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Sulfur-based materials for infrared optics and thermal imaging. This project aims to investigate novel sulfur polymers for use in infrared optics and thermal imaging. Current thermal imaging lenses are made in energy-intensive processes from expensive semiconductors and toxic chalcogenide glasses. In contrast, highly abundant elemental sulfur can be converted into polymers that are highly transparent to mid- and long-wave infrared light, providing a promising low-cost alternative. In developing ....Sulfur-based materials for infrared optics and thermal imaging. This project aims to investigate novel sulfur polymers for use in infrared optics and thermal imaging. Current thermal imaging lenses are made in energy-intensive processes from expensive semiconductors and toxic chalcogenide glasses. In contrast, highly abundant elemental sulfur can be converted into polymers that are highly transparent to mid- and long-wave infrared light, providing a promising low-cost alternative. In developing this technology, expected outcomes include novel methods to manufacture polymers from low-cost sulfur and their use as lenses for thermal imaging. Significant benefits are expected, such as access to low-cost, recyclable materials for thermal imaging required in surveillance, diagnostics, and spectroscopy.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE240100502
Funder
Australian Research Council
Funding Amount
$424,875.00
Summary
Building Molecular Complexity Through Enzyme-Enabled Synthesis. Many valuable natural molecules are too complex to be commercially synthesised by current technologies. Despite advances in synthetic chemistry there is great need to adopt the elegant biocatalytic strategies for complex molecule synthesis found in nature, employing sophisticated enzyme catalysts. This interdisciplinary research program aims to address the shortcomings of traditional synthetic methods through the development of enzy ....Building Molecular Complexity Through Enzyme-Enabled Synthesis. Many valuable natural molecules are too complex to be commercially synthesised by current technologies. Despite advances in synthetic chemistry there is great need to adopt the elegant biocatalytic strategies for complex molecule synthesis found in nature, employing sophisticated enzyme catalysts. This interdisciplinary research program aims to address the shortcomings of traditional synthetic methods through the development of enzyme catalysts to rapidly generate complex molecular structures. These novel molecules can be readily converted into pharmaceuticals and agrochemicals leading to advancements in the bio-enabled production and application of organic molecules in these vital fields. Read moreRead less
Site-specific protein functionalisation at diselenides via photocatalysis . This project aims to develop a new photocatalytic reaction for the on demand functionalisation of proteins. The synthetic methodology will solve a major technological gap in the field by enabling efficient access to proteins with defined modifications at specific locations. Functionalised proteins generated in the project will underpin a detailed understanding of how specific modifications influence the structure and fun ....Site-specific protein functionalisation at diselenides via photocatalysis . This project aims to develop a new photocatalytic reaction for the on demand functionalisation of proteins. The synthetic methodology will solve a major technological gap in the field by enabling efficient access to proteins with defined modifications at specific locations. Functionalised proteins generated in the project will underpin a detailed understanding of how specific modifications influence the structure and function of several important proteins. The project will generate significant new knowledge in the fields of chemistry and biology and will foster interdisciplinary collaboration, nationally and internationally. The breakthrough technology also has the potential to benefit Australia’s biotechnology sector.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE230100634
Funder
Australian Research Council
Funding Amount
$410,140.00
Summary
Phos-Ligation: A powerful new tool for chemoselective protein modification. The project aims to develop a powerful new method for the generation of pure modified proteins. Tools for modification of proteins are integral to the study of protein structure and function as well as the commercial production of biopharmaceuticals. The extremely cost effective and operationally simple chemistry that will be developed in this project will overcome a number of pitfalls of currently available methods for ....Phos-Ligation: A powerful new tool for chemoselective protein modification. The project aims to develop a powerful new method for the generation of pure modified proteins. Tools for modification of proteins are integral to the study of protein structure and function as well as the commercial production of biopharmaceuticals. The extremely cost effective and operationally simple chemistry that will be developed in this project will overcome a number of pitfalls of currently available methods for protein modification, and will therefore deliver substantial technological innovation to both academia and industry. Through domestic and international collaboration, this new technology will be applied to study proteins involved in the defence of wheat against fungal rust disease and in inflammatory signalling in humans.Read moreRead less
Data Driven Discovery of New Catalysts for Asymmetric Synthesis. This project aims to discover new catalytic strategies for the synthesis of valuable nitrogen-containing molecules. An innovative approach combining statistical modelling techniques and chemical synthesis tactics will be used to establish a unique platform for predictable catalyst design that significantly accelerates the discovery process. As a result, new organometallic catalysts that efficiently convert simple and readily access ....Data Driven Discovery of New Catalysts for Asymmetric Synthesis. This project aims to discover new catalytic strategies for the synthesis of valuable nitrogen-containing molecules. An innovative approach combining statistical modelling techniques and chemical synthesis tactics will be used to establish a unique platform for predictable catalyst design that significantly accelerates the discovery process. As a result, new organometallic catalysts that efficiently convert simple and readily accessible chemical building blocks into complex chiral amine derivatives in a safer and more cost effective manner will be identified. These new catalytic strategies will be of significant utility, enabling the invention and more sustainable manufacture of agrochemicals, life-saving medicines, and functional materials.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE240100449
Funder
Australian Research Council
Funding Amount
$426,600.00
Summary
Diversity Oriented Clicking - Streamlined Synthesis of Molecular Frameworks. Innovation in synthetic chemistry drives the discovery of new life-changing drugs, agrochemicals and functional materials. This project aims to use a novel chemical concept, termed Diversity Oriented Clicking, for new sustainable and streamlined synthetic transformations. The new chemical processes are expected to deliver improved economy, efficiency and precision in the synthesis of bioactive molecules and functional m ....Diversity Oriented Clicking - Streamlined Synthesis of Molecular Frameworks. Innovation in synthetic chemistry drives the discovery of new life-changing drugs, agrochemicals and functional materials. This project aims to use a novel chemical concept, termed Diversity Oriented Clicking, for new sustainable and streamlined synthetic transformations. The new chemical processes are expected to deliver improved economy, efficiency and precision in the synthesis of bioactive molecules and functional materials that are inaccessible or challenging to prepare with existing technologies. The conceptual and practical outcomes of this project are expected to benefit both academia and industry as the synthetic routes to diverse complex molecules can be greatly streamlined, and reducing chemical waste and required purification.Read moreRead less
Advances in Peptide Synthesis: Exploiting Underutilised Functional Groups. The translation of therapeutically-relevant classes of peptides to the clinic is often limited by chemists' ability to synthesise these complex biomolecules efficiently and sustainably. This project aims to develop new tools for the preparation of designer peptides that are broadly inspired by an underutilised reactive group found in naturally-occurring peptide sequences. Expected outcomes encompass health and economic be ....Advances in Peptide Synthesis: Exploiting Underutilised Functional Groups. The translation of therapeutically-relevant classes of peptides to the clinic is often limited by chemists' ability to synthesise these complex biomolecules efficiently and sustainably. This project aims to develop new tools for the preparation of designer peptides that are broadly inspired by an underutilised reactive group found in naturally-occurring peptide sequences. Expected outcomes encompass health and economic benefits for the Australian community, including: the first approach to a class of promising antibiotic peptide natural product analogues, the development of a mild electrochemical approach to peptide modification, and the production of a library of novel amino acids for incorporation into potential antibiotic leads.Read moreRead less
New Horizons in Quinonedimethide Chemistry. Quinonedimethides (QDMs) are organic molecules with a notorious reputation for instability, hence they are poorly understood and an underexploited resource. This project will unite the ideally suited computational and experimental skills of the CIs to perform the first thorough investigation into fundamental QDM chemistry. It aims to map structure-reactivity in QDMs, investigate their ability to rapidly generate complex structures, and demonstrate thei ....New Horizons in Quinonedimethide Chemistry. Quinonedimethides (QDMs) are organic molecules with a notorious reputation for instability, hence they are poorly understood and an underexploited resource. This project will unite the ideally suited computational and experimental skills of the CIs to perform the first thorough investigation into fundamental QDM chemistry. It aims to map structure-reactivity in QDMs, investigate their ability to rapidly generate complex structures, and demonstrate their potential in spintronics and other applications. Anticipated outcomes include powerful and general new synthetic concepts, methods, strategies and tactics. This should provide significant benefits, such as better ways to manufacture important medicines and other materials.Read moreRead less
AI Assisted Continuous Flow Electrochemistry for Pharmaceutical Manufacture. This project aims to develop new chemical manufacturing processes for pharmaceutical products. In collaboration with Sun Pharma, it will tackle the challenge of replacing expensive and toxic chemicals in industrial reactions, to lower cost of manufacturing and improve its sustainability profile. Central to the realisation of this ambition is the use of electrocatalysis, machine learning and implementation of advanced co ....AI Assisted Continuous Flow Electrochemistry for Pharmaceutical Manufacture. This project aims to develop new chemical manufacturing processes for pharmaceutical products. In collaboration with Sun Pharma, it will tackle the challenge of replacing expensive and toxic chemicals in industrial reactions, to lower cost of manufacturing and improve its sustainability profile. Central to the realisation of this ambition is the use of electrocatalysis, machine learning and implementation of advanced continuous flow methods. These electricity- and technology-driven reactions will develop new strategies for the generation of important classes of molecules relevant to the Australia’s pharmaceutical sector, as well as their manufacture at industrially relevant scales.Read moreRead less
Unusual trisulfide chemistry. This project aims to investigate the mechanism of an unexpected reaction of trisulfides with common amide-containing solvents. Specifically, these solvents (such as dimethylformamide) were discovered to cleave S-S bonds in trisulfides and related polysulfides. This project expects to generate new knowledge in the understanding of the reaction mechanism and then use that understanding for useful chemistry. Expected outcomes of this project include a mechanistic under ....Unusual trisulfide chemistry. This project aims to investigate the mechanism of an unexpected reaction of trisulfides with common amide-containing solvents. Specifically, these solvents (such as dimethylformamide) were discovered to cleave S-S bonds in trisulfides and related polysulfides. This project expects to generate new knowledge in the understanding of the reaction mechanism and then use that understanding for useful chemistry. Expected outcomes of this project include a mechanistic understanding of a new reaction, and the use of this chemistry in polymer synthesis and polymer recycling. This project should provide significant benefits in new knowledge, as well as support new strategies in polymer synthesis and recycling to benefit the environment.Read moreRead less