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Discovery Early Career Researcher Award - Grant ID: DE210101102
Funder
Australian Research Council
Funding Amount
$404,748.00
Summary
Single-Atom Catalysts on Atomically Thin Nanomaterials for H2O2 Production. Single-atomic sites supported on graphene analogs is an ideal structural mode for the design of electrocatalysts due to its ultimate small size limit, atomic thickness, and easily tuned electronic properties. This project aims to use a theory-guided approach to develop efficient electrocatalysts for the production of value-added hydrogen peroxide. The structural advantages of graphene analogs will be fully utilised to un ....Single-Atom Catalysts on Atomically Thin Nanomaterials for H2O2 Production. Single-atomic sites supported on graphene analogs is an ideal structural mode for the design of electrocatalysts due to its ultimate small size limit, atomic thickness, and easily tuned electronic properties. This project aims to use a theory-guided approach to develop efficient electrocatalysts for the production of value-added hydrogen peroxide. The structural advantages of graphene analogs will be fully utilised to unlock the catalytic power of single-atomic sites, and consequently achieve high catalytic activity and selectivity. The outcome will set a solid scientific foundation to enable economically viable technologies for eco-friendly hydrogen peroxide production and bring significant socioeconomic benefits to Australia.Read moreRead less
Tuning catalyst reaction environments towards photoreforming of wastewater. This project aims to combine high-throughput computation and machine learning to screen photocatalysts more thoroughly for photoreforming of wastewater. The reaction environments effects on surface active units will be tailored for COx-emission-free selective organic synthesis with hydrogen production from organic-contained wastewater at ambient conditions. The project expects to expand our knowledge on the fast, reliabl ....Tuning catalyst reaction environments towards photoreforming of wastewater. This project aims to combine high-throughput computation and machine learning to screen photocatalysts more thoroughly for photoreforming of wastewater. The reaction environments effects on surface active units will be tailored for COx-emission-free selective organic synthesis with hydrogen production from organic-contained wastewater at ambient conditions. The project expects to expand our knowledge on the fast, reliable screening strategies, and the relationship between electric field (or lattice strain) and reaction pathways. This project will develop a photoreforming system for selective co-production of organics and hydrogen from wastewater, benefiting sustainable technologies development for chemical synthesis and hydrogen economy.Read moreRead less
Atomically Thin 3d Transition Metal Electrocatalysts for Water Splitting. The current industrial-scale hydrogen productions are reliant on high temperature steam reforming fossil fuels, consuming large quantity of energy and fossil resources, and emitting huge amounts of CO2. This project aims to develop cheap and plentiful transition metal-based high performance water splitting electrocatalysts, enabling economically viable large-scale water electrolytic hydrogen production driven by renewable ....Atomically Thin 3d Transition Metal Electrocatalysts for Water Splitting. The current industrial-scale hydrogen productions are reliant on high temperature steam reforming fossil fuels, consuming large quantity of energy and fossil resources, and emitting huge amounts of CO2. This project aims to develop cheap and plentiful transition metal-based high performance water splitting electrocatalysts, enabling economically viable large-scale water electrolytic hydrogen production driven by renewable electricity. A theory-guided catalyst approach will be used to guide the efficient design and development of high performance electrocatalysts. The success of the project will lead to a suit of high performance water splitting electrocatalysts, leaping forward water electrolytic hydrogen production technology.Read moreRead less
Charging transition metals with activating alkanes. The project aims to engineer positively charged metal complexes and use them to explore the chemistry of bound activated alkane ligands. The transformation of cheap, plentiful alkanes into more valuable products is a major quest in chemistry, and complexes of alkanes bound to metals are expected to play a key role in transformations of alkanes. The project intends to use the activated metal bound alkane to transform the normally inert alkane in ....Charging transition metals with activating alkanes. The project aims to engineer positively charged metal complexes and use them to explore the chemistry of bound activated alkane ligands. The transformation of cheap, plentiful alkanes into more valuable products is a major quest in chemistry, and complexes of alkanes bound to metals are expected to play a key role in transformations of alkanes. The project intends to use the activated metal bound alkane to transform the normally inert alkane into compounds with desirable functional groups. This should make the synthesis of alkane complexes stable at room temperature in solution a realistic possibility. These cheap, plentiful alkanes can be turned into more valuable products, bringing benefits to industry.Read moreRead less
Alkane transformations through binding to metals. Alkanes are fully saturated hydrocarbons and they are the major components of petroleum, including natural gas and liquid hydrocarbon fuels. They are abundant but finite, and their primary usage has been as fuels since they burn readily and release energy. Alkanes are relatively low-value, high-volume chemical feedstocks which are not easy to convert into more useful value-added materials. This project focuses on developing positively charged met ....Alkane transformations through binding to metals. Alkanes are fully saturated hydrocarbons and they are the major components of petroleum, including natural gas and liquid hydrocarbon fuels. They are abundant but finite, and their primary usage has been as fuels since they burn readily and release energy. Alkanes are relatively low-value, high-volume chemical feedstocks which are not easy to convert into more useful value-added materials. This project focuses on developing positively charged metal-based compounds that can bind directly to alkanes to increase their reactivity and enable their transformation into higher value products such as alcohols and olefins which are important chemical feedstocks.Read moreRead less
Plasmonic nanoparticle catalysis for nitrogen-based synthesis. Light can generate an optical force to capture small objects. This requires intense light – a laser, which limits optical trapping in catalysis applications. This project aims to apply plasmonic nanoparticles with normal-intensity light to take advantage of plasmonic-generated optical forces for catalytic chemical synthesis. The optical trapping/releasing of small molecules is highly selective and responsive to molecule structure and ....Plasmonic nanoparticle catalysis for nitrogen-based synthesis. Light can generate an optical force to capture small objects. This requires intense light – a laser, which limits optical trapping in catalysis applications. This project aims to apply plasmonic nanoparticles with normal-intensity light to take advantage of plasmonic-generated optical forces for catalytic chemical synthesis. The optical trapping/releasing of small molecules is highly selective and responsive to molecule structure and so presents a great opportunity to radically alter chemical synthesis pathways, which will be illustrated with reactions on liquid-solid and gas-solid interfaces. This highly innovative strategy will be used to discover new nitrogen-based syntheses which are both fundamentally and industrially important.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE230100021
Funder
Australian Research Council
Funding Amount
$440,154.00
Summary
Kesterite/Si Tandem Structure for Unassisted Overall Solar Fuel Production. This project aims to develop Kesterite/Si tandem device for photoelectrochemical carbon dioxide reduction to produce solar fuels. It is expected to reveal the photoelectrochemical mechanism of the p-n heterojunction, thereby promoting solar energy utilisation and greenhouse gas reduction. Expected outcomes include delivery of a high-performance kesterite photocathode for efficient CO2 reduction, a kesterite/Si tandem dev ....Kesterite/Si Tandem Structure for Unassisted Overall Solar Fuel Production. This project aims to develop Kesterite/Si tandem device for photoelectrochemical carbon dioxide reduction to produce solar fuels. It is expected to reveal the photoelectrochemical mechanism of the p-n heterojunction, thereby promoting solar energy utilisation and greenhouse gas reduction. Expected outcomes include delivery of a high-performance kesterite photocathode for efficient CO2 reduction, a kesterite/Si tandem device for overall unassisted solar fuel production, and an in-depth understanding of structure-performance correlation to guide future heterojunction photocathode design. This project should provide significant benefits in minimising fossil fuel consumption, increasing energy security, and expanding the clean energy industry.Read moreRead less
High-productivity ammonia electrosynthesis. The aim of this project is to develop and demonstrate high-performance devices for ammonia production from renewables by a scalable electrolysis method. This will be achieved by experimental and modelling investigations of the nitrogen reduction reaction to guide the design of tailor-made cathodes. New knowledge in catalysis and materials science is expected to be generated. The target outcome of the project is a sustainable and affordable ammonia synt ....High-productivity ammonia electrosynthesis. The aim of this project is to develop and demonstrate high-performance devices for ammonia production from renewables by a scalable electrolysis method. This will be achieved by experimental and modelling investigations of the nitrogen reduction reaction to guide the design of tailor-made cathodes. New knowledge in catalysis and materials science is expected to be generated. The target outcome of the project is a sustainable and affordable ammonia synthesis method as an alternative to the current fossil-fuels-based and excessively greenhouse-emitting process. The technology to be developed in this project is anticipated to be of significant benefit to the Australian agriculture sector as a local, on-demand source of low-cost fertilisers.Read moreRead less
A Midas touch for electrophiles in new reaction development. This project aims to address the lack of knowledge about how high-value organic molecules are formed in gold-catalysed reactions by advancing a novel mode of catalysis. This project expects to generate new knowledge about these gold-catalysed reactions using an innovative, interdisciplinary approach incorporating computational and synthetic techniques. Expected outcomes of this project include the optimisation and development of import ....A Midas touch for electrophiles in new reaction development. This project aims to address the lack of knowledge about how high-value organic molecules are formed in gold-catalysed reactions by advancing a novel mode of catalysis. This project expects to generate new knowledge about these gold-catalysed reactions using an innovative, interdisciplinary approach incorporating computational and synthetic techniques. Expected outcomes of this project include the optimisation and development of important organic reactions and enhancing collaboration nationally and internationally between computational and synthetic chemists. This should provide significant benefits in the form of improved chemical reactions for chemists to prepare new pharmaceuticals, agrochemicals and materials.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE230100978
Funder
Australian Research Council
Funding Amount
$406,818.00
Summary
A new Iron Age! Making Iron complexes fit for C-C cross-coupling catalysis. This project aims to develop new iron catalysts as alternatives to the expensive and increasingly rare noble metals currently used in C-C bond forming reactions, the most important single-step in the fine-chemicals sector.
This project expects to create a flexible yet robust framework by introducing a hemilabile ligand into the backbone of the iron complex to control the number of vacant coordination sites.
Expected outc ....A new Iron Age! Making Iron complexes fit for C-C cross-coupling catalysis. This project aims to develop new iron catalysts as alternatives to the expensive and increasingly rare noble metals currently used in C-C bond forming reactions, the most important single-step in the fine-chemicals sector.
This project expects to create a flexible yet robust framework by introducing a hemilabile ligand into the backbone of the iron complex to control the number of vacant coordination sites.
Expected outcomes of this project are 1) iron complexes able to catalyse biaryl couplings from sustainable substrates and 2) knowledge on structure-property relationships of iron-based catalytic processes.
Australia will benefit by applying its own resources and help preserving the valuable noble metals for processes relying on them.Read moreRead less