ORCID Profile
0000-0003-2065-4354
Current Organisations
Hubei University
,
Deakin University
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Publisher: Springer Science and Business Media LLC
Date: 07-10-2022
Publisher: Elsevier BV
Date: 2022
DOI: 10.1016/J.JHAZMAT.2021.126834
Abstract: Microplastic accumulation in agricultural soils can stress plants and affects quality of the products. Current research on the effects of microplastics on plants is not consistent and the underlying mechanisms are yet unknown. Here, the molecular mechanisms of the stress response were investigated via metabolomic and transcriptomic analyses of rice Oryza sativa L. II Y900 and XS123 under the exposure of polystyrene microplastics (PS-MPs) in a field study. Distinct responses were obtained in these two rice subspecies, showing decreased head rice yield by 10.62% in Y900 and increase by 6.35% in XS123. The metabolomics results showed that PS-MPs exposure inhibited 29.63% of the substance accumulation-related metabolic pathways and 43.25% of the energy expenditure-related metabolic pathways in the Y900 grains however, these related pathways were promoted in the XS123 grains. The transcriptomics results indicated that the expression of genes encoding proteins involved in the tricarboxylic acid cycle in the Y900 grains was inhibited, but it was enhanced in the XS123 grains. The XS123 subspecies could response against microplastic exposure stress through the metabolite accumulation and energy expenditure pathways, while the Y900 could not. The results provide insight into the perturbation of rice grains in farmlands with microplastics contamination.
Publisher: Elsevier BV
Date: 03-2019
DOI: 10.1016/J.ENVPOL.2018.11.066
Abstract: Predicting the translocation of organic contaminants to plants is crucial to ensure the quality of agricultural goods and assess the risk of human exposure through the food web. In this study, the performance of a modified plant uptake model was evaluated considering a number of chemicals, such as polycyclic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs) and polybrominated diphenyl ethers (PBDEs), with a range of physicochemical properties different plant species (Ipomoea aquatica Forsk (sw morning glory), Chrysanthemum coronarium L. (crown daisy), Zea mays L. (corn), Brassica rapa pekinensis (Chinese cabbage), Cucurbita moschata (pumpkin), Raphanus sativus L. (radish), Spinacia oleracea L. (spinach) and Capsicum annuum L. (pepper)) and different types of soil (paddy soil, laterite soil and black soil). The biases of predictions from a previously used partition-limited model were -76.4% to -99.9% relative to the measured concentrations. An overall transmission factor (α
Publisher: Elsevier BV
Date: 08-2014
Publisher: Elsevier BV
Date: 08-2016
DOI: 10.1016/J.CHEMOSPHERE.2016.04.113
Abstract: Under current retrospective risk assessment framework, the total concentrations of organic pollutants in soils have been employed as the standard for over 30 years. The total concentrations reflect the overall accumulation in soils but tend to be overly conservative for assessing the ecological risks, where the bioavailability plays an important role. In this study, the bioavailability of organic pollutants in soils was evaluated using a stepwise and tiered classification method, namely the sequential ultrasonic extraction procedure (SEUP). The water-soluble and acid-soluble fractions extracted by the SEUP were the bioavailable fractions. The reliability and environmental relevance of the speciation method were examined with representative organic pollutants using the root uptake methods and the semipermeable membrane devices (SPMDs). The plant uptake amounts corrected with weight were highly correlated with the bioavailable fractions (R(2) > 0.75). The amounts of the bioavailable fractions were negatively correlated with the logKow values (R(2) ranging from 0.71 to 0.77) of the organic pollutants and the contents of soil organic matter (R(2) ranging from 0.68 to 0.96). As a refinement of the current risk assessment framework, the SUEP that has proved to be a reliable and convenient is thus highly recommended for evaluating the bioavailability of organic pollutants in soils.
Publisher: Elsevier BV
Date: 02-2022
DOI: 10.1016/J.SCITOTENV.2021.150941
Abstract: Biological wastewater treatment generates a large quantity of sewage sludge that requires proper treatments. In this study, the biochar pyrolyzed by sludge conditioned with Fenton's reagent and lime (referred to as Fenton-lime system) was first used as an efficient silicon fertilizer for rice cultivation. When the pyrolysis temperature was 750 °C, the dissolved silicon and available silicon contents in biochar derived from sludge conditioned with Fenton-lime system were much higher than those in raw sludge derived biochar without conditioning (3.49 vs. 0.72, 77.25 vs. 2.33 mg/g dry solid, respectively). The enhanced available silicon content was attributed to the newly formed calcium aluminosilicate from the reactions between the added lime and silicon-rich phases in sludge. The rice cultivated with biochar derived from Fenton-lime conditioned sludge showed improved biomass of stem and root by 76.85% and 36.11%, respectively, compared to blank group without the addition of Si source. Heavy metals and the reactive oxygen species (ROS) accumulation in rice were not observed after a culture period of 30 days in the application of sludge-derived biochar as silicon fertilizer. This study provides a promising approach for sewage sludge recycling as an efficient silicon fertilizer in silicon-deficiency land.
Publisher: Elsevier BV
Date: 12-2023
Publisher: Springer Science and Business Media LLC
Date: 13-01-2022
DOI: 10.1007/S11356-022-18624-1
Abstract: Activated persulfate oxidation has been proven to be an efficient advanced sludge treatment technique to improve sludge dewaterability. This study investigates the influence of persulfate on the transformation of phosphorus (P) and heavy metals (HMs) during the hydrothermal treatment of sewage sludge. The hydrothermal temperature, time, and persulfate concentration are optimized by a Box-Behnken design to obtain the best sludge dewaterability, which is expressed by capillary suction time (CST). The highest CST reduction efficiency is 90.5% at the optimal hydrothermal temperature, time, and concentration of persulfate, which are 145 °C, 2 h, and 150 mg/g dry sludge (DS), respectively. The distribution and transformation of P and HMs with different persulfate concentrations (100-200 mg/g DS) during the hydrothermal process are investigated. Results show that more than 90% of the P and HMs in the sludge are retained in sludge cakes after the hydrothermal treatment. The addition of SPS can make the P in the sludge cakes transform into more stable P species according to the extraction capacity of sequential extracts. It can be found from the ecological risk indexes of the HMs that the addition of SPS during the hydrothermal treatment of sludge can reduce the environmental risk of HMs. This study provides insights into the P and HM distribution and transformation during hydrothermal treatment with persulfate, providing a reference for sludge recovery strategies.
Publisher: Elsevier BV
Date: 11-2020
Publisher: Elsevier BV
Date: 10-2021
Publisher: Elsevier BV
Date: 04-2021
Publisher: IWA Publishing
Date: 05-2013
DOI: 10.2166/WST.2013.072
Abstract: The material of this study is provided by biological aerobic treatment of high saline wastewater from pesticide production. The microorganism used for biodegradation has been identified by gene-sequencing as a strain of Bacillus sp. SCUN. The best growth condition for the salt-tolerant microorganism has been studied by varying the pH, immobilized microorganism dosage and temperature conditions. The feasibility of pretreating wastewater in ethyl chloride production containing 4% NaCl has been discussed. It was found that under the pH range of 6.0–8.0, immobilized microorganism dosage of 1.5 g/L, temperature of 30 °C, and NaCl concentration of 0–3%, the microorganism achieves the best growth for biodegradation. After domestication, the strain can grow under 4% NaCl. This salt-tolerant microorganism is effective in the pretreated high saline wastewater. With a newly developed ternary cycle treatment, the chemical oxygen demand removal approaches 58.3%. The theoretical basis and a new method for biological treatments in biodegradation of high saline wastewater in ethyl chloride production are discussed.
Publisher: Elsevier BV
Date: 09-2019
DOI: 10.1016/J.ENVINT.2019.06.002
Abstract: The prediction of toxicological interactions and hormesis of chemical mixtures is important because organisms are mostly exposed to numerous contaminants and typically to low dose of these mixtures, and it is still a challenge. Although many models have been developed to predict the mixture toxicities such as concentration addition (CA) and independent action (IA), they cannot solve these challenges perfectly. This study has developed an improved inverse distance weighted (IDW) interpolation for prediction of the mixture toxicities. IDW uses the mixture and the single compound as scatter points in space, and the space can be constructed by the concentration axes of various components in the mixture system. Some known mixtures (or the single compound) closest to the unknown mixture are selected as interpolation nodes. To be more accurate in calculation, a new normalization method for concentration has been proposed through iding the concentration of the mixture and the single compound by the respective EC
Publisher: Elsevier BV
Date: 09-2018
DOI: 10.1016/J.ENVPOL.2018.04.072
Abstract: The mechanism of enhanced accumulation of organic contaminants in crops with engineered nanomaterials (ENMs) were investigated by co-exposure of crops (Ipomoea aquatica Forsk (Sw morning-glory), Cucumis sativus L. (cucumber), Zea mays L. (corn), Spinacia oleracea L. (spinach) and Cucurbita moschata (pumpkin))to a range of chemicals (polycyclic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs) and polybrominated diphenyl ether (PBDE)) and ENMs (TiO
Publisher: Springer Science and Business Media LLC
Date: 06-02-2017
DOI: 10.1038/SREP42037
Abstract: Representative biomarkers (e.g., n -alkanes), ersity and microbial community in the aquifers contaminated by high concentration of arsenic (As) in different sediment depth (0–30 m) in Jianghan Plain, Hubei, China, were analyzed to investigate the potential mechanism of As enrichment in groundwater. The concentration of As was abundant in top soil and sand, but not in clay. The analysis of the distribution of n -alkanes, CPI values, and wax to total n -alkane ratio (Wax(n)%) indicated that the organic matter (OM) from fresh terrestrial plants were abundant in the shallow sediment. However, n -alkanes have suffered from significant biodegradation from the depth of 16 m to 30 m. The deposition of fresh terrestrial derived organic matters may facilitate the release of As from sediment to groundwater in the sediment of 0–16 m. However, the petroleum derived organic matters may do the favor to the release of As in the deeper section of borehole (16 m to 30 m). The 16S rRNA gene sequences identification indicated that Acidobacteria, Actinomycetes and Hydrogenophaga are abundant in the sediments with high arsenic. Therefore, microbes and organic matters from different sources may play important roles in arsenic mobilization in the aquifers of the study area.
No related grants have been discovered for Xiang Wu.