Discovery Early Career Researcher Award - Grant ID: DE200100477
Funder
Australian Research Council
Funding Amount
$420,770.00
Summary
Developing sustainable liquid fuels from carbon dioxide conversion. This project aims to develop new electrochemical materials and systems capable of converting carbon dioxide to liquid fuels. It expects to generate new knowledge in the area of advanced materials and systems for sustainable fuel production by interdisciplinary integration of catalyst design, real-time characterisation and system engineering. Expected outcomes include electrochemical carbon dioxide-to-alcohol systems with commerc ....Developing sustainable liquid fuels from carbon dioxide conversion. This project aims to develop new electrochemical materials and systems capable of converting carbon dioxide to liquid fuels. It expects to generate new knowledge in the area of advanced materials and systems for sustainable fuel production by interdisciplinary integration of catalyst design, real-time characterisation and system engineering. Expected outcomes include electrochemical carbon dioxide-to-alcohol systems with commercially relevant performances and in-depth understanding of reaction mechanisms at nano and molecular levels. Significant economic, energy and environmental benefits are expected from the concerted greenhouse gas emissions reduction and the development of sustainable, clean, non-fossil fuels, enabled by this project.Read moreRead less
Ambient Electrochemical C-N Coupling via Co-electrolysis of N2 and CO2. To overcome the hurdles in N2 fixation (massive energy consumption and CO2 emission), investigators creatively hypothesize that the simultaneous electrocatalytic coupling of N2 and CO2 would enable the selective formation of N-products and thus realize their conversion into N--fertilizers and acetamides. Based on the CI's recent discoveries, this project will develop an innovative / sustainable system, which could promote th ....Ambient Electrochemical C-N Coupling via Co-electrolysis of N2 and CO2. To overcome the hurdles in N2 fixation (massive energy consumption and CO2 emission), investigators creatively hypothesize that the simultaneous electrocatalytic coupling of N2 and CO2 would enable the selective formation of N-products and thus realize their conversion into N--fertilizers and acetamides. Based on the CI's recent discoveries, this project will develop an innovative / sustainable system, which could promote the N2 fixation along with CO2 conversion process, a significant alternative approach to simplify the pathways of C-N bond formation. It will thereby contribute to mitigation of greenhouse emissions and create an ecofriendly protocol/technology for distributed production of C-N products under ambient conditions. Read moreRead less
New dimensions of electrocatalyst design for sustainable energy future. This project aims to produce valuable chemicals from air, water and Australia’s abundant renewable energy, by developing efficient, robust catalysts for water oxidation, nitrogen reduction and ammonia oxidation — key processes for sustainable production of green fuels and fertilisers. The interdisciplinary project strategy will use a suite of advanced instrumental and theoretical tools to understand and control how catalysts ....New dimensions of electrocatalyst design for sustainable energy future. This project aims to produce valuable chemicals from air, water and Australia’s abundant renewable energy, by developing efficient, robust catalysts for water oxidation, nitrogen reduction and ammonia oxidation — key processes for sustainable production of green fuels and fertilisers. The interdisciplinary project strategy will use a suite of advanced instrumental and theoretical tools to understand and control how catalysts operate. Expected outcomes include new techniques to study catalysts, new catalyst design concepts, and novel high-performance catalytic materials and devices for sustainable electrosynthesis. These new technologies should reduce emissions and help Australia be a world leader in renewable-energy and fertiliser export.Read moreRead less
Nano-engineered multi-functional materials for catalysis and sensing by an integrated chemical and electrochemical approach. This project aims to deliver a facile and cheap method to produce a class of nanostructured materials to be used in applications which will have environmental and social benefits such as: green synthesis of fine chemicals, catalyst development for clean energy fuel cells and sensor technology for the detection of potent biotoxins.
Electrocatalytic Generation of Ammonia from Air and Water. The aim is to directly convert nitrogen under mild conditions, using renewable power, to form ammonia for fertilisers and fuels, enabled by new, nanostructured, electrocatalysts based on single-sheet and composite materials. Unlike nitrogen fixation using a three-electrode system, the project will use a novel mixed gas- and liquid-phase electrocatalytic nitrogen reduction two-electrode reactor. Based on fuel cells, it is designed to acce ....Electrocatalytic Generation of Ammonia from Air and Water. The aim is to directly convert nitrogen under mild conditions, using renewable power, to form ammonia for fertilisers and fuels, enabled by new, nanostructured, electrocatalysts based on single-sheet and composite materials. Unlike nitrogen fixation using a three-electrode system, the project will use a novel mixed gas- and liquid-phase electrocatalytic nitrogen reduction two-electrode reactor. Based on fuel cells, it is designed to accelerate the naturally sluggish nitrogen reduction reaction, NRR, significantly improving the reaction rate and selectivity. The project will also gain atomic-level understanding of the mechanism of NRR, based on in-situ spectroscopies used under operando conditions, e.g., Raman or X-ray absorption.Read moreRead less
Chlorine Evolution Catalysts for Efferent Seawater Electrolysis. Seawater is the most abundant aqueous resource on earth that is readily accessible at very low costs, but yet to be directly utilised for production of hydrogen fuel and commodity chemicals. This project aims to develop cheap and plentiful carbon-based high performance chlorine evolution electrocatalysts for seawater electrolysis powered by renewable electricity to realise the production of hydrogen, chlorine and sodium hydroxide d ....Chlorine Evolution Catalysts for Efferent Seawater Electrolysis. Seawater is the most abundant aqueous resource on earth that is readily accessible at very low costs, but yet to be directly utilised for production of hydrogen fuel and commodity chemicals. This project aims to develop cheap and plentiful carbon-based high performance chlorine evolution electrocatalysts for seawater electrolysis powered by renewable electricity to realise the production of hydrogen, chlorine and sodium hydroxide directly from seawater. The electrolyser can also be used to treat desalination brine while produce hydrogen and chemicals. The success of the project will set a firm technological foundation for seawater utilisation, which will add to Australian capability to meet future energy and environment challenges.Read moreRead less
Artificial photosynthesis for solar fuel production. We aim to realise an artificial system that converts solar energy to hydrogen (artificial photosynthesis). The resulting device will be able to 'split' water into oxygen and hydrogen, whereas hydrogen can be further converted into electricity or heat (combustion).