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New metal-molecule binding motifs for self-assembled monolayers and nanodevices. The goal of this research is to investigate technologically interesting electronic materials using new molecular assemblies. We explore their application in some fundamental components of molecular electronic systems and anticipate that knowledge gained from our investigations will have significant impact on the field of nanotechnology, especially in the area of molecular electronics. Our basic research will contrib ....New metal-molecule binding motifs for self-assembled monolayers and nanodevices. The goal of this research is to investigate technologically interesting electronic materials using new molecular assemblies. We explore their application in some fundamental components of molecular electronic systems and anticipate that knowledge gained from our investigations will have significant impact on the field of nanotechnology, especially in the area of molecular electronics. Our basic research will contribute to Australia's reputation as a source of innovative research and ideas in an area where there is growing international momentum.Read moreRead less
Repulsive van der Waals forces and Brownian ratchet motors: manipulating thermal and quantum Fluctuations. A fundamental problem with miniaturizing machines and mechanical devices below the micron scale is the issue of friction and lubrication. One way to completely circumvent the need for lubrication is to use a little-studied phenomenon known as 'repulsive van der Waals forces', to create materials that fundamentally repel each other in certain fluid environments. This effect is very large at ....Repulsive van der Waals forces and Brownian ratchet motors: manipulating thermal and quantum Fluctuations. A fundamental problem with miniaturizing machines and mechanical devices below the micron scale is the issue of friction and lubrication. One way to completely circumvent the need for lubrication is to use a little-studied phenomenon known as 'repulsive van der Waals forces', to create materials that fundamentally repel each other in certain fluid environments. This effect is very large at the nanoscale and this proposal examines how such forces can be used to make 'lubricant free' motors and nanomachines. This will open up the possibility of building small and portable sensors, actuators, microfluidic devices and eventually active drug delivery systems for health applications.Read moreRead less
Targeted process development for drug delivery. Matrix assisted ball milling and continuous flow process intensification on rotating surfaces in the form of spinning discs and rotating tubes, and combinations of these, allow the fabrication of nanoparticles for the pharmaceutical industry, with the ability to fine tune the properties of the particles to improve their uptake profiles, while minimising side effects. The research will be conducted through the Centre for Strategic Nano-Fabrication w ....Targeted process development for drug delivery. Matrix assisted ball milling and continuous flow process intensification on rotating surfaces in the form of spinning discs and rotating tubes, and combinations of these, allow the fabrication of nanoparticles for the pharmaceutical industry, with the ability to fine tune the properties of the particles to improve their uptake profiles, while minimising side effects. The research will be conducted through the Centre for Strategic Nano-Fabrication with its science based attention to quality by design for product development at the inception of the science. This, coupled with the involvement of iCeutica which has a strong commercially focused R and D profile, provides a more innovative research culture, and excellent research training. Read moreRead less
Self-Organised 3-D Arrays of Stimulus Responsive Block Copolymer Micelles. At the core of developments in nanotechnology is a desire to manufacture functional devices from molecular or colloidal building blocks. A significant component of this effort is directed at the self-assembly of these materials on solid substrates. Ultimately, the development of higher order functional nanomaterials requires a fine control over the 3-dimensional location of each component; this is a significant problem. I ....Self-Organised 3-D Arrays of Stimulus Responsive Block Copolymer Micelles. At the core of developments in nanotechnology is a desire to manufacture functional devices from molecular or colloidal building blocks. A significant component of this effort is directed at the self-assembly of these materials on solid substrates. Ultimately, the development of higher order functional nanomaterials requires a fine control over the 3-dimensional location of each component; this is a significant problem. In this project our aim is to develop novel self-assembled surface coatings using block copolymer micelles. Spatial control of the micelle adsorption at the solid-aqueous interface will give us a significant degree of control over molecular location in 3-dimensions.Read moreRead less
An in-built depolymerisation solution for polyethylene waste. This project aims to design enzymes that can be embedded into polyethylene, and later activated by the elevated temperatures of a compost heap, to depolymerise the plastic to small molecules. There are no good options available for the controlled decomposition of polyethylene waste at present, and instead researchers have focussed on solutions that rely on modifications to the underlying chemistry of the backbone and or collection to ....An in-built depolymerisation solution for polyethylene waste. This project aims to design enzymes that can be embedded into polyethylene, and later activated by the elevated temperatures of a compost heap, to depolymerise the plastic to small molecules. There are no good options available for the controlled decomposition of polyethylene waste at present, and instead researchers have focussed on solutions that rely on modifications to the underlying chemistry of the backbone and or collection to a central facility. Our approach would result in an in-built decomposition that does not require collection and recycling in a central facility. Since it is based on a depolymerisation mechanism it does not result in the production of harmful, partially disintegrated microplastics.Read moreRead less
Electronic and Optical Properties of Doped Titanium Dioxide. Titanium dioxide, is widely used as a white pigment, owing to its high refractive index, second, only after diamond. Yellowing of rutile pigment particles, observed on prolonged exposure to sunlight, is a serious problem that pigment manufacturers would like to overcome. It is proposed that aluminium-doping of rutile limits this discolouration by altering the electronic structure of the rutile particles. This project seeks to identify ....Electronic and Optical Properties of Doped Titanium Dioxide. Titanium dioxide, is widely used as a white pigment, owing to its high refractive index, second, only after diamond. Yellowing of rutile pigment particles, observed on prolonged exposure to sunlight, is a serious problem that pigment manufacturers would like to overcome. It is proposed that aluminium-doping of rutile limits this discolouration by altering the electronic structure of the rutile particles. This project seeks to identify the specific electronic cause of the yellowing process, the nature of the Al defect,it's effect on the electronic structure of rutile, and the electronic perturbations that may occur when other dopants are used.Read moreRead less
Enhanced pigment weathering resistance by coating with high dielectric ceramic. The partner company, Tiwest, based in Western Australia, is a major contributor to the economy, and earns more than $A400m annually in exports. It is the only company in the world that mines, separates, refines and manufactures titania products, including pigments, in one region. The current post-titania particle formation wet-coating process, however, presents a major capital and recurrent cost and necessitates a pi ....Enhanced pigment weathering resistance by coating with high dielectric ceramic. The partner company, Tiwest, based in Western Australia, is a major contributor to the economy, and earns more than $A400m annually in exports. It is the only company in the world that mines, separates, refines and manufactures titania products, including pigments, in one region. The current post-titania particle formation wet-coating process, however, presents a major capital and recurrent cost and necessitates a pigment regrind stage. The research will investigate the development of a highly durable dry-coated pigment utilising a novel high dielectric coating. This development has the potential to ensure the partner company's future competitiveness through reduced processing costs and improved product performance.Read moreRead less
Preparation of nanostructured surfaces by electrochemical deposition through lyotropic liquid-crystal templates. Hexagonal-phase lyotropic liquid crystals may be used as templates to deposit metals on electrodes. The sizes of the structures made by this method are a few nanometres. We propose to exploit both the aqueous and non-aqueous parts of the liquid crystal to deposit different metals, polymers or metals and polymers. Thin metal wires (nano-wires) sheathed in polymer will be the thinnest i ....Preparation of nanostructured surfaces by electrochemical deposition through lyotropic liquid-crystal templates. Hexagonal-phase lyotropic liquid crystals may be used as templates to deposit metals on electrodes. The sizes of the structures made by this method are a few nanometres. We propose to exploit both the aqueous and non-aqueous parts of the liquid crystal to deposit different metals, polymers or metals and polymers. Thin metal wires (nano-wires) sheathed in polymer will be the thinnest insulated wires ever made. Carbon nanotubes will also be aligned in the hexagonal hole in the template allowing exploitation of these unique species. The structures that will be fabricated will be candidates for catalysts, sensor arrays and electronic devices.Read moreRead less
The Interface of Oil-in-Water Emulsions. The interface between two immiscible liquids controls many phenomena including the formation and properties of emulsions, the nature of many chemical separation processes and the behaviour of biological systems. There are few methods to study such interfaces and most of these are susceptible to trace contamination by adventitious surfactants, but emulsions with their large surface area avoid this problem. Significant advances are possible with the new Aus ....The Interface of Oil-in-Water Emulsions. The interface between two immiscible liquids controls many phenomena including the formation and properties of emulsions, the nature of many chemical separation processes and the behaviour of biological systems. There are few methods to study such interfaces and most of these are susceptible to trace contamination by adventitious surfactants, but emulsions with their large surface area avoid this problem. Significant advances are possible with the new Australian technique of electroacoustics, complemented by neutron scattering, nmr, rheological and dielectric response measurements on concentrated emulsions. Our surfactant-free emulsions provide a fundamental breakthrough in such studies, leading to new materials from nanostructures.Read moreRead less