical industry, bioconversion of carbohydrates to chemicals such as succinic acid via fermentation is cosiderably environmental friendly. For the sugar industry this project will provide an opportunity to produce not only conventional sugar products but also high value commodities via the process integration of succinic acid production using agricultural residues such as bagasse. This will contribute to significant levels of job creation in Australia, and further benefits will be that such products will be important both for import replacement and export potential.Read moreRead less
Metabolic engineering to develop recombinant Zymomonas mobilis for the production of fuel ethanol and fermentation chemicals. This project will provide an opportunity to revolutionise the Australian chemical and sugar industries. Unlike the traditional methods of the petrochemical industry, bioconversion of carbohydrates to chemicals, such as succinic acid via fermentation is more considerably environmentally friendly. For the sugar industry this project will provide an opportunity to produce no ....Metabolic engineering to develop recombinant Zymomonas mobilis for the production of fuel ethanol and fermentation chemicals. This project will provide an opportunity to revolutionise the Australian chemical and sugar industries. Unlike the traditional methods of the petrochemical industry, bioconversion of carbohydrates to chemicals, such as succinic acid via fermentation is more considerably environmentally friendly. For the sugar industry this project will provide an opportunity to produce not only conventional sugar products but also high value commodities via the process integration of succinic acid production using agricultural residues, such as bagasse. This will contribute to significant levels of job creation in Australia, with the further benefit that such products will be important for both import replacement and export potential.Read moreRead less
The Development of Novel Task Specific and Biodegradable Ionic Liquids. The advance of ?Green Chemistry? has become a forefront issue in mainstream chemistry. Green Chemistry is aimed at the reduction or elimination of hazardous substances in the design, manufacture and application of chemical products. The advent of ionic liquids (ILs) has made a significant contribution towards these goals. ILs have many beneficial properties including non-volatility, non-flammability, and a large stable liq ....The Development of Novel Task Specific and Biodegradable Ionic Liquids. The advance of ?Green Chemistry? has become a forefront issue in mainstream chemistry. Green Chemistry is aimed at the reduction or elimination of hazardous substances in the design, manufacture and application of chemical products. The advent of ionic liquids (ILs) has made a significant contribution towards these goals. ILs have many beneficial properties including non-volatility, non-flammability, and a large stable liquid range. As ILs advance from academic curiosities to industrial solvents, the need to address the issue of their biodegradability and toxicity is paramount. The key objective of this project is to design new biodegradable and task specific ILs for environmentally friendly industrial use.Read moreRead less
Gating, specificity and regulation of the YggB channel protein from Corynebacterium glutamicum. The proposed research will greatly contribute to our understanding of the functioning of a bacterial membrane channel/transporter, which has played a significant role in biotechnology of commercially important amino acids. A direct national benefit will result from establishing collaboration with a leading German laboratory providing expertise in protein biochemistry and molecular microbiology not ava ....Gating, specificity and regulation of the YggB channel protein from Corynebacterium glutamicum. The proposed research will greatly contribute to our understanding of the functioning of a bacterial membrane channel/transporter, which has played a significant role in biotechnology of commercially important amino acids. A direct national benefit will result from establishing collaboration with a leading German laboratory providing expertise in protein biochemistry and molecular microbiology not available in Australia. The acquired knowledge will present an original contribution which will have a strong impact on a very competitive field of molecular microbiology and biotechnology.Read moreRead less