ORCID Profile
0000-0002-1109-0772
Current Organisations
Max Planck Institute for Chemistry
,
University of South Australia
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In Research Link Australia (RLA), "Research Topics" refer to ANZSRC FOR and SEO codes. These topics are either sourced from ANZSRC FOR and SEO codes listed in researchers' related grants or generated by a large language model (LLM) based on their publications.
Functional Materials | Materials Engineering | Nanomaterials | Water Treatment Processes | Energy Generation, Conversion and Storage Engineering | Colloid and Surface Chemistry | Nanotechnology | Nanofabrication, Growth and Self Assembly
Expanding Knowledge in the Chemical Sciences | Solar-Thermal Energy | Expanding Knowledge in the Physical Sciences |
Publisher: Elsevier BV
Date: 05-2022
Publisher: American Chemical Society (ACS)
Date: 08-2018
Abstract: Employing nanoscaled materials as photosensitizer (PS) carriers is an effective strategy to solve the problem of poor solubility and low tumor selectivity of hydrophobic PS in photodynamic therapy (PDT), which compulsorily requires the PS release in PDT implementation. However, the complicated environment in vivo makes it difficult to precisely design and control the release process and the delivery process requires real-time tracking. Developing a delivery strategy of hydrophobic PS in the monomeric form with fluorescent emission and without consideration of the PS release in the PDT process, is in urgent demand. Herein, we report a versatile and potent strategy for fabrication of photodynamic nanoparticles (nanoPSs) with featuring the monomeric PS based on aromatic peptide-modulated self-assembly of porphyrin derivatives. Aromatic peptides within nanoPSs can isolate hydrophobic porphyrins from each other, resulting in monomeric porphyrin delivery with real-time fluorescence tracking property and avoiding self-aggregation and hence porphyrin release. Moreover, partially charged porphyrins tend to expose on the surface of nanoPSs, facilitating production and diffusion of
Publisher: Wiley
Date: 07-2020
Publisher: Springer Science and Business Media LLC
Date: 07-2021
DOI: 10.1038/S41567-021-01225-Z
Abstract: Leptons with essentially the same properties apart from their mass are grouped into three families (or flavours). The number of leptons of each flavour is conserved in interactions, but this is not imposed by fundamental principles. Since the formulation of the standard model of particle physics, the observation of flavour oscillations among neutrinos has shown that lepton flavour is not conserved in neutrino weak interactions. So far, there has been no experimental evidence that this also occurs in interactions between charged leptons. Such an observation would be a sign of undiscovered particles or a yet unknown type of interaction. Here the ATLAS experiment at the Large Hadron Collider at CERN reports a constraint on lepton-flavour-violating effects in weak interactions, searching for Z -boson decays into a τ lepton and another lepton of different flavour with opposite electric charge. The branching fractions for these decays are measured to be less than 8.1 × 10 −6 ( e τ ) and 9.5 × 10 −6 ( μ τ ) at the 95% confidence level using 139 fb −1 of proton–proton collision data at a centre-of-mass energy of $$\\sqrt{s}=13\\,{\\rm{TeV}}$$ s = 13 TeV and 20.3 fb −1 at $$\\sqrt{s}=8\\,{\\rm{TeV}}.$$ s = 8 TeV . These results supersede the limits from the Large Electron–Positron Collider experiments conducted more than two decades ago.
Publisher: American Physical Society (APS)
Date: 26-03-2021
Publisher: Informa UK Limited
Date: 19-09-2018
Publisher: American Chemical Society (ACS)
Date: 29-10-2008
DOI: 10.1021/JP807379C
Publisher: American Chemical Society (ACS)
Date: 16-03-1616
DOI: 10.1021/CM2028417
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 05-2019
Publisher: Springer Science and Business Media LLC
Date: 06-2021
Abstract: Fiducial and differential cross-section measurements of W + W − production in association with at least one hadronic jet are presented. These measurements are sensitive to the properties of electroweak-boson self-interactions and provide a test of perturbative quantum chromodynamics and the electroweak theory. The analysis is performed using proton-proton collision data collected at $$ \sqrt{s} $$ s = 13 TeV with the ATLAS experiment, corresponding to an integrated luminosity of 139 fb − 1 . Events are selected with exactly one oppositely charged electron-muon pair and at least one hadronic jet with a transverse momentum of p T 30 GeV and a pseudorapidity of | η | 4 . 5. After subtracting the background contributions and correcting for detector effects, the jet-inclusive W + W − + ≥ 1 jet fiducial cross-section and W + W − + jets differential cross-sections with respect to several kinematic variables are measured. These measurements include leptonic quantities, such as the lepton transverse momenta and the transverse mass of the W + W − system, as well as jet-related observables such as the leading jet transverse momentum and the jet multiplicity. Limits on anomalous triple-gauge-boson couplings are obtained in a phase space where interference between the Standard Model litude and the anomalous litude is enhanced.
Publisher: Elsevier BV
Date: 03-2023
Publisher: Royal Society of Chemistry (RSC)
Date: 2020
DOI: 10.1039/D0CC04779A
Abstract: High CO selectivity for the CO 2 electroreduction reaction was achieved on Ni–Cu bimetallic catalysts. We observed that changing the Cu content in the catalysts causes charge redistribution which results in a negative correlation with CO selectivity.
Publisher: Wiley
Date: 13-07-2022
Abstract: With the increase in water consumption and pollution resulting from the rising world population and industrial development, severe fresh water shortage has been regarded as one of the critical problems facing the world. Solar‐driven water purification is an environment friendly and promising technology to address the problem. However, low photothermal conversion efficiency impedes its practical application. Herein, a natural spruce wood‐based solar evaporator functionalized with zeolitic imidazolate framework (ZIF‐8) nanoparticles and polydopamine (PDA) layers is designed, which significantly reduces the equivalent evaporation enthalpy and substantially boosts solar evaporation efficiency. The evaporation rate of the optimized wood‐based evaporator reached 2.28 kg m −2 h −1 with a high evaporation efficiency of 87.5% under 1.0 sun. Furthermore, the integrated spruce wood/ZIF‐8/PDA hybrids can remove organic pollutants after solar evaporation. Notably, the constructed multifunctional solar evaporator takes advantage of sustainable solar energy, low‐cost biomass, and ZIF‐8/PDA nanostructures to acquire desirable performance in water evaporation and sewage purification.
Publisher: Royal Society of Chemistry (RSC)
Date: 2019
DOI: 10.1039/C8SE00538A
Abstract: Highly efficient nanocatalysts which can selectively decompose hydrous hydrazine for hydrogen production are introduced.
Publisher: Springer Science and Business Media LLC
Date: 10-2021
Abstract: A search for dark-matter particles in events with large missing transverse momentum and a Higgs boson candidate decaying into two photons is reported. The search uses 139 fb − 1 of proton-proton collision data collected at $$ \\sqrt{s} $$ s = 13 TeV with the ATLAS detector at the CERN LHC between 2015 and 2018. No significant excess of events over the Standard Model predictions is observed. The results are interpreted by extracting limits on three simplified models that include either vector or pseudoscalar mediators and predict a final state with a pair of dark-matter candidates and a Higgs boson decaying into two photons.
Publisher: American Physical Society (APS)
Date: 19-02-2021
Publisher: American Chemical Society (ACS)
Date: 10-06-2021
Publisher: Elsevier BV
Date: 09-2006
Publisher: American Physical Society (APS)
Date: 11-05-2022
Publisher: American Chemical Society (ACS)
Date: 11-07-2022
Publisher: American Chemical Society (ACS)
Date: 08-05-2014
DOI: 10.1021/AM501632F
Abstract: We report a facile method to synthesize Fe3O4@polydopamine (PDA)-Ag core-shell microspheres. Ag nanoparticles (NPs) are deposited on PDA surfaces via in situ reduction by mussel-inspired PDA layers. High catalytic activity and fast adsorption of a model dye methylene blue (MB) at different pH values are achieved mainly due to the presence of monodisperse Ag NPs and electrostatic interactions between PDA and MB. The as-prepared Fe3O4@PDA-Ag microspheres also show high cyclic stability (>27 cycles), good acid stability, and fast regeneration ability, which can be achieved efficiently within several minutes by using NaBH4 as the desorption agent, showing great potentials in a wide range of applications.
Publisher: American Chemical Society (ACS)
Date: 30-10-2015
DOI: 10.1021/ACS.LANGMUIR.5B03303
Abstract: Solvent exchange is a simple process to form oil nanodroplets at solid-liquid interfaces with well-defined location and morphology. In this process, a good solvent of the oil is displaced by a poor solvent, leading to the nucleation and growth of oil droplets from a transient oversaturation at the mixing front. Our recent work has shown that the final volume of the droplets is related to the flow conditions. In this work, we investigate the effects of the type and the composition of solvents on the droplet formation under the same flow conditions. Water nanodroplets were produced by ethanol/cyclohexane (solution A) and cyclohexane (solution B) on a hydrophilic substrate. We found that the droplet size increases first and then decreases with an increase of the initial ethanol concentration in solution A. This is attributed to the phase separation of ethanol-cyclohexane-water in particular, the composition of solution A on the phase boundary above the Ouzo region. The same reason also contributes to the lower efficiency in droplet formation for a longer alkane. The important implication from this work is that the maximal droplet volume is limited by the phase separation of the solvents used in the solvent exchange.
Publisher: Elsevier BV
Date: 2021
Publisher: Elsevier BV
Date: 05-2022
Publisher: Elsevier BV
Date: 10-2017
Publisher: IEEE
Date: 07-2017
Publisher: IOP Publishing
Date: 07-2021
DOI: 10.1088/1748-0221/16/07/P07029
Abstract: The ATLAS experiment at the Large Hadron Collider (LHC) employs a trigger system consisting of a first-level hardware trigger (L1) and a software-based high-level trigger. The L1 muon trigger system selects muon candidates, assigns them to the correct LHC bunch crossing and classifies them into one of six transverse-momentum threshold classes. The L1 muon trigger system uses resistive-plate chambers (RPCs) to generate the muon-induced trigger signals in the central (barrel) region of the ATLAS detector. The ATLAS RPCs are arranged in six concentric layers and operate in a toroidal magnetic field with a bending power of 1.5 to 5.5 Tm. The RPC detector consists of about 3700 gas volumes with a total surface area of more than 4000 m 2 . This paper reports on the performance of the RPC detector and L1 muon barrel trigger using 60.8 fb -1 of proton-proton collision data recorded by the ATLAS experiment in 2018 at a centre-of-mass energy of 13 TeV. Detector and trigger performance are studied using Z boson decays into a muon pair. Measurements of the RPC detector response, efficiency, and time resolution are reported. Measurements of the L1 muon barrel trigger efficiencies and rates are presented, along with measurements of the properties of the selected s le of muon candidates. Measurements of the RPC currents, counting rates and mean avalanche charge are performed using zero-bias collisions. Finally, RPC detector response and efficiency are studied at different high voltage and front-end discriminator threshold settings in order to extrapolate detector response to the higher luminosity expected for the High Luminosity LHC.
Publisher: Springer Science and Business Media LLC
Date: 11-2021
Abstract: A measurement of prompt photon-pair production in proton-proton collisions at $$ \\sqrt{s} $$ s = 13 TeV is presented. The data were recorded by the ATLAS detector at the LHC with an integrated luminosity of 139 fb − 1 . Events with two photons in the well-instrumented region of the detector are selected. The photons are required to be isolated and have a transverse momentum of $$ {p}_{\\mathrm{T}{,}_{\\gamma 1(2)}} $$ p T , γ 1 2 40 (30) GeV for the leading (sub-leading) photon. The differential cross sections as functions of several observables for the diphoton system are measured and compared with theoretical predictions from state-of-the-art Monte Carlo and fixed-order calculations. The QCD predictions from next-to-next-to-leading-order calculations and multi-leg merged calculations are able to describe the measured integrated and differential cross sections within uncertainties, whereas lower-order calculations show significant deviations, demonstrating that higher-order perturbative QCD corrections are crucial for this process. The resummed predictions with parton showers additionally provide an excellent description of the low transverse-momentum regime of the diphoton system.
Publisher: Wiley
Date: 06-2017
Publisher: Elsevier BV
Date: 12-2022
Publisher: Wiley
Date: 08-03-2023
Abstract: The rational design of economic and high‐performance electrocatalytic water‐splitting systems is of great significance for energy and environmental sustainability. Developing a sustainable energy conversion‐assisted electrocatalytic process provides a promising novel approach to effectively boost its performance. Herein, a self‐sustained water‐splitting system originated from the heterostructure of perovskite oxide with 2D Ti 3 C 2 T x MXene on Ni foam (La 1‐x Sr x CoO 3 /Ti 3 C 2 T x MXene/Ni) that shows high activity for solar‐powered water evaporation and simultaneous electrocatalytic water splitting is presented. The all‐in‐one interfacial electrocatalyst exhibits highly improved oxygen evolution reaction (OER) performance with a low overpotential of 279 mV at 10 mA cm −2 and a small Tafel slope of 74.3 mV dec −1 , superior to previously reported perovskite oxide‐based electrocatalysts. Density functional theory calculations reveal that the integration of La 0.9 Sr 0.1 CoO 3 with Ti 3 C 2 T x MXene can lower the energy barrier for the electron transfer and decrease the OER overpotential, while COMSOL simulations unveil that interfacial solar evaporation could induce OH − enrichment near the catalyst surfaces and enhance the convection flow above the catalysts to remove the generated gas, remarkably accelerating the kinetics of electrocatalytic water splitting.
Publisher: Wiley
Date: 17-04-2020
Publisher: Elsevier BV
Date: 10-2023
Publisher: Elsevier BV
Date: 08-2021
Publisher: Elsevier BV
Date: 2021
Publisher: Elsevier BV
Date: 02-2019
Publisher: Wiley
Date: 11-05-2021
Abstract: Present one‐step N 2 fixation is impeded by tough activation of the N≡N bond and low selectivity to NH 3 . Here we report fixation of N 2 ‐to‐NH 3 can be decoupled to a two‐step process with one problem effectively solved in each step, including: 1) facile activation of N 2 to NO x − by a non‐thermal plasma technique, and 2) highly selective conversion of NO x − to NH 3 by electrocatalytic reduction. Importantly, this process uses air and water as low‐cost raw materials for scalable ammonia production under ambient conditions. For NO x − reduction to NH 3 , we present a surface boron‐rich core–shell nickel boride electrocatalyst. The surface boron‐rich feature is the key to boosting activity, selectivity, and stability via enhanced NO x − adsorption, and suppression of hydrogen evolution and surface Ni oxidation. A significant ammonia production of 198.3 μmol cm −2 h −1 was achieved, together with nearly 100 % Faradaic efficiency.
Publisher: Royal Society of Chemistry (RSC)
Date: 2014
DOI: 10.1039/C4RA03024A
Abstract: In this work, we developed a facile electrochemical deposition approach to prepare Gd-doped CeO x nanoflowers on porous carbon foam with improved supercapacitor characteristics by UV irradiation.
Publisher: Springer Science and Business Media LLC
Date: 22-03-2018
DOI: 10.1038/S41598-018-22956-9
Abstract: A correction to this article has been published and is linked from the HTML and PDF versions of this paper. The error has been fixed in the paper.
Publisher: Wiley
Date: 22-09-2022
Abstract: Power generation by converting energy from the ambient environment has been considered a promising strategy for developing decentralized electrification systems to complement the electricity supply for daily use. Wet gases, such as water evaporation or moisture in the atmosphere, can be utilized as a tremendous source of electricity by emerging power generation devices, that is, moisture‐enabled‐electric nanogenerators (MEENGs). As a promising technology, MEENGs provided a novel manner to generate electricity by harvesting energy from moisture, originating from the interactions between water molecules and hydrophilic functional groups. Though the remarkable progress of MEENGs has been achieved, a systematic review in this specific area is urgently needed to summarize previous works and provide sharp points to further develop low‐cost and high‐performing MEENGs through overcoming current limitations. Herein, the working mechanisms of MEENGs reported so far are comprehensively compared. Subsequently, a systematic summary of the materials selection and fabrication methods for currently reported MEENG construction is presented. Then, the improvement strategies and development directions of MEENG are provided. At last, the demonstrations of the applications assembled with MEENGs are extracted. This work aims to pave the way for the further MEENGs to break through the performance limitations and promote the popularization of future micron electronic self‐powered equipment.
Publisher: American Chemical Society (ACS)
Date: 15-11-2007
DOI: 10.1021/CG060727K
Publisher: Springer Science and Business Media LLC
Date: 06-2021
DOI: 10.1140/EPJC/S10052-021-09192-8
Abstract: The paper presents a measurement of the Standard Model Higgs Boson decaying to b -quark pairs in the vector boson fusion (VBF) production mode. A s le corresponding to 126 $$\\hbox {fb}^{-1}$$ fb - 1 of $$\\sqrt{s} = 13\\,\\text {TeV}$$ s = 13 TeV proton–proton collision data, collected with the ATLAS experiment at the Large Hadron Collider, is analyzed utilizing an adversarial neural network for event classification. The signal strength, defined as the ratio of the measured signal yield to that predicted by the Standard Model for VBF Higgs production, is measured to be $$0.95^{+0.38}_{-0.36}$$ 0 . 95 - 0.36 + 0.38 , corresponding to an observed (expected) significance of 2.6 (2.8) standard deviations from the background only hypothesis. The results are additionally combined with an analysis of Higgs bosons decaying to b -quarks, produced via VBF in association with a photon.
Publisher: Elsevier BV
Date: 10-2022
Publisher: Springer Science and Business Media LLC
Date: 11-2021
Publisher: Elsevier BV
Date: 09-2006
Publisher: Springer Science and Business Media LLC
Date: 02-2014
Publisher: Elsevier BV
Date: 12-2021
Publisher: Springer Science and Business Media LLC
Date: 06-2021
Abstract: A search for charged Higgs bosons decaying into a top quark and a bottom quark is presented. The data analysed correspond to 139 fb − 1 of proton-proton collisions at $$ \\sqrt{s} $$ s = 13 TeV, recorded with the ATLAS detector at the LHC. The production of a heavy charged Higgs boson in association with a top quark and a bottom quark, pp → tbH + → tbtb , is explored in the H + mass range from 200 to 2000 GeV using final states with jets and one electron or muon. Events are categorised according to the multiplicity of jets and b -tagged jets, and multivariate analysis techniques are used to discriminate between signal and background events. No significant excess above the background-only hypothesis is observed and exclusion limits are derived for the production cross-section times branching ratio of a charged Higgs boson as a function of its mass they range from 3.6 pb at 200 GeV to 0.036 pb at 2000 GeV at 95% confidence level. The results are interpreted in the hMSSM and $$ {M}_h^{125} $$ M h 125 scenarios.
Publisher: Wiley
Date: 08-02-2021
Publisher: Elsevier BV
Date: 10-2021
Publisher: Elsevier BV
Date: 05-2021
Publisher: Springer Science and Business Media LLC
Date: 2021
Abstract: Differential cross-sections are measured for top-quark pair production in the all-hadronic decay mode, using proton-proton collision events collected by the ATLAS experiment in which all six decay jets are separately resolved. Absolute and normalised single- and double-differential cross-sections are measured at particle and parton level as a function of various kinematic variables. Emphasis is placed on well-measured observables in fully reconstructed final states, as well as on the study of correlations between the top-quark pair system and additional jet radiation identified in the event. The study is performed using data from proton-proton collisions at $$ \\sqrt{s} $$ s = 13 TeV collected by the ATLAS detector at CERN’s Large Hadron Collider in 2015 and 2016, corresponding to an integrated luminosity of 36.1 fb − 1 . The rapidities of the in idual top quarks and of the top-quark pair are well modelled by several independent event generators. Significant mismodelling is observed in the transverse momenta of the leading three jet emissions, while the leading top-quark transverse momentum and top-quark pair transverse momentum are both found to be incompatible with several theoretical predictions.
Publisher: Royal Society of Chemistry (RSC)
Date: 2018
DOI: 10.1039/C8SM00623G
Abstract: Understanding the surface properties and rheology of colloidal suspensions in the presence of polymer additives with high salinity is of great importance in a wide range of industrial applications.
Publisher: Informa UK Limited
Date: 20-12-2018
Publisher: Wiley
Date: 11-03-2021
Publisher: Elsevier BV
Date: 08-2020
Publisher: American Chemical Society (ACS)
Date: 24-03-2015
Publisher: Royal Society of Chemistry (RSC)
Date: 2020
DOI: 10.1039/D0TA03799K
Abstract: Ni 1 Co 3 @PDA nanosheets were utilized as photothermal materials in a kerosene l -like evaporator for solar steam generation. A high evaporation rate of 2.42 kg m −2 h −1 with a corresponding energy efficiency beyond the theoretical limit was achieved.
Publisher: Elsevier BV
Date: 06-2022
Publisher: Royal Society of Chemistry (RSC)
Date: 2016
DOI: 10.1039/C6RA17663A
Publisher: American Chemical Society (ACS)
Date: 23-01-2008
DOI: 10.1021/CG0705761
Publisher: Wiley
Date: 28-07-2023
Abstract: Porous‐structured evaporators have been fabricated for achieving a high clean water throughput due to their maximized surface area. However, most of the evaporation surfaces in the porous structure are not active because of the trapped vapor in pores. Herein, a three‐dimensional (3D) cylindrical aerogel‐based photothermal evaporator with a disordered interconnected hierarchical porous structure is developed via a Pickering emulsion‐involved polymerization method. The obtained cotton cellulose/aramid nanofibers olypyrrole (CAP) aerogel‐based evaporator achieved all‐cold evaporation under 1.0 sun irradiation, which not only completely eliminated energy loss via radiation, convection, and conduction, but also harvested massive extra energy from the surrounding environment and bulk water, thus significantly increasing the total energy input for vapor generation to deliver an extremely high evaporation rate of 5.368 kg m −2 h −1 . In addition, with the external convective flow, solar steam generation over the evaporator can be dramatically enhanced due to fast vapor diffusion out of its unique opened porous structure, realizing an ultrahigh evaporation rate of 18.539 kg m −2 h −1 under 1.0 sun and 4.0 m s −1 . Moreover, this evaporator can continuously operate with concentrated salt solution (20 wt.% NaCl). This work advances rational design and construction of solar evaporator to promote the application of solar evaporation technology in freshwater production.
Publisher: American Chemical Society (ACS)
Date: 17-09-2012
DOI: 10.1021/LA3027804
Abstract: In this report, we demonstrate a rapid and simple seeded growth method for synthesizing monodisperse, quasi-spherical, citrate-stabilized Au nanoparticles (Au NPs) via H(2)O(2) reduction of HAuCl(4). Au NPs with diameter ranging from 30 to 230 nm can be synthesized by simply adding 12 nm citrate stabilized Au NP seeds to an aqueous solution of H(2)O(2) and HAuCl(4) under ambient conditions. The diameter of the resulting Au NPs can be quantitatively controlled by the molar ratio of HAuCl(4) to the Au seeds. The standard deviation of the Au NP sizes is less than 10%, and the ellipticity (ratio of major to minor axes) of the NPs is less than 1.1. Compared to existing ones, the present seeded growth approach is implemented within 1 min under ambient condition, and no unfavorable additives are involved because H(2)O(2) can readily decompose into H(2)O during storage or via boiling.
Publisher: Elsevier BV
Date: 2023
Publisher: American Chemical Society (ACS)
Date: 26-09-2014
DOI: 10.1021/JP5076109
Publisher: Springer Science and Business Media LLC
Date: 07-06-2023
DOI: 10.1007/S41101-023-00195-Y
Abstract: It is well accepted that moisture ingress in concrete reduces durability and life span of water assets. Condition assessment is an important tool to inform decision for maintenance, retrofit or replacement. However, the most significant challenge is to obtain accurate condition information, particularly when the inspection points are physically difficult to access or inaccessible. Therefore, a reliable and cost-effective monitoring (sensor) system, preferably real-time with ability to streaming online, would be a useful management tool, particularly for water utilities. This paper describes an approach to develop a distributed optical fibre humidly sensor for condition assessment and environmental monitoring both inside and outside of infrastructures, such as inside the concrete and surrounding soil. A new polyelectrolyte multilayer (PEM) coating with higher sensitive was evaluated for relative humidity measurement in soil and concrete, respectively. In this study, two simulated conditions, in concrete and soil, were conducted to evaluate the sensing concept with the development of appropriate measuring methodologies including fibre installation and protection. The optical fibre sensor setup in laboratory environment showed that optical sensor can detect and indicate voltage change with the variation of moisture contents in both soil and concrete. The test results indicate a good correlation between high levels of relative humidity/moisture and transmitted optical power. A simple relative humidity (RH) calibration can be used to convert signal to RH in percentage for soil and concrete measurements and the procedure used to imbed the fibre in both s les is effective. Nevertheless, the sensor measures soil humidity (not moisture content) therefore, further investigation is required to identify the consequence for the variation of the measured parameter.
Publisher: Wiley
Date: 26-01-2009
Abstract: By introducing VO(3)(-) into the reaction system, uniform hierarchical nanostructures of Bi(2)O(3) have been successfully synthesized by a template-free aqueous method at 60-80 degrees C for 6 h. The as-prepared hierarchitectures are composed of 2D nanosheets, which intercross with each other. Based on the electron microscope observations, the growth of such hierarchitectures has been proposed as an Ostwald ripening process followed by self-assembly. The nucleation, growth, and self-assembly of Bi(2)O(3) nanosheets could be readily tuned, which brought different morphologies and microstructures to the final products. Pore-size distribution analysis revealed that both mesopores and macropores existed in the product. UV-vis spectroscopy was employed to estimate the band gap energies of the hierarchical nanostructures. The photocatalytic activities of as-prepared Bi(2)O(3) hierarchitectures were 6-10 times higher than that of the commercial s le, which was evaluated by the degradation of RhB dye under visible light irradiation (lambda>420 nm).
Publisher: Royal Society of Chemistry (RSC)
Date: 2013
DOI: 10.1039/C3CC47509C
Abstract: It is found that emulsion droplets could adsorb onto particle (Cu2O) surfaces to form interfacial nanodroplets. The emulsion droplets capped domains on surfaces are protected, while the uncapped domains are exposed, thus allowing direct heterogeneous surface engineering in particle suspension.
Publisher: Royal Society of Chemistry (RSC)
Date: 2018
DOI: 10.1039/C8RA00454D
Abstract: Porous ion-exchange resins with features of high selectivity, high capacity, fast adsorption kinetics and chemical stability over a wide pH range are attractive for extracting precious metals like copper and upcycling waste.
Publisher: Elsevier BV
Date: 2022
Publisher: Springer Science and Business Media LLC
Date: 07-2021
Abstract: Measurements of four-lepton differential and integrated fiducial cross-sections in events with two same-flavour, opposite-charge electron or muon pairs are presented. The data correspond to 139 fb − 1 of $$ \\sqrt{s} $$ s = 13 TeV proton-proton collisions, collected by the ATLAS detector during Run 2 of the Large Hadron Collider (2015–2018). The final state has contributions from a number of interesting Standard Model processes that dominate in different four-lepton invariant mass regions, including single Z boson production, Higgs boson production and on-shell ZZ production, with a complex mix of interference terms, and possible contributions from physics beyond the Standard Model. The differential cross-sections include the four-lepton invariant mass inclusively, in slices of other kinematic variables, and in different lepton flavour categories. Also measured are dilepton invariant masses, transverse momenta, and angular correlation variables, in four regions of four-lepton invariant mass, each dominated by different processes. The measurements are corrected for detector effects and are compared with state-of-the-art Standard Model calculations, which are found to be consistent with the data. The Z → 4 ℓ branching fraction is extracted, giving a value of (4 . 41 ± 0 . 30) × 10 − 6 . Constraints on effective field theory parameters and a model based on a spontaneously broken B − L gauge symmetry are also evaluated. Further reinterpretations can be performed with the provided information.
Publisher: Royal Society of Chemistry (RSC)
Date: 2007
DOI: 10.1039/B616460A
Publisher: American Chemical Society (ACS)
Date: 28-08-2007
DOI: 10.1021/JP065155T
Publisher: Elsevier BV
Date: 02-2019
Publisher: MDPI AG
Date: 03-04-2014
DOI: 10.3390/NANO4020256
Publisher: Royal Society of Chemistry (RSC)
Date: 2023
DOI: 10.1039/D3EE00770G
Abstract: Illustration of protein-based MEG generating electricity by absorbing water from moisture.
Publisher: Elsevier BV
Date: 06-2006
Publisher: Elsevier BV
Date: 10-2015
DOI: 10.1016/J.CIS.2015.07.004
Abstract: Nanoscale oil droplets locating at solid-liquid interfaces significantly impact the interfacial properties, which are concerned in both industry applications and fundamental studies. This review article presents an overview of the current progress in nanodroplet research. We will start from the characterization of interfacial nanodroplets and the formation of interfacial nanodroplets by direct adsorption from emulsions and by the solvent exchange protocol. Then we will review the experimental and theoretical studies on the evolution of oil nanodroplets including spreading, dissolution, and detachment. We will also cover the emerging applications of the interfacial nanodroplets in the fields of surface functionalization and nanostructure engineering, and particularly, highlight the potential application as capping agents to obtain architectures on microparticle surface. Finally we propose the challenges and the opportunities in this area. In our opinion, the nanodroplets have not only of high relevance to practical applications, but also serve as a model system for understanding many interfacial phenomena, such as phase separation and wetting on a microscopic scale.
Publisher: Wiley
Date: 22-05-2017
Publisher: Springer Science and Business Media LLC
Date: 15-02-2006
Publisher: Elsevier BV
Date: 05-2022
Publisher: Elsevier BV
Date: 06-2023
Publisher: Springer Science and Business Media LLC
Date: 06-05-2014
DOI: 10.1038/SREP04849
Publisher: Institute of Electrical and Electronics Engineers (IEEE)
Date: 05-2019
Publisher: Elsevier BV
Date: 12-2013
Publisher: American Chemical Society (ACS)
Date: 30-08-2012
DOI: 10.1021/LA302394E
Abstract: Polydopamine (PDA)-Au Janus particles were obtained by simply adding HAuCl(4) to a PDA particle suspension, prepared via self-polymerization of dopamine in basic solution at room temperature. The structures of the PDA-Au particles are readily controlled by electrostatic repulsion between the constituent particles, which can be realized simply via adjusting the environmental pH. PDA-Au Janus particles are formed only in a narrow pH range of 2.5-3.0 due to the properly enhanced electrostatic repulsion between the Au particles growing on as-prepared PDA particles and between the Au and PDA particles. The obtained PDA-Au Janus particles can become interfacially active and self-assemble at oil/water interfaces as a result of spatially well-separated hydrophilic (PDA) and hydrophobic (Au) domains on the surfaces, reminiscent of hiphilic molecules.
Publisher: IOP Publishing
Date: 08-2018
Publisher: IOP Publishing
Date: 08-2021
DOI: 10.1088/1748-0221/16/08/P08025
Abstract: Non-ionizing energy loss causes bulk damage to the silicon sensors of the ATLAS pixel and strip detectors. This damage has important implications for data-taking operations, charged-particle track reconstruction, detector simulations, and physics analysis. This paper presents simulations and measurements of the leakage current in the ATLAS pixel detector and semiconductor tracker as a function of location in the detector and time, using data collected in Run 1 (2010–2012) and Run 2 (2015–2018) of the Large Hadron Collider. The extracted fluence shows a much stronger | z |-dependence in the innermost layers than is seen in simulation. Furthermore, the overall fluence on the second innermost layer is significantly higher than in simulation, with better agreement in layers at higher radii. These measurements are important for validating the simulation models and can be used in part to justify safety factors for future detector designs and interventions.
Publisher: Royal Society of Chemistry (RSC)
Date: 2018
DOI: 10.1039/C8TA03280G
Abstract: Inspired by a kerosene oil l , a highly efficient solar-evaporation system with the evaporation surface located above the bulk water surface is realized.
Publisher: American Physical Society (APS)
Date: 24-03-2021
Publisher: Springer Science and Business Media LLC
Date: 11-2021
Abstract: A measurement of four-top-quark production using proton-proton collision data at a centre-of-mass energy of 13 TeV collected by the ATLAS detector at the Large Hadron Collider corresponding to an integrated luminosity of 139 fb − 1 is presented. Events are selected if they contain a single lepton (electron or muon) or an opposite-sign lepton pair, in association with multiple jets. The events are categorised according to the number of jets and how likely these are to contain b -hadrons. A multivariate technique is then used to discriminate between signal and background events. The measured four-top-quark production cross section is found to be $$ {26}_{-15}^{+17} $$ 26 − 15 + 17 fb, with a corresponding observed (expected) significance of 1.9 (1.0) standard deviations over the background-only hypothesis. The result is combined with the previous measurement performed by the ATLAS Collaboration in the multilepton final state. The combined four-top-quark production cross section is measured to be $$ {24}_{-6}^{+7} $$ 24 − 6 + 7 fb, with a corresponding observed (expected) signal significance of 4.7 (2.6) standard deviations over the background-only predictions. It is consistent within 2.0 standard deviations with the Standard Model expectation of 12 . 0 ± 2 . 4 fb.
Publisher: Elsevier BV
Date: 10-2006
Publisher: Elsevier BV
Date: 05-2008
Publisher: Hindawi Limited
Date: 2014
DOI: 10.1155/2014/902730
Abstract: Metal oxide nanosheets have promising potential applications in novel energy storage devices. In this work, Co 3 O 4 nanosheets/carbon foam with excellent supercapacitor characteristics was successfully fabricated, without using metal substrates. The experimental results demonstrate that the electrochemical tests showed that the as-prepared Co 3 O 4 nanosheets exhibited an ideal capacitive behavior with a maximum specific capacitance of 106 F/g in 1 M NaOH solution at a scan rate of 0.1 V s −1 .
Publisher: Wiley
Date: 30-04-2022
Abstract: Herein, using hierarchical porous CuS–cellulose composite as photothermal materials, a 3D opened hollow photothermal evaporator is designed and fabricated to target high solar evaporation rates. Such a unique structure not only imparts the solar evaporator with an efficient water evaporation by minimizing energy loss, introducing cold evaporation surfaces for drawing additional energy from the bulk water and surrounding air, but also fully activates evaporation on both inner and outer evaporation surfaces, thus delivering superior evaporation rates compared to the enclosed evaporators. Moreover, under convective flow, this special structure effectively promotes the escape of vapor inside the evaporator to avoid the vapor accumulation, further enhancing the evaporation on inner evaporation surfaces, thus improving the evaporation rate up to11.911 kg m −2 h −1 under a convective flow rate of 4.0 m s −1 and 1.0 sun irradiation. The operability of the as‐prepared solar evaporator under natural environmental conditions is examined by outdoor evaporation tests. The obtained solar evaporator is demonstrated to be applicable for generating clean water from model seawater and dye wastewater. An impetus for promoting practical application of solar steam generation in seawater desalination and wastewater purification is provided.
Publisher: American Chemical Society (ACS)
Date: 08-01-2009
DOI: 10.1021/IE801516U
Publisher: Wiley
Date: 18-06-2021
Abstract: Interfacial solar steam generation offers a promising and cost‐effective way for saline water desalination. However, salt accumulation and deposition on photothermal materials during saline and brine evaporation is detrimental to the stability and sustainability of solar evaporation. Although several antisalt strategies are developed, it is difficult to simultaneously achieve high evaporation rates ( 2.0 kg m −2 h −1 ) and energy efficiencies. In this study, a self‐rotating photothermal evaporator with dual evaporation zones (i.e., high‐temperature and low‐temperature evaporation zones) is developed. This photothermal evaporator is sensitive to weight imbalance ( 15 mg) thus is able to quickly respond to salt accumulation by rotation to refresh the evaporation surface, while the dual evaporation zones optimize the energy nexus during solar evaporation, simultaneously realizing excellent salt‐resistant performance and high evaporation rate (2.6 kg m −2 h −1 ), which can significantly contribute to the real‐world application of solar steam generation technology.
Publisher: Elsevier BV
Date: 03-2010
Publisher: Wiley
Date: 29-03-2010
Publisher: Springer Science and Business Media LLC
Date: 11-08-2017
DOI: 10.1038/S41598-017-08562-1
Abstract: Real-time measurement of the relative humidity of air has applications ranging from process control to safety. By using a microfiber form-factor, we demonstrate a miniature and fast-response hygrometer with the shortest-ever response time (3 ms). The sensor head consists of an optical microfiber of 10 µm diameter and 2 mm length configured to form a compact U-shaped probe, and functionalized with a polyelectrolyte multilayer coating of 1.0 bilayer. The sensing mechanism is primarily water-absorption-based optical loss. We have measured a response time of 3 ms and a recovery time of 36 ms. The sensitivity is as high as 0.4%/%RH, and the detection limit is as low as 1.6%RH. The maximum relative humidity is 99%RH, before reaching a recoverable dew-point.
Publisher: American Physical Society (APS)
Date: 27-07-2021
Publisher: American Association for the Advancement of Science (AAAS)
Date: 02-10-2020
Abstract: Poor water quality driven by increased nutrients is the main cause of coral ersity loss in southern China’s Greater Bay Area.
Publisher: American Chemical Society (ACS)
Date: 28-06-2006
DOI: 10.1021/JP061934Y
Abstract: Octahedral Cu(2)O crystals with tunable edge length were synthesized by reducing copper hydroxide with hydrazine without using any surfactant. Systematic experiments were carried out to investigate the factors which impact on the morphology and size of the products. The molar ratios of the reagents (NH(3):Cu(2+) and OH(-):Cu(2+)) determined the morphology and size of the corresponding products via affecting the coordination between NH(3) and Cu(2+). It is demonstrated that the ratio of growth rate along 111 versus 100 was varied by adjusting the molar ratio of NH(3) to Cu(2+), thus Cu(2)O crystals with different morphologies such as spheres, cubelike, and octahedra were obtained. The edge lengths of octahedra can be easily tuned from 130 to 600 nm by adjusting the molar ratio of OH(-) to Cu(2+). It is an effective and facile method for the controlled synthesis of octahedral Cu(2)O. The obtained octahedral Cu(2)O particles show improved ability on adsorption and photodegradation of methyl orange compared with cubic Cu(2)O particles.
Publisher: Elsevier BV
Date: 2014
Publisher: American Chemical Society (ACS)
Date: 03-10-2018
Abstract: The aim of this study was to test the performance of a novel method for acid rock drainage (ARD) control through the formation of Al(OH)
Publisher: Springer Science and Business Media LLC
Date: 02-2021
Abstract: A search for dark matter is conducted in final states containing a photon and missing transverse momentum in proton-proton collisions at $$ \\sqrt{s} $$ s = 13 TeV. The data, collected during 2015–2018 by the ATLAS experiment at the CERN LHC, correspond to an integrated luminosity of 139 fb − 1 . No deviations from the predictions of the Standard Model are observed and 95% confidence-level upper limits between 2.45 fb and 0.5 fb are set on the visible cross section for contributions from physics beyond the Standard Model, in different ranges of the missing transverse momentum. The results are interpreted as 95% confidence-level limits in models where weakly interacting dark-matter candidates are pair-produced via an s -channel axial-vector or vector mediator. Dark-matter candidates with masses up to 415 (580) GeV are excluded for axial-vector (vector) mediators, while the maximum excluded mass of the mediator is 1460 (1470) GeV. In addition, the results are expressed in terms of 95% confidence-level limits on the parameters of a model with an axion-like particle produced in association with a photon, and are used to constrain the coupling g a Z γ of an axion-like particle to the electroweak gauge bosons.
Publisher: American Chemical Society (ACS)
Date: 29-08-2008
DOI: 10.1021/CG800077H
Publisher: Springer Science and Business Media LLC
Date: 12-2021
Abstract: The fragmentation properties of jets containing b -hadrons are studied using charged B mesons in 139 fb − 1 of pp collisions at $$ \\sqrt{s} $$ s = 13 TeV, recorded with the ATLAS detector at the LHC during the period from 2015 to 2018. The B mesons are reconstructed using the decay of B ± into J/ψK ± , with the J/ψ decaying into a pair of muons. Jets are reconstructed using the anti- k t algorithm with radius parameter R = 0 . 4. The measurement determines the longitudinal and transverse momentum profiles of the reconstructed B hadrons with respect to the axes of the jets to which they are geometrically associated. These distributions are measured in intervals of the jet transverse momentum, ranging from 50 GeV to above 100 GeV. The results are corrected for detector effects and compared with several Monte Carlo predictions using different parton shower and hadronisation models. The results for the longitudinal and transverse profiles provide useful inputs to improve the description of heavy-flavour fragmentation in jets.
Publisher: American Physical Society (APS)
Date: 19-08-2021
Publisher: IOP Publishing
Date: 27-06-2006
Publisher: Elsevier BV
Date: 11-2023
Publisher: Springer Science and Business Media LLC
Date: 07-2021
Abstract: This article presents a new set of proton parton distribution functions, ATLASepWZVjet20, produced in an analysis at next-to-next-to-leading order in QCD. The new data sets considered are the measurements of W + and W − boson and Z boson production in association with jets in pp collisions at $$ \\sqrt{s} $$ s = 8 TeV performed by the ATLAS experiment at the LHC with integrated luminosities of 20 . 2 fb − 1 and 19 . 9 fb − 1 , respectively. The analysis also considers the ATLAS measurements of differential W ± and Z boson production at $$ \\sqrt{s} $$ s = 7 TeV with an integrated luminosity of 4 . 6 fb − 1 and deep-inelastic-scattering data from e ± p collisions at the HERA accelerator. An improved determination of the sea-quark densities at high Bjorken x is shown, while confirming a strange-quark density similar in size to the up- and down-sea-quark densities in the range x ≲ 0 . 02 found by previous ATLAS analyses.
Publisher: Royal Society of Chemistry (RSC)
Date: 2013
DOI: 10.1039/C3RA43929A
Publisher: Springer Science and Business Media LLC
Date: 04-11-2020
Publisher: American Chemical Society (ACS)
Date: 08-01-2016
Abstract: Herein we report a simple and substrate-independent approach to fabricate transparent oil-repellent coatings, which involves alternate deposition of poly(diallyldimethylammonium) (PDDA) and poly(styrenesulfonate) (PSS) onto substrates, followed by incubation of the coated objects into perfluorooctanoate (PFO) aqueous solutions for 2 min. Various low-surface-tension liquids can easily slide down the coating surfaces on flat substrates at a sliding angle lower than 12° for 10 μL droplets. The coatings are applicable to different substrates including Si, glass, plastic, steel, and wood, and those with complex shapes and large surface areas. They are also applicable to rough substrates with roughness at both micro/nanoscale and macroscopic scales to realize the easy-sliding oil repellency. Incubation of the PDDA/PSS polyelectrolyte multilayers (PEMs) into PFO solutions induces an effective but nondestructive substitution of PFO anions for PSS in the PEMs, which results in a composite coating with PFO anions homogeneously interspersed in both the coating surface and the bulk. Thanks to the as-described "repeating-layer" composition/structure of the coatings, their easy-sliding oil repellency can be self-healed after surface decomposition or well maintained after physical damages, due to the replenishing surface. Therefore, the advantageous characteristics of the as-developed oil-repellent coatings and the simplicity of the preparation protocol make the coatings highly practical for real-world applications. It is believed that the coatings can perform as antismudge coatings that shield against oil-borne contaminants, chemical-shield coatings that protect coated plastics from dissolution by organic solvents, and nonstick coatings (of oil tankers or pipelines) that enable loss-free oil transportation.
Publisher: Elsevier BV
Date: 12-2020
Publisher: Springer Science and Business Media LLC
Date: 2021
Abstract: A measurement of event-shape variables in proton-proton collisions at large momentum transfer is presented using data collected at $$ \\sqrt{s} $$ s = 13 TeV with the ATLAS detector at the Large Hadron Collider. Six event-shape variables calculated using hadronic jets are studied in inclusive multijet events using data corresponding to an integrated luminosity of 139 fb − 1 . Measurements are performed in bins of jet multiplicity and in different ranges of the scalar sum of the transverse momenta of the two leading jets, reaching scales beyond 2 TeV. These measurements are compared with predictions from Monte Carlo event generators containing leading-order or next-to-leading order matrix elements matched to parton showers simulated to leading-logarithm accuracy. At low jet multiplicities, shape discrepancies between the measurements and the Monte Carlo predictions are observed. At high jet multiplicities, the shapes are better described but discrepancies in the normalisation are observed.
Publisher: Elsevier BV
Date: 09-2020
Publisher: American Chemical Society (ACS)
Date: 27-09-2013
DOI: 10.1021/JP4067789
Publisher: Royal Society of Chemistry (RSC)
Date: 2020
DOI: 10.1039/D0CC03566A
Abstract: A cell-inspired microreactor can modulate the phase-oriented transport of reagents at interfaces, affording a powerful tool to optimize reaction selectivity.
Publisher: Royal Society of Chemistry (RSC)
Date: 2018
DOI: 10.1039/C8SC00678D
Abstract: Unconventionally, by placing hydrophilic particles in an oil phase before emulsification, the energy barrier is successfully eliminated and Pickering emulsions are easily formed.
Publisher: American Physical Society (APS)
Date: 26-07-2021
Publisher: Royal Society of Chemistry (RSC)
Date: 2015
DOI: 10.1039/C4CC08489F
Abstract: The polydopamine carrier causes the enrichment of methylene blue toward its surface, leading to the improved catalytic performance of the carried Au nanoparticles.
Publisher: Wiley
Date: 28-01-2022
Abstract: Solar anti‐/deicing can solve icing problems by converting sunlight into heat. One of the biggest problems, which has long been plaguing the design of solar anti‐/deicing surfaces, is that photothermal materials are always lightproof and appear black, because of the mutual exclusiveness between generating heat and retaining transparency. Herein, a highly transparent and scalable solar anti‐/deicing surface is reported, which enables the coated glass to exhibit high transparency ( % transmittance at 550 nm) and meanwhile causes a °C surface temperature increase relative to the ambient environment under 1.0 sun illumination. Such a transparent anti‐/deicing surface can be fabricated onto a large class of substrates (e.g., glass, ceramics, metals, plastics), by applying a solid omniphobic slippery coating onto layer‐by‐layer‐assembled ultrathin MXene multilayers. Hence, the surface possesses a self‐cleaning ability to shed waterborne and oil‐based liquids thanks to residue‐free slipping motion. Passive anti‐icing and active deicing capabilities are, respectively, obtained on the solar thermal surface, which effectively prevents water from freezing and simultaneously melts pre‐formed ice and thick frost. The self‐cleaning effect enables residue‐free removal of unfrozen water and interfacially melted ice/frost to boost the anti‐/deicing efficiency. Importantly, the surface is capable of self‐healing under illumination to repair physical damage and chemical degradation.
Publisher: Elsevier BV
Date: 08-2022
Publisher: Springer Science and Business Media LLC
Date: 03-2021
Abstract: A search is presented for the production of the Standard Model Higgs boson in association with a high-energy photon. With a focus on the vector-boson fusion process and the dominant Higgs boson decay into b -quark pairs, the search benefits from a large reduction of multijet background compared to more inclusive searches. Results are reported from the analysis of 132 fb − 1 of pp collision data at $$ \\sqrt{s} $$ s = 13 TeV collected with the ATLAS detector at the LHC. The measured Higgs boson signal yield in this final-state signature is 1 . 3 ± 1 . 0 times the Standard Model prediction. The observed significance of the Higgs boson signal above the background is 1 . 3 standard deviations, compared to an expected significance of 1 . 0 standard deviations.
Publisher: Springer Science and Business Media LLC
Date: 02-2021
DOI: 10.1140/EPJC/S10052-020-08734-W
Abstract: Differential cross-section measurements are presented for the electroweak production of two jets in association with a Z boson. These measurements are sensitive to the vector-boson fusion production mechanism and provide a fundamental test of the gauge structure of the Standard Model. The analysis is performed using proton–proton collision data collected by ATLAS at $$\\sqrt{s}=13\\ \\hbox {TeV}$$ s = 13 TeV and with an integrated luminosity of $$139\\ \\hbox {fb}^{-1}$$ 139 fb - 1 . The differential cross-sections are measured in the $$Z\\rightarrow \\ell ^+\\ell ^-$$ Z → ℓ + ℓ - decay channel ( $$\\ell =e,\\mu $$ ℓ = e , μ ) as a function of four observables: the dijet invariant mass, the rapidity interval spanned by the two jets, the signed azimuthal angle between the two jets, and the transverse momentum of the dilepton pair. The data are corrected for the effects of detector inefficiency and resolution and are sufficiently precise to distinguish between different state-of-the-art theoretical predictions calculated using Powheg+Pythia8 , Herwig7+Vbfnlo and Sherpa 2.2. The differential cross-sections are used to search for anomalous weak-boson self-interactions using a dimension-six effective field theory. The measurement of the signed azimuthal angle between the two jets is found to be particularly sensitive to the interference between the Standard Model and dimension-six scattering litudes and provides a direct test of charge-conjugation and parity invariance in the weak-boson self-interactions.
Publisher: Chinese Chemical Society
Date: 08-2020
Publisher: Springer Science and Business Media LLC
Date: 08-2021
DOI: 10.1140/EPJC/S10052-021-09402-3
Abstract: Jet energy scale and resolution measurements with their associated uncertainties are reported for jets using 36–81 fb $$^{-1}$$ - 1 of proton–proton collision data with a centre-of-mass energy of $$\sqrt{s}=13$$ s = 13 $${\text {Te}}{\text {V}}$$ TeV collected by the ATLAS detector at the LHC. Jets are reconstructed using two different input types: topo-clusters formed from energy deposits in calorimeter cells, as well as an algorithmic combination of charged-particle tracks with those topo-clusters, referred to as the ATLAS particle-flow reconstruction method. The anti- $$k_t$$ k t jet algorithm with radius parameter $$R=0.4$$ R = 0.4 is the primary jet definition used for both jet types. This result presents new jet energy scale and resolution measurements in the high pile-up conditions of late LHC Run 2 as well as a full calibration of particle-flow jets in ATLAS. Jets are initially calibrated using a sequence of simulation-based corrections. Next, several in situ techniques are employed to correct for differences between data and simulation and to measure the resolution of jets. The systematic uncertainties in the jet energy scale for central jets ( $$|\eta | .2$$ | η | 1.2 ) vary from 1% for a wide range of high- $$p_{{\text {T}}}$$ p T jets ( $$250 _{{\text {T}}} ~{\text {Ge}}{\text {V}}$$ 250 p T 2000 GeV ), to 5% at very low $$p_{{\text {T}}}$$ p T ( $$20~{\text {Ge}}{\text {V}}$$ 20 GeV ) and 3.5% at very high $$p_{{\text {T}}}$$ p T ( $$ .5~{\text {Te}}{\text {V}}$$ 2.5 TeV ). The relative jet energy resolution is measured and ranges from ( $$24 \pm 1.5$$ 24 ± 1.5 )% at 20 $${\text {Ge}}{\text {V}}$$ GeV to ( $$6 \pm 0.5$$ 6 ± 0.5 )% at 300 $${\text {Ge}}{\text {V}}$$ GeV .
Publisher: American Chemical Society (ACS)
Date: 07-12-2015
Publisher: American Chemical Society (ACS)
Date: 29-08-2008
DOI: 10.1021/CG800258N
Publisher: Royal Society of Chemistry (RSC)
Date: 2017
DOI: 10.1039/C6MH00317F
Abstract: A touchless control system that can be operated by a humidity signal is developed based on colorimetric humidity-sensitive materials.
Publisher: The Chemical Society of Japan
Date: 03-2006
DOI: 10.1246/CL.2006.264
Publisher: SPIE
Date: 23-04-2017
DOI: 10.1117/12.2263428
Publisher: American Chemical Society (ACS)
Date: 09-03-2020
Publisher: Elsevier BV
Date: 2021
Publisher: Wiley
Date: 14-03-2023
Abstract: Improving interfacial solar evaporation performance is crucial for the practical application of this technology in solar‐driven seawater desalination. Lowering evaporation enthalpy is one of the most promising and effective strategies to significantly improve solar evaporation rate. In this study, a new pathway to lower vaporization enthalpy by introducing heterogeneous interactions between hydrophilic hybrid materials and water molecules is developed. 2D MoN 1.2 nanosheets are synthesized and integrated with rGO nanosheets to form stacked MoN 1.2 ‐rGO heterostructures with massive junction interfaces for interfacial solar evaporation. Molecular dynamics simulation confirms that atomic thick 2D MoN 1.2 and rGO in the MoN 1.2 ‐rGO heterostructures simultaneously interact with water molecules, while the interactions are remarkably different. These heterogeneous interactions cause an imbalanced water state, which easily breaks the hydrogen bonds between water molecules, leading to dramatically lowered vaporization enthalpy and improved solar evaporation rate (2.6 kg m −2 h −1 ). This study provides a promising strategy for designing 2D‐2D heterostructures to regulate evaporation enthalpy to improve solar evaporate rate for clean water production.
Publisher: American Physical Society (APS)
Date: 27-12-2021
Publisher: American Chemical Society (ACS)
Date: 18-10-2006
DOI: 10.1021/CG060439O
Publisher: Elsevier BV
Date: 10-2019
Publisher: Royal Society of Chemistry (RSC)
Date: 2022
DOI: 10.1039/D2TA03004G
Abstract: An affordable and easy-to-fabricate solar evaporation-based crystallizer (SEC) was developed to implement interfacial brine evaporation towards zero liquid discharge (ZLD).
Publisher: Wiley
Date: 11-05-2021
Abstract: Present one‐step N 2 fixation is impeded by tough activation of the N≡N bond and low selectivity to NH 3 . Here we report fixation of N 2 ‐to‐NH 3 can be decoupled to a two‐step process with one problem effectively solved in each step, including: 1) facile activation of N 2 to NO x − by a non‐thermal plasma technique, and 2) highly selective conversion of NO x − to NH 3 by electrocatalytic reduction. Importantly, this process uses air and water as low‐cost raw materials for scalable ammonia production under ambient conditions. For NO x − reduction to NH 3 , we present a surface boron‐rich core–shell nickel boride electrocatalyst. The surface boron‐rich feature is the key to boosting activity, selectivity, and stability via enhanced NO x − adsorption, and suppression of hydrogen evolution and surface Ni oxidation. A significant ammonia production of 198.3 μmol cm −2 h −1 was achieved, together with nearly 100 % Faradaic efficiency.
Publisher: Wiley
Date: 15-11-2022
Abstract: Photocatalytic performance can be optimized via introduction of reactive sites. However, it is practically difficult to engineer these on specific photocatalyst surfaces, because of limited understanding of atomic‐level structure‐activity. Here we report a facile sonication‐assisted chemical reduction for specific facets regulation via oxygen deprivation on Bi‐based photocatalysts. The modified Bi 2 MoO 6 nanosheets exhibit 61.5 and 12.4 μmol g −1 for CO and CH 4 production respectively, ≈3 times greater than for pristine catalyst, together with excellent stability/reproducibility of ≈20 h. By combining advanced characterizations and simulation, we confirm the reaction mechanism on surface‐regulated photocatalysts, namely, induced defects on highly‐active surface accelerate charge separation/transfer and lower the energy barrier for surface CO 2 adsorption/activation/reduction. Promisingly, this method appears generalizable to a wider range of materials.
Publisher: Tsinghua University Press
Date: 06-2023
Publisher: American Chemical Society (ACS)
Date: 06-06-2016
Publisher: Royal Society of Chemistry (RSC)
Date: 2020
DOI: 10.1039/D0TA08539A
Abstract: An interfacial gelation coating method is developed to selectively coat photothermal materials on 3D substrate surfaces which dramatically reduces the consumption of photothermal materials while delivering superior performance in solar evaporation.
Publisher: Royal Society of Chemistry (RSC)
Date: 2013
DOI: 10.1039/C3CC46738D
Abstract: Janus-like emulsions stabilized by OH(-) and polydopamine (PDA) particles were realized. The OH(-) and particle occupied areas on emulsion droplet surfaces are spatially separated. Via controlling the pH and ionic strength, the coalescence of Janus-like emulsion droplets could be manipulated.
Publisher: Springer Science and Business Media LLC
Date: 31-01-2017
DOI: 10.1038/SREP41895
Abstract: We present a new type of fiber-coupled photodetector with a thermal-based optical sensor head, which enables it to operate even in the presence of strong electro-magnetic interference and in electrically sensitive environments. The optical sensor head consists of three cascaded Fabry-Perot interferometers. The end-face surface is coated with copper-oxide micro-particles embedded in hydrogel, which is a new photo-thermal coating that can be readily coated on many different surfaces. Under irradiation, photons are absorbed by the photo-thermal coating, and are converted into heat, changing the optical path length of the probing light and induces a resonant wavelength shift. For white-light irradiation, the photodetector exhibits a power sensitivity of 760 pm/mW, a power detection limit of 16.4 μW (i.e. specific detectivity of 2.2 × 10 5 cm.√Hz/W), and an optical damage threshold of ~100 mW or ~800 mW/cm 2 . The response and recovery times are 3.0 s (~90% of change within 100 ms) and 16.0 s respectively.
Publisher: American Physical Society (APS)
Date: 31-08-2021
Publisher: Springer Science and Business Media LLC
Date: 02-2021
DOI: 10.1140/EPJC/S10052-020-08677-2
Abstract: Measurements of the Standard Model Higgs boson decaying into a $$b\\bar{b}$$ b b ¯ pair and produced in association with a W or Z boson decaying into leptons, using proton–proton collision data collected between 2015 and 2018 by the ATLAS detector, are presented. The measurements use collisions produced by the Large Hadron Collider at a centre-of-mass energy of $$\\sqrt{s} = 13\\,\\text {Te}\\text {V}$$ s = 13 Te , corresponding to an integrated luminosity of $$139\\,\\mathrm {fb}^{-1}$$ 139 fb - 1 . The production of a Higgs boson in association with a W or Z boson is established with observed (expected) significances of 4.0 (4.1) and 5.3 (5.1) standard deviations, respectively. Cross-sections of associated production of a Higgs boson decaying into bottom quark pairs with an electroweak gauge boson, W or Z , decaying into leptons are measured as a function of the gauge boson transverse momentum in kinematic fiducial volumes. The cross-section measurements are all consistent with the Standard Model expectations, and the total uncertainties vary from 30% in the high gauge boson transverse momentum regions to 85% in the low regions. Limits are subsequently set on the parameters of an effective Lagrangian sensitive to modifications of the WH and ZH processes as well as the Higgs boson decay into $$b\\bar{b}$$ b b ¯ .
Publisher: American Chemical Society (ACS)
Date: 03-10-2008
DOI: 10.1021/JP805359R
Publisher: Wiley
Date: 07-11-2023
DOI: 10.1002/EOM2.12302
Abstract: Direct conversion of low‐grade heat into electricity by thermal electrochemical cells is a promising strategy for energy generation. For stable heat‐to‐electricity conversion, maintaining a low‐grade heat induced temperature difference between the cell electrodes is essential. Here, a thermogalvanic cell consisting of a cellulose fiber‐based porous aerogel, a liquid electrolyte, a reduced graphene oxide light absorber, and carbon nanotube‐based electrodes is designed for low‐grade thermal energy harvesting and conversion. The low thermal conductivity of the porous cellulose aerogel enables limited heat transfer from the hot side to the cold side, and thermal energy management effectively reduces heat loss from the hot side to the environment. Thus, a sustainable temperature difference between the electrodes is maintained and a corresponding maximum power output of 6.94 mW m −2 is achieved under natural solar irradiation. The obtained thermal electrochemical cells are also integrated into an enclosed interfacial solar evaporation device to harvest the latent heat released from vapor condensation for electricity generation. In addition, the thermal electrochemical cells can be regenerated after 18 months of storage and show no performance degradation. This design thus offers a novel alternative strategy for practical low‐grade heat harvesting. image
Publisher: Elsevier BV
Date: 04-2022
DOI: 10.1016/J.WATRES.2022.118099
Abstract: Interfacial solar steam generation is an efficient way to produce freshwater from saline water. This technology was further harnessed here for simultaneous saline soil remediation and enhanced agricultural sustainability. An interfacial solar evaporation and planting system was designed that uses treated seawater for saline soil washing and agricultural irrigation. In outdoor experiments the evaporator realized high freshwater production (10.95 kg m
Publisher: Elsevier BV
Date: 06-2019
Publisher: Elsevier BV
Date: 11-2019
Publisher: Springer Science and Business Media LLC
Date: 07-2021
Abstract: A search for long-lived particles, which have come to rest within the ATLAS detector, is presented. The subsequent decays of these particles can produce high-momentum jets, resulting in large out-of-time energy deposits in the ATLAS calorimeters. These de- cays are detected using data collected during periods in the LHC bunch structure when collisions are absent. The analysed dataset is composed of events from proton-proton collisions produced by the Large Hadron Collider at a centre-of-mass energy of $$ \\sqrt{s} $$ s = 13 TeV and recorded by the ATLAS experiment during 2017 and 2018. The dataset used for this search corresponds to a total live time of 579 hours. The results of this search are used to derive lower limits on the mass of gluino R -hadrons, assuming a branching fraction $$ \\mathcal{B}\\left(\\overset{\\sim }{g}\\to q\\overline{q}{\\chi}_1^0\\right) $$ B g ~ → q q ¯ χ 1 0 = 100%, with masses of up to 1 . 4 TeV excluded for gluino lifetimes of 10 − 5 to 10 3 s.
Publisher: AIP
Date: 2010
DOI: 10.1063/1.3505074
Publisher: Royal Society of Chemistry (RSC)
Date: 2018
DOI: 10.1039/C8TB00603B
Abstract: Novel robust and multifunctional polymer nanofilms were prepared through facile and highly efficient covalent layer-by-layer assembly.
Publisher: American Physical Society (APS)
Date: 10-2021
Publisher: American Physical Society (APS)
Date: 28-12-2021
Publisher: American Chemical Society (ACS)
Date: 13-05-2021
DOI: 10.1021/JACS.1C03135
Publisher: American Chemical Society (ACS)
Date: 09-12-2020
DOI: 10.1021/ACSSENSORS.9B01897
Abstract: A stronger absorption of pump robe light is desirable for maximizing the sensitivity to enable accurate measurements of trace chemical elements. We introduce a new sensing technique built on light-sheet excitation of skew rays in a multimode fiber with an additional enhancement of localized surface plasmon resonance (LSPR) and its evanescent-field hotspots between gold nanospheres on the coated fiber. A skewed light-sheet (i.e., a thin plane of light) can exploit the optimum ray group, producing enhanced and uniform interactions between light and matter for higher absorption/sensitivity and higher power threshold. The heightened evanescent field couples to the localized surface plasmon resonant modes to attain even greater sensitivity. We compared this excitation method with the previously demonstrated light-sheet skew ray-based sensor without LSPR and observed an enhancement in normalized attenuation of pump light up to seven orders of magnitude for low-concentration rhodamine B. The improvement in the normalized detection limit is almost three orders of magnitude. This new sensing technique uses a functionalized fiber rather than pairing a passive fiber with added functional particles in the analyte, which offers better area-selectivity. The potentially low-cost chemical sensors can be used on a range of sensing mechanisms such as pump robe light absorption.
Publisher: Elsevier BV
Date: 07-2022
Publisher: American Chemical Society (ACS)
Date: 10-08-2023
Publisher: American Chemical Society (ACS)
Date: 29-12-2020
Publisher: Wiley
Date: 09-02-2007
Publisher: Wiley
Date: 05-09-2021
DOI: 10.1002/EOM2.12140
Abstract: Interfacial solar steam generation is a green and sustainable technology which has been intensively studied in the fields of seawater desalination and wastewater purification for clean water production. Here, this technology is further developed for soil remediation. A new photothermal evaporator is designed to accelerate the extraction of lead (Pb) from soil solution, thereby successfully rapidly remediating a Pb contaminated soil. Within 2 weeks, this solar‐driven evaporative remediation (SDER) simultaneously decreases the bioavailable Pb fraction by 38.4% (from 359 to 221 mg kg −1 ) with no excessive nutrient loss nor secondary pollution. Post remediation plant assay indicates that the treated soil is significantly less phytotoxic, with shoot/root Pb contents decreasing by 50%. Since SDER involves no external energy input other than solar irradiation ongoing operating costs are low leading to significant potential for sustainable practical applications. Overall, this study demonstrates for the first time that interfacial solar evaporation can be successfully applied to soil remediation. image
Publisher: Elsevier BV
Date: 08-2006
Publisher: Wiley
Date: 03-09-2007
Abstract: The shape-controlled synthesis of nano- and microstructured materials has opened up new possibilities to improve their physical and chemical properties. In this work, new types of Bi(2)WO(6) with complex morphologies, namely, flowerlike, tyre- and helixlike, and platelike shapes, have been controllably synthesized by a facile hydrothermal process. The benefits of the present work also stem from the first report on the transformation of Bi(2)WO(6) from three-dimensional (3D) flowerlike superstructures to 2D platelike structures, and on the formation of tyre- and helixlike Bi(2)WO(6) superstructures. UV/Vis absorption spectra show that the optical properties of Bi(2)WO(6) s les are relevant to their size and shape. More importantly, the photocatalytic activities of Bi(2)WO(6) nano- and microstructures are strongly dependent on their shape, size, and structure for the degradation of Rhodamine B (RhB) under visible-light irradiation. The reasons for the differences in the photocatalytic activities of these Bi(2)WO(6) nano- and microstructures are further investigated.
Publisher: Elsevier BV
Date: 05-2021
Start Date: 2012
End Date: 2014
Funder: Australian Research Council
View Funded ActivityStart Date: 2019
End Date: 2024
Funder: Australian Research Council
View Funded ActivityStart Date: 2009
End Date: 2010
Funder: Alexander von Humboldt Foundation
View Funded ActivityStart Date: 2022
End Date: 12-2025
Amount: $405,000.00
Funder: Australian Research Council
View Funded ActivityStart Date: 2020
End Date: 12-2023
Amount: $890,287.00
Funder: Australian Research Council
View Funded ActivityStart Date: 01-2012
End Date: 12-2015
Amount: $375,000.00
Funder: Australian Research Council
View Funded Activity