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Discovery Early Career Researcher Award - Grant ID: DE190101450
Funder
Australian Research Council
Funding Amount
$392,556.00
Summary
Tuning non-plasmonic metals to high performance photocatalysts. This project aims to develop non-plasmonic, transition metal-based, photocatalysts with enhanced light absorption, to achieve irradiation controllable product selectivity in organic synthesis. The project demonstrates how hollow-particle morphology alloy nano-structures can enhance photocatalytic activity. Alloy structures such as iridium-nickel (IrNi), iridium-cobalt (IrCo) and iridium-tin (IrSn) nanoparticles with a hollow morphol ....Tuning non-plasmonic metals to high performance photocatalysts. This project aims to develop non-plasmonic, transition metal-based, photocatalysts with enhanced light absorption, to achieve irradiation controllable product selectivity in organic synthesis. The project demonstrates how hollow-particle morphology alloy nano-structures can enhance photocatalytic activity. Alloy structures such as iridium-nickel (IrNi), iridium-cobalt (IrCo) and iridium-tin (IrSn) nanoparticles with a hollow morphology, exhibit dramatically increased photocatalytic activity over their individual components, Ir, Ni, Co and Sn respectively. The project is expected to expand the application of photocatalysis and generate knowledge that can be used to design efficient photocatalysts from non-plasmonic metals. Intended benefits are the generation of new knowledge and capabilities in synthetic catalysis and applications in fields such as the conversion of solar energy to chemical energy.Read moreRead less
Discovery Early Career Researcher Award - Grant ID: DE200100477
Funder
Australian Research Council
Funding Amount
$420,770.00
Summary
Developing sustainable liquid fuels from carbon dioxide conversion. This project aims to develop new electrochemical materials and systems capable of converting carbon dioxide to liquid fuels. It expects to generate new knowledge in the area of advanced materials and systems for sustainable fuel production by interdisciplinary integration of catalyst design, real-time characterisation and system engineering. Expected outcomes include electrochemical carbon dioxide-to-alcohol systems with commerc ....Developing sustainable liquid fuels from carbon dioxide conversion. This project aims to develop new electrochemical materials and systems capable of converting carbon dioxide to liquid fuels. It expects to generate new knowledge in the area of advanced materials and systems for sustainable fuel production by interdisciplinary integration of catalyst design, real-time characterisation and system engineering. Expected outcomes include electrochemical carbon dioxide-to-alcohol systems with commercially relevant performances and in-depth understanding of reaction mechanisms at nano and molecular levels. Significant economic, energy and environmental benefits are expected from the concerted greenhouse gas emissions reduction and the development of sustainable, clean, non-fossil fuels, enabled by this project.Read moreRead less
Solar-driven thermochemical dissociation of carbon dioxide and water to produce carbon-neutral fuels. The biggest challenge to humanity of the century is to develop enabling clean energy resources to encounter rapidly diminished fossil fuel and accelerated global warming conditions. This project will offer a solution by developing a unique solar-driven thermochemical system capable of cleaving carbon dioxide and water to produce artificial syngas.
To identify and to understand highly reactive surfaces for solar hydrogen production. This project aims to develop advanced technology to produce hydrogen - carbon-free fuel - from water with sunlight as the only energy input. Using clean energy to replace fossil fuels can help address the issues of energy supply and reduce carbon emissions, which is critically important for a sustainable Australia.
Two-dimensional plasmonic heterogeneous nanostructures for photocatalysis. This project aims to design and explore two-dimensional heterogeneous photocatalysts that can convert solar energy into usable chemical energy. This project will investigate the correlation between surface plasmonic resonance and photocatalytic activities on the atomic level. Heterogeneous engineering and in-situ investigation of atomic-level photocatalytic dynamics is expected to yield several new full-solar-spectrum pho ....Two-dimensional plasmonic heterogeneous nanostructures for photocatalysis. This project aims to design and explore two-dimensional heterogeneous photocatalysts that can convert solar energy into usable chemical energy. This project will investigate the correlation between surface plasmonic resonance and photocatalytic activities on the atomic level. Heterogeneous engineering and in-situ investigation of atomic-level photocatalytic dynamics is expected to yield several new full-solar-spectrum photocatalysts. The project is expected to contribute to the understanding of the processes and mechanisms underlying photocatalysis, and lead to useable, stable and durable photocatalytics. The outcomes will enable efficient, cost-effective and reliable production of clean energy in a low-emission way.Read moreRead less
Selective photocatalytic lignin biomass conversion. If the prospective ‘hydrogen economy’ is to use hydrogen as a fuel and energy carrier to replace fossil sources, vast amounts of renewable cheap hydrogen must be available. A likely candidate is catalytic water splitting by sunlight. The hydrogen can be made affordable, by coupling hydrogen production to a higher value-added stream. The aim of this project is to produce a stable, hybrid heterogenous catalyst system able to oxidise organic subst ....Selective photocatalytic lignin biomass conversion. If the prospective ‘hydrogen economy’ is to use hydrogen as a fuel and energy carrier to replace fossil sources, vast amounts of renewable cheap hydrogen must be available. A likely candidate is catalytic water splitting by sunlight. The hydrogen can be made affordable, by coupling hydrogen production to a higher value-added stream. The aim of this project is to produce a stable, hybrid heterogenous catalyst system able to oxidise organic substrates derived from lignin biomass as an adjunct to visible light hydrogen generation from water. The significance will be to provide fuels and organic chemicals for industry from biomass, water and sunlight and catalytically remediate waste water with sunlight.Read moreRead less
Special Research Initiatives - Grant ID: SR180100036
Funder
Australian Research Council
Funding Amount
$650,054.00
Summary
Remediation of PFAS in current and legacy biosolids application sites. This project aims to develop novel immobilisation, adsorption and/or thermal destruction methods for biosolids, soil and groundwater in current and legacy per- and poly-fluroalkyl substance (PFAS) sites receiving biosolids. Biosolids generated during waste water treatment carry an unknown potential risk of soil and groundwater PFAS contamination, through their application in agriculture and rehabilitation sites. This project ....Remediation of PFAS in current and legacy biosolids application sites. This project aims to develop novel immobilisation, adsorption and/or thermal destruction methods for biosolids, soil and groundwater in current and legacy per- and poly-fluroalkyl substance (PFAS) sites receiving biosolids. Biosolids generated during waste water treatment carry an unknown potential risk of soil and groundwater PFAS contamination, through their application in agriculture and rehabilitation sites. This project will provide the first major investigation of the release, fate and remediation of perfluorinated compounds in relation to their environmental pathways through wastewater treatment plants in Australia. The data will be evaluated to determine if perfluorinated compounds should be further incorporated into Australian soil and water quality monitoring programs. The project will provide evidence of research advice and methodologies being successfully adopted by water industry end-users, government regulatory agencies and private remediation industries.Read moreRead less
Ambient Electrochemical C-N Coupling via Co-electrolysis of N2 and CO2. To overcome the hurdles in N2 fixation (massive energy consumption and CO2 emission), investigators creatively hypothesize that the simultaneous electrocatalytic coupling of N2 and CO2 would enable the selective formation of N-products and thus realize their conversion into N--fertilizers and acetamides. Based on the CI's recent discoveries, this project will develop an innovative / sustainable system, which could promote th ....Ambient Electrochemical C-N Coupling via Co-electrolysis of N2 and CO2. To overcome the hurdles in N2 fixation (massive energy consumption and CO2 emission), investigators creatively hypothesize that the simultaneous electrocatalytic coupling of N2 and CO2 would enable the selective formation of N-products and thus realize their conversion into N--fertilizers and acetamides. Based on the CI's recent discoveries, this project will develop an innovative / sustainable system, which could promote the N2 fixation along with CO2 conversion process, a significant alternative approach to simplify the pathways of C-N bond formation. It will thereby contribute to mitigation of greenhouse emissions and create an ecofriendly protocol/technology for distributed production of C-N products under ambient conditions. Read moreRead less
Computer-Aided Design of High-Performance Photocatalysts for Solar Hydrogen Production Based on Red Titanium Dioxide. Large-scale generation of energy by solar conversion is critical for future sustainability. This project aims to develop high performance materials to efficiently convert solar energy to hydrogen - a clean fuel. Starting from the newly developed material red titanium dioxide, novel strategies for improved photocatalytic materials will be proposed and evaluated by advanced computa ....Computer-Aided Design of High-Performance Photocatalysts for Solar Hydrogen Production Based on Red Titanium Dioxide. Large-scale generation of energy by solar conversion is critical for future sustainability. This project aims to develop high performance materials to efficiently convert solar energy to hydrogen - a clean fuel. Starting from the newly developed material red titanium dioxide, novel strategies for improved photocatalytic materials will be proposed and evaluated by advanced computational approaches. Key issues for solar-to-hydrogen conversion will be clarified. The materials, knowledge and strategies achieved by this project will dramatically enhance current solar technology and in particular will advance the development of low-cost hydrogen production from water. Read moreRead less
New dimensions of electrocatalyst design for sustainable energy future. This project aims to produce valuable chemicals from air, water and Australia’s abundant renewable energy, by developing efficient, robust catalysts for water oxidation, nitrogen reduction and ammonia oxidation — key processes for sustainable production of green fuels and fertilisers. The interdisciplinary project strategy will use a suite of advanced instrumental and theoretical tools to understand and control how catalysts ....New dimensions of electrocatalyst design for sustainable energy future. This project aims to produce valuable chemicals from air, water and Australia’s abundant renewable energy, by developing efficient, robust catalysts for water oxidation, nitrogen reduction and ammonia oxidation — key processes for sustainable production of green fuels and fertilisers. The interdisciplinary project strategy will use a suite of advanced instrumental and theoretical tools to understand and control how catalysts operate. Expected outcomes include new techniques to study catalysts, new catalyst design concepts, and novel high-performance catalytic materials and devices for sustainable electrosynthesis. These new technologies should reduce emissions and help Australia be a world leader in renewable-energy and fertiliser export.Read moreRead less