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Selective photocatalytic lignin biomass conversion. If the prospective ‘hydrogen economy’ is to use hydrogen as a fuel and energy carrier to replace fossil sources, vast amounts of renewable cheap hydrogen must be available. A likely candidate is catalytic water splitting by sunlight. The hydrogen can be made affordable, by coupling hydrogen production to a higher value-added stream. The aim of this project is to produce a stable, hybrid heterogenous catalyst system able to oxidise organic subst ....Selective photocatalytic lignin biomass conversion. If the prospective ‘hydrogen economy’ is to use hydrogen as a fuel and energy carrier to replace fossil sources, vast amounts of renewable cheap hydrogen must be available. A likely candidate is catalytic water splitting by sunlight. The hydrogen can be made affordable, by coupling hydrogen production to a higher value-added stream. The aim of this project is to produce a stable, hybrid heterogenous catalyst system able to oxidise organic substrates derived from lignin biomass as an adjunct to visible light hydrogen generation from water. The significance will be to provide fuels and organic chemicals for industry from biomass, water and sunlight and catalytically remediate waste water with sunlight.Read moreRead less
Precision luminescent solar concentrators from robust quantum dot arrays. Precision luminescent solar concentrators from robust quantum dot arrays. This project aims to make luminescent solar concentrators that can harness solar energy from surfaces not suited for conventional solar cells, such as car windows. It will design, synthesise and conduct detailed energy transfer studies of robust inorganic quantum dot arrays with fit-for-purpose precise spectral properties. Synthetic light-harvesting ....Precision luminescent solar concentrators from robust quantum dot arrays. Precision luminescent solar concentrators from robust quantum dot arrays. This project aims to make luminescent solar concentrators that can harness solar energy from surfaces not suited for conventional solar cells, such as car windows. It will design, synthesise and conduct detailed energy transfer studies of robust inorganic quantum dot arrays with fit-for-purpose precise spectral properties. Synthetic light-harvesting dye arrays have often been proposed to solve bottleneck challenges in the solar energy sector but there are issues with stability, processing and their photophysical output matching market needs. This project’s dyes are expected to create market opportunities for Australian luminescent solar concentrator technology.Read moreRead less
Tuning the electrolytes for high efficiency solar splitting of water. This project will develop a new technology that uses ionic liquids and sunlight to split water into hydrogen and oxygen to be used as a clean fuel. Australia has abundant sunlight, is very close to the growing energy markets of the Asia-Pacific region, and is ideally placed to benefit from this new technology.
Interactions, phase behavior and self-assembly of colloidal nanorods: Establishing design rules for creating new nano-structured materials. This project aims to apply new computational methods developed by the applicant to characterise the interactions between colloidal nanorods and their self-assembly in the presence of interfaces and directional interactions. While nanoparticles can currently be made in a staggering array of shapes, patterns and materials, organising such objects into extended ....Interactions, phase behavior and self-assembly of colloidal nanorods: Establishing design rules for creating new nano-structured materials. This project aims to apply new computational methods developed by the applicant to characterise the interactions between colloidal nanorods and their self-assembly in the presence of interfaces and directional interactions. While nanoparticles can currently be made in a staggering array of shapes, patterns and materials, organising such objects into extended structures that could revolutionise technology remains a challenge. The expected outcome is a robust strategy for making monolayer films of rods aligned perpendicular to a variety of interfaces for the fabrication of solar cells, microfiltration membranes and biosensors.Read moreRead less
Faster interfacial electron transfer: the effect of molecule shape and size. This project aims to explore the effect of shape and size of pi-conjugated molecules on interfacial electron transfer reactions, which are fundamentally important in all applications of photo-electrochemical conversion and storage of energy. By making two series of pi-conjugated molecules and determining electron transfer rates using a combination of transient spectroscopies and computational chemistry, the project expe ....Faster interfacial electron transfer: the effect of molecule shape and size. This project aims to explore the effect of shape and size of pi-conjugated molecules on interfacial electron transfer reactions, which are fundamentally important in all applications of photo-electrochemical conversion and storage of energy. By making two series of pi-conjugated molecules and determining electron transfer rates using a combination of transient spectroscopies and computational chemistry, the project expects to generate new design principles for molecules with the potential to significantly improve the efficiencies of solar energy conversion and photo-catalytic processes. The new materials and findings will be exploited in a novel redox-mediated water splitting device as a practical outcome with potential end user benefits.Read moreRead less
Chemical physics for nanotechnology and biotechnology. Computational methods solving the motions of electrons and nuclei will be developed and applied to the science and technology of single-molecule devices. Applications include design of extremely dense memories, photosynthesis, design of a new type of solar cell, concepts in quantum computing, and high-quality protein structure determination.
Discovery Early Career Researcher Award - Grant ID: DE130100970
Funder
Australian Research Council
Funding Amount
$370,600.00
Summary
Solar energy conversion: illuminating the origin of long-lived charge-separated states in organic donor/acceptor blends. The origin of exceptionally long-lived charges in organic donor/acceptor solid-state blends will be established. This will substantially enhance the efficiency and commercial viability of applications that rely on these long-lived charge-separated states, such as organic solar cells.
Hot exciton dissociation in donor / acceptor organic solar cells: breaking the efficiency limit of organic photovoltaics. Australia will benefit from this project in several key areas with immediate impact. The development of an innovative solar cell architecture through the use of hot exiton dissociation will deliver a potential increase in the maximum achievable power conversion efficiency. The experimental results will significantly advance fundamental knowledge of organic solar cells. This ....Hot exciton dissociation in donor / acceptor organic solar cells: breaking the efficiency limit of organic photovoltaics. Australia will benefit from this project in several key areas with immediate impact. The development of an innovative solar cell architecture through the use of hot exiton dissociation will deliver a potential increase in the maximum achievable power conversion efficiency. The experimental results will significantly advance fundamental knowledge of organic solar cells. This has significant economic benefits by making these solar cells more affordable and also opening up the opportunity to use new materials unconstrained by existing proprietary interests. The training of personnel will contribute towards solving the biggest challenge facing the solar industry in Australia: lack of skilled personnel in a highly specialised industry.Read moreRead less
Nanostructured Upconvertors for Advanced Solar Energy Harvesting. The efficiency of many solar energy conversion processes, such as solar photovoltaic and solar hydrogen, can be improved by management of the solar spectrum. One photon management strategy is up-conversion, whereby two lower energy, unusable photons are conjoined to bring about a higher energy photon. Photochemical up-conversion, where light harvesting and energy-pooling is performed in organic molecules, has been rapidly advanced ....Nanostructured Upconvertors for Advanced Solar Energy Harvesting. The efficiency of many solar energy conversion processes, such as solar photovoltaic and solar hydrogen, can be improved by management of the solar spectrum. One photon management strategy is up-conversion, whereby two lower energy, unusable photons are conjoined to bring about a higher energy photon. Photochemical up-conversion, where light harvesting and energy-pooling is performed in organic molecules, has been rapidly advanced in recent years, and promises to deliver the efficiencies required to find real-world application. This project brings together laser spectroscopy, organic and materials chemistry and nanotechnology to realise efficient up-convertors which will be applied to solar cells and solar fuels.Read moreRead less
Porphyrin arrays - Light Harvesting in three dimensions. The emulation of photosynthesis, the efficient and sustainable utilization of solar energy using renewable materials represents one of the great scientific challenges. This project will explore one aspect of this by determining the nature and scope of using assemblies of artificial chlorophylls for three dimensional light harvesting in titania solar cells.