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Extending the frontiers of organocatalysis: new reactions involving nucleophilic carbenes. High technology solutions to the problems of today and tomorrow require new materials designed for specific activities. This project will deliver new technologies for the rapid and efficient assembly of materials designed for function.
Challenges to organocatalysis. This project aims to use organocatalysis to generate organocatalytic C=C insertion, C-H functionalisation and carbonyl ylide/1,3-dipolar cycloaddition reactions. Organocatalysis has transformed the way chemical synthesis is performed. However, in the early years the focus of this discipline has primarily been enolate type chemistry, and more challenging reactions, such as those involving carbenoid intermediates, have not been contemplated. Previously such reactions ....Challenges to organocatalysis. This project aims to use organocatalysis to generate organocatalytic C=C insertion, C-H functionalisation and carbonyl ylide/1,3-dipolar cycloaddition reactions. Organocatalysis has transformed the way chemical synthesis is performed. However, in the early years the focus of this discipline has primarily been enolate type chemistry, and more challenging reactions, such as those involving carbenoid intermediates, have not been contemplated. Previously such reactions have only been achieved using transition metal catalysts. This project addresses this limitation, allowing the strengths of organocatalysis (abundance and diversity, access to enantiopurity, elemental sustainability) to affect the broader landscape of catalysis. This approach could present an opportunity to examine reactivity patterns, stereoselectivity and cascade design and may lead to new reaction technologies.Read moreRead less
New Reaction Cascades Exploiting N-Heterocyclic Carbenes. Catalytic reactions can enhance the efficiency of chemical synthesis, decreasing environmental and financial cost. This project will undertake the discovery and development of reactions in which a catalyst enables a "production line" of events to provide complex and valuable products. These reactions will proceed with high shape selectivity (enantioselectivity). In addition to new chemical transformations the output of these studies inclu ....New Reaction Cascades Exploiting N-Heterocyclic Carbenes. Catalytic reactions can enhance the efficiency of chemical synthesis, decreasing environmental and financial cost. This project will undertake the discovery and development of reactions in which a catalyst enables a "production line" of events to provide complex and valuable products. These reactions will proceed with high shape selectivity (enantioselectivity). In addition to new chemical transformations the output of these studies includes intellectual capital and human resources, all of which are integral to sustaining a strong chemical manufacturing sector.Read moreRead less
Ring-Strain Relief: Applications in Total Synthesis. This proposal aims to investigate the chemical synthesis of a number of structurally different natural product target molecules by strategies involving the use of either three or four membered ring-strained compounds to afford key synthetic intermediates in an efficient manner. The key aim of this research is to provide more efficient routes to complex natural products and analogues. The research strives to be at the forefront of modern synthe ....Ring-Strain Relief: Applications in Total Synthesis. This proposal aims to investigate the chemical synthesis of a number of structurally different natural product target molecules by strategies involving the use of either three or four membered ring-strained compounds to afford key synthetic intermediates in an efficient manner. The key aim of this research is to provide more efficient routes to complex natural products and analogues. The research strives to be at the forefront of modern synthetic organic chemistry and aims to contribute to the Science of complex molecule synthesis.Read moreRead less
Direct substitution acyl azolium catalysis: new approaches in reaction discovery. New chemical reactions play a central role in the creation of new materials and knowledge for society. This project will develop new catalytic reactions that create useful materials in a rapid and efficient fashion without creating an excessive drain on resources.
Biogenesis inspired total synthesis of natural products. The project will study the chemical synthesis of a number of novel natural products. Most significantly, this project will deliver new methods for organic synthesis of complex molecules. The rewards from the total synthesis of bioactive compounds are enormous for the community and in the education and training of scientists.
Total Synthesis of Myxobacteria Metabolites and Analogues. This project will investigate the total chemical synthesis of complex myxobacteria metabolites. In addition, the synthesis of new analogues of some of these natural products will also be investigated. The project endeavours to develop new methods for chemical synthesis and also to produce new therapeutic products which may possess greater efficacy and superior biological activities than the natural compounds. Most significantly, this pro ....Total Synthesis of Myxobacteria Metabolites and Analogues. This project will investigate the total chemical synthesis of complex myxobacteria metabolites. In addition, the synthesis of new analogues of some of these natural products will also be investigated. The project endeavours to develop new methods for chemical synthesis and also to produce new therapeutic products which may possess greater efficacy and superior biological activities than the natural compounds. Most significantly, this project will deliver natural and new compounds for analysis of anti-cancer activity. The rewards of the development of new synthetic methods are enormous for the community and in the education of our scientists.Read moreRead less
Production and testing of novel bioactive honeys and honey-based cosmetic formulations. The purpose of this project is to evaluate the entire spectrum of plant bioactive compounds that are transferred to the honey and develop novel bioactive honeys with enhanced antimicrobial, antioxidant and anti-inflammatory properties. This project will also develop new honey-based cosmetic products like creams, gels and foams.
Discovery Early Career Researcher Award - Grant ID: DE170101452
Funder
Australian Research Council
Funding Amount
$360,000.00
Summary
Silk-based conformal pressure sensing devices. This project aims to develop silk biomaterials-based biocompatible and conformal pressure sensing devices and systems for sustainable wearable electronics. Biocompatible conformal sensing interfaces and sensor arrays will be developed for real-time highly sensitive measurement of pressure, critical for accurate and comprehensive health monitoring and electronic skins. It is believed that the wearable products will provide comfort, utility and accura ....Silk-based conformal pressure sensing devices. This project aims to develop silk biomaterials-based biocompatible and conformal pressure sensing devices and systems for sustainable wearable electronics. Biocompatible conformal sensing interfaces and sensor arrays will be developed for real-time highly sensitive measurement of pressure, critical for accurate and comprehensive health monitoring and electronic skins. It is believed that the wearable products will provide comfort, utility and accurate physical information to end users, and improve the performance of personnel working in demanding environments, such as in defence forces, athletics and outfield industrial operations, by continuously monitoring physiological parameters.Read moreRead less
Contemporary ecological threats from historical pollution events and their modification by environmental conditions. Many Australian ports have contaminated sediments that are a legacy of industrial pollution. The resuspension of these sediments through shipping or dredging activity represents an obvious, yet unsubstantiated, threat to the biodiversity and health of marine communities living well above the seafloor. This research proposal addresses a strategic knowledge gap with implications for ....Contemporary ecological threats from historical pollution events and their modification by environmental conditions. Many Australian ports have contaminated sediments that are a legacy of industrial pollution. The resuspension of these sediments through shipping or dredging activity represents an obvious, yet unsubstantiated, threat to the biodiversity and health of marine communities living well above the seafloor. This research proposal addresses a strategic knowledge gap with implications for appropriate management of port operations. Identifying the conditions under which contaminated sediments may cause an impact, and the environmental factors that modify these effects, will produce significant advances in scientific understanding and the results will be of strategic interest to all Australian Port Authorities. Read moreRead less