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Mechanistic Studies on Biologically Active Iron Chelators. The need for orally effective drugs as alternatives to invasive treatment regimens such as subcutaneous infusion is an ongoing concern in health care. This is particularly true in people suffering iron overload. In many cases this condition is present at birth and thus the administration of vital iron chelation therapy via the oral route is a much preferred option. We have unearthed a novel series of candidates for iron chelation therapy ....Mechanistic Studies on Biologically Active Iron Chelators. The need for orally effective drugs as alternatives to invasive treatment regimens such as subcutaneous infusion is an ongoing concern in health care. This is particularly true in people suffering iron overload. In many cases this condition is present at birth and thus the administration of vital iron chelation therapy via the oral route is a much preferred option. We have unearthed a novel series of candidates for iron chelation therapy (the pyridine-2-carboxaldehyde isonicotinoyl hydrazone [PCIH] analogues) which show oral activity. These chelators undergo some interesting iron catalysed oxidation chemistry and it is vital that the mechanism of this reaction be elucidated to determine whether it will be of biological significance upon administration of these compounds as iron chelators.Read moreRead less
New Synthetic Routes to the Immobilisation of Mixed Valence Transition Metal Complexes on Conducting Metal Oxides. Highly coloured, electrochemically active transition metal dyes may find application electrochromic devices, where they may switch between contrasting coloured forms through a simple redox reaction. A prerequisite is that the dye be immobilised onto a solid conducting support whilst preserving the electrochemical and optical properties of the dye found in solution. This project tack ....New Synthetic Routes to the Immobilisation of Mixed Valence Transition Metal Complexes on Conducting Metal Oxides. Highly coloured, electrochemically active transition metal dyes may find application electrochromic devices, where they may switch between contrasting coloured forms through a simple redox reaction. A prerequisite is that the dye be immobilised onto a solid conducting support whilst preserving the electrochemical and optical properties of the dye found in solution. This project tackles this problem through a combination of organic and inorganic synthesis to develop new electrochromic dyes that may be attached to mesoporous titania.Read moreRead less
Adsorption and recovery of gold thiosulfate using nanoporous carbon. The gold industry is a major export earner for both Australia and the United States. This collaborative project aims to develop an environmentally acceptable, cost effective process for the recovery of gold from thiosulfate leachate. Development of this process will remove one of the barriers to the acceptance of thiosulfate leaching over conventional cyanide extraction, leading to substantial benefits to the gold industry and ....Adsorption and recovery of gold thiosulfate using nanoporous carbon. The gold industry is a major export earner for both Australia and the United States. This collaborative project aims to develop an environmentally acceptable, cost effective process for the recovery of gold from thiosulfate leachate. Development of this process will remove one of the barriers to the acceptance of thiosulfate leaching over conventional cyanide extraction, leading to substantial benefits to the gold industry and the environment. A successful outcome in the research project would also lead to export earnings resulting from technology transfer and an enhanced reputation for high quality research.Read moreRead less
Green Machining of Powder Metallurgy Based Aluminium Composites. This project will initiate and establish a collaborative research program between Professor Wojciech Z. Misiolek of Lehigh University (Bethlehem, PA, USA) and Professor Graham Schaffer at The University of Queensland. Professor Misiolek will spend an extended six month period at The University of Queensland. The specific aim of the project is to develop a method to machine aluminium composites in the green, or unsintered, state. Th ....Green Machining of Powder Metallurgy Based Aluminium Composites. This project will initiate and establish a collaborative research program between Professor Wojciech Z. Misiolek of Lehigh University (Bethlehem, PA, USA) and Professor Graham Schaffer at The University of Queensland. Professor Misiolek will spend an extended six month period at The University of Queensland. The specific aim of the project is to develop a method to machine aluminium composites in the green, or unsintered, state. This will overcome a major impediment to the wider utilisation of aluminium matrix composites, which have an attractive combination of properties but cannot be formed into complex shapes using conventional processing methodologies.Read moreRead less
Relative quantum information theory. Quantum information encoded in relative degrees of freedom of multiple quantum systems offers striking advantages in communication and cryptography: it is immune to common types of noise and does not require reference systems shared between parties. This project aims to formulate a theory of relative quantum information, to develop practical information processing protocols that take advantage of relative encodings, and to propose proof-of-principle experim ....Relative quantum information theory. Quantum information encoded in relative degrees of freedom of multiple quantum systems offers striking advantages in communication and cryptography: it is immune to common types of noise and does not require reference systems shared between parties. This project aims to formulate a theory of relative quantum information, to develop practical information processing protocols that take advantage of relative encodings, and to propose proof-of-principle experiments in quantum optics that reveal these advantages. Expected outcomes include powerful communication and cryptographic protocols, a design for programmable quantum computation, and a fundamentally relative theory of quantum information connecting with other foundational fields of physics.Read moreRead less
Nanostructures of Titanium Dioxide and Titanates by Wet-chemistry. One-dimensional (1D) nanoparticulates of titanium dioxide (TiO2) and titanate synthesized by wet-chemistry approaches are new advanced materials of unusual properties. This project will investigate the formation and phase transition mechanism of these 1D particulates by various techniques. With such knowledge, we can effectively control the morphology on a scale of nanometers, and tailor the energy gap of these materials. This wi ....Nanostructures of Titanium Dioxide and Titanates by Wet-chemistry. One-dimensional (1D) nanoparticulates of titanium dioxide (TiO2) and titanate synthesized by wet-chemistry approaches are new advanced materials of unusual properties. This project will investigate the formation and phase transition mechanism of these 1D particulates by various techniques. With such knowledge, we can effectively control the morphology on a scale of nanometers, and tailor the energy gap of these materials. This will significantly influence the photosemiconductive photocatalytic and lithium ions insertion behaviours of the particles so that advanced materials for solar energy conversion, photocatalysts for decomposing organic pollutants in environment, eletrode materials of lithium batteries can be developed.Read moreRead less
Bimolecular chemistry at very low temperatures. Many chemical reactions involve short-lived and highly reactive intermediates that cannot be observed under ordinary reaction conditions. Hence, much of this chemistry is shrouded in mystery. This project aims to develop the ability to observe and monitor such reactions directly using a combination of spectroscopies at very low temperatures, where the molecules are more stable and reactions slower. These studies will give quantitative information ....Bimolecular chemistry at very low temperatures. Many chemical reactions involve short-lived and highly reactive intermediates that cannot be observed under ordinary reaction conditions. Hence, much of this chemistry is shrouded in mystery. This project aims to develop the ability to observe and monitor such reactions directly using a combination of spectroscopies at very low temperatures, where the molecules are more stable and reactions slower. These studies will give quantitative information on the nature of the reactive intermediates themselves, the nature of the products formed, and the reaction dynamics, and they are of fundamental importance for an understanding of chemical reactivity generally. The methodology developed will be applicable to the investigation of a wide range of processes.Read moreRead less
Investigation of novel sialic acid mimetics to target the spread of cancer. The mortality rates for many cancers afflicting the world's population are extremely high and these rates are consistent with the Australian experience. It is generally accepted that colon cancer, and cancers as a whole, are a significant healthcare issue and have immense socioeconomic impact. Alternative treatments preventing the spread of cancers would be of very significant benefit. This fellowship will provide the ....Investigation of novel sialic acid mimetics to target the spread of cancer. The mortality rates for many cancers afflicting the world's population are extremely high and these rates are consistent with the Australian experience. It is generally accepted that colon cancer, and cancers as a whole, are a significant healthcare issue and have immense socioeconomic impact. Alternative treatments preventing the spread of cancers would be of very significant benefit. This fellowship will provide the opportunity for the discovery and development of such treatments that are based on the processes that utilise carbohydrates to facilitate the spread of tumours.Read moreRead less
Modifying Structure and Properties of Carbon Nanotubes for Device Applications (MWN). The focus of this project is to develop new heteroatom-doped carbon nanotube materials for use in conjugated-polymer composite photovoltaic cells. Synthesis of boron and of nitrogen doped carbon nanotubes (CNTs) by the US researchers will be complemented by ion-implantation post-synthesis of CNTs by the Australian team, to gain a thorough and detailed understanding of how the CNTs can act effectively as both an ....Modifying Structure and Properties of Carbon Nanotubes for Device Applications (MWN). The focus of this project is to develop new heteroatom-doped carbon nanotube materials for use in conjugated-polymer composite photovoltaic cells. Synthesis of boron and of nitrogen doped carbon nanotubes (CNTs) by the US researchers will be complemented by ion-implantation post-synthesis of CNTs by the Australian team, to gain a thorough and detailed understanding of how the CNTs can act effectively as both an electron acceptor and charge transport medium in a conjugated polymer. Outcomes will include fundamental advances in our understanding of charge transport in the composite devices and prototype organic photovoltaic devices of improved efficiency.Read moreRead less
The investigation of the effects of catalyst doping, element substitution and defects design in carbon materials for hydrogen storage. The successful introduction of an efficient and clean hydrogen economy is contingent on developing a cost-effective storage technology. Carbon materials have demonstrated significant promise in this area. The project aims to investigate the storage capacity of hydrogen in carbon materials by doping catalysts, substituting elements and introducing designed defect ....The investigation of the effects of catalyst doping, element substitution and defects design in carbon materials for hydrogen storage. The successful introduction of an efficient and clean hydrogen economy is contingent on developing a cost-effective storage technology. Carbon materials have demonstrated significant promise in this area. The project aims to investigate the storage capacity of hydrogen in carbon materials by doping catalysts, substituting elements and introducing designed defects into the structures of carbon materials, with both theoretical and experimental methods. This project also aims to foster a long term linkage with the National Institute of Advanced Industrial Science and Technology, Japan thus enhancing Australian Universities's integration with the research institutions overseas in research and developmentRead moreRead less