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Renewable solar hydrogen generated from waste streams. Sunlight is the largest available carbon-neutral energy source, with enough energy striking the planet in one hour to satisfy our current requirements for about a year. With the novel catalysts designed in this project, we will use this energy to simultaneously generate hydrogen and destroy organic pollutants by oxidation.
Adding hydride punch to transition metal complexes for CO2 electroreduction. This project plans to apply an innovative methodology to the selective conversion of carbon dioxide (CO2) waste into useful C1 chemicals. The new inorganic chemistry approach is based on the invention of transition metal–organic hydride coordination complexes, which are designed to punch hydride ion (= a proton and two electrons) into metal-activated CO2-derived intermediates. The approach should naturally overcome the ....Adding hydride punch to transition metal complexes for CO2 electroreduction. This project plans to apply an innovative methodology to the selective conversion of carbon dioxide (CO2) waste into useful C1 chemicals. The new inorganic chemistry approach is based on the invention of transition metal–organic hydride coordination complexes, which are designed to punch hydride ion (= a proton and two electrons) into metal-activated CO2-derived intermediates. The approach should naturally overcome the two-electron barrier found for today's best transition metal electrocatalysts of CO2 reduction and, hence, enable the selective production of formaldehyde, a four-electron reduction product and bulk industrial feedstock chemical, or methanol, a six-electron reduction product and future transport fuel.Read moreRead less
Biomimetic ligands for catalytic iron-mediated degradation of contaminants. This project aims to develop and apply ligands attached to solid supports that bind iron and which, on activation, form high valence state iron species capable of catalytically oxidising contaminants present in waters and wastewaters. Of particular interest in this work are ligands that are simple analogues of biological molecules and which are stable in the presence of the high valent iron species formed following activ ....Biomimetic ligands for catalytic iron-mediated degradation of contaminants. This project aims to develop and apply ligands attached to solid supports that bind iron and which, on activation, form high valence state iron species capable of catalytically oxidising contaminants present in waters and wastewaters. Of particular interest in this work are ligands that are simple analogues of biological molecules and which are stable in the presence of the high valent iron species formed following activation. The end result of this project is a water treatment process suited to the effective removal of trace contaminants such as hormones, pharmaceuticals and pesticides from wastewaters such that the treated waters are suitable for discharge to pristine environments or to reuse for potable purposes.Read moreRead less
Metal Directed Assembly of New Discrete and Framework Supramolecular Systems. An important aspect of this project is the development of strategies for assembling molecules and metals into larger units - leading to novel compounds and materials for which unusual and potentially useful properties can be anticipated. These may include materials that act as catalysts for chemical reactions or absorb and store gases (such as hydrogen for use as a fuel). More generally, the area is one that will under ....Metal Directed Assembly of New Discrete and Framework Supramolecular Systems. An important aspect of this project is the development of strategies for assembling molecules and metals into larger units - leading to novel compounds and materials for which unusual and potentially useful properties can be anticipated. These may include materials that act as catalysts for chemical reactions or absorb and store gases (such as hydrogen for use as a fuel). More generally, the area is one that will underpin the 'bottom-up' approach (building tiny components from individual molecules and ions) in the rapidly expanding field of nanotechnology. Clearly, if Australia is to remain internationally competitive in such new technologies then an understanding of processes of the type outlined in this proposal will be essential.Read moreRead less
Metal Directed Assembly of New Supramolecular Systems. An important aspect of this project is the development of strategies for assembling molecules and metals into larger units - leading to novel compounds and materials for which unusual and potentially useful properties can be anticipated. These may include materials that act as catalysts for chemical reactions or absorb and store gases (such as hydrogen for use as a fuel). More generally, the area is one that will underpin the 'bottom-up' ap ....Metal Directed Assembly of New Supramolecular Systems. An important aspect of this project is the development of strategies for assembling molecules and metals into larger units - leading to novel compounds and materials for which unusual and potentially useful properties can be anticipated. These may include materials that act as catalysts for chemical reactions or absorb and store gases (such as hydrogen for use as a fuel). More generally, the area is one that will underpin the 'bottom-up' approach (building tiny components from individual molecules and ions) in the rapidly expanding field of nanotechnology. Clearly, if Australia is to remain internationally competitive in such new technologies then an understanding of processes of the type outlined in this proposal will be essential.Read moreRead less
Nanoscale Molecular Architectures - New Metallo Cages and Capsules. The design and synthesis of novel cage and capsule-like supermolecular structures will be undertaken, including rare examples of two large cage types - one designed to incorporate two adjacent metal ions in an extended (chiral) cavity while the other utilises macrocyclic metal complexes as the 'walls' of the cage. In the latter case metal variation makes possible the alteration of the electronic environment of a guest occupying ....Nanoscale Molecular Architectures - New Metallo Cages and Capsules. The design and synthesis of novel cage and capsule-like supermolecular structures will be undertaken, including rare examples of two large cage types - one designed to incorporate two adjacent metal ions in an extended (chiral) cavity while the other utilises macrocyclic metal complexes as the 'walls' of the cage. In the latter case metal variation makes possible the alteration of the electronic environment of a guest occupying the central cavity . A third (capsule-like) system is designed to 'open' and 'close' under pH control. The present studies hold promise for underpinning the future development of nano-scale molecular devices.
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Metal Directed Assembly of New Supramolecular Systems. This project is concerned with the use of designed metal-ion directed assembly for the construction of new supramolecular entities incorporating metal complexes as structural elements. A range of novel nanometre-scale architectures is planned, including supramolecular ellipses, squares, cubes and mechanically linked systems. The proposed research has implications for elucidating fundamental aspects of both supramolecular and metal complexati ....Metal Directed Assembly of New Supramolecular Systems. This project is concerned with the use of designed metal-ion directed assembly for the construction of new supramolecular entities incorporating metal complexes as structural elements. A range of novel nanometre-scale architectures is planned, including supramolecular ellipses, squares, cubes and mechanically linked systems. The proposed research has implications for elucidating fundamental aspects of both supramolecular and metal complexation behaviour. It also holds promise for the production of novel materials for which unusual and potentially useful properties can be anticipated.Read moreRead less
DNA Nanoshuttles: A New Class of DNA-Binding Molecules. The interaction of molecules with DNA, the molecule that controls genetic information, is fundamental to drug design, diagnosis of disease and the environment. DNA-nanoshuttles are ring-shaped molecules that thread onto DNA and shuttle from one end to the other. This threading interaction is without precedent and hence DNA-nanoshuttles have significant potential applications in all areas of medicine, biotechnology and nanotechnology that in ....DNA Nanoshuttles: A New Class of DNA-Binding Molecules. The interaction of molecules with DNA, the molecule that controls genetic information, is fundamental to drug design, diagnosis of disease and the environment. DNA-nanoshuttles are ring-shaped molecules that thread onto DNA and shuttle from one end to the other. This threading interaction is without precedent and hence DNA-nanoshuttles have significant potential applications in all areas of medicine, biotechnology and nanotechnology that involve DNA interactions. This research may lead to the design of new diagnostics and applications that will benefit the Australian community, and will provide excellent training of researchers in skills required for employment in the biotechnology and pharmaceutical fields.Read moreRead less
Ditopic receptors for the cooperative binding of cations and anions. This project is concerned with the design, synthesis and investigation of new receptor molecules that are capable of simultaneously binding metal cations and anions in a cooperative fashion. The new systems are based on a macrocyclic platform which acts as the metal binding site together with side-arms incorporating functional groups that are designed to cooperatively interact with a suitable anion. Potential applications exist ....Ditopic receptors for the cooperative binding of cations and anions. This project is concerned with the design, synthesis and investigation of new receptor molecules that are capable of simultaneously binding metal cations and anions in a cooperative fashion. The new systems are based on a macrocyclic platform which acts as the metal binding site together with side-arms incorporating functional groups that are designed to cooperatively interact with a suitable anion. Potential applications exist for this category of ditopic receptors in mineral processing where the ability to extract a metal as its metal salt may lead to more efficient solvent extraction processes.Read moreRead less
Electrode-Supported Ionogels for Reversible Energy Storage. The project aims to generate an understanding of electrode-supported ionic liquid gel films to form the basis for the rational design and development of new energy storage technology. For the world to truly move into a new age of low carbon power, it needs transformational battery technology. The creation of novel ionic liquid systems to capture redox-active species would allow for revolutionary designs with the potential to eliminate m ....Electrode-Supported Ionogels for Reversible Energy Storage. The project aims to generate an understanding of electrode-supported ionic liquid gel films to form the basis for the rational design and development of new energy storage technology. For the world to truly move into a new age of low carbon power, it needs transformational battery technology. The creation of novel ionic liquid systems to capture redox-active species would allow for revolutionary designs with the potential to eliminate membranes, with major advantages for charging/discharging speed and deep cyclability. This would directly translate to storage systems that combine high power with high energy density.Read moreRead less